Cavity-control of interlayer excitons in van der Waals heterostructures
Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterob...
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| Published in | Nature communications Vol. 10; no. 1; pp. 3697 - 6 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
16.08.2019
Nature Publishing Group Nature Portfolio |
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| Abstract | Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe
2
-WSe
2
heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity – van der Waals heterostructure systems.
Cavity-enhanced light-matter interaction in the weak-coupling regime is known to result in Purcell enhancement. Here the authors demonstrate Purcell enhancement in the photoluminescence of vertical MoSe
2
-WSe
2
heterostructures coupled to a micro-cavity and determine the light-matter coupling strength for interlayer excitons. |
|---|---|
| AbstractList | Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe
2
-WSe
2
heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity – van der Waals heterostructure systems.
Cavity-enhanced light-matter interaction in the weak-coupling regime is known to result in Purcell enhancement. Here the authors demonstrate Purcell enhancement in the photoluminescence of vertical MoSe
2
-WSe
2
heterostructures coupled to a micro-cavity and determine the light-matter coupling strength for interlayer excitons. Abstract Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe 2 -WSe 2 heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity – van der Waals heterostructure systems. Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe -WSe heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity - van der Waals heterostructure systems. Cavity-enhanced light-matter interaction in the weak-coupling regime is known to result in Purcell enhancement. Here the authors demonstrate Purcell enhancement in the photoluminescence of vertical MoSe2-WSe2 heterostructures coupled to a micro-cavity and determine the light-matter coupling strength for interlayer excitons. Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing spatially indirect excitons with a permanent electric dipole moment in heterobilayer crystals promise realizations of exciton-polariton gases and condensates with inherent dipolar interactions. Here, we implement cavity-control of interlayer excitons in vertical MoSe2-WSe2 heterostructures. Our experiments demonstrate the Purcell effect for heterobilayer emission in cavity-modified photonic environments, and quantify the light-matter coupling strength of interlayer excitons. The results will facilitate further developments of dipolar exciton-polariton gases and condensates in hybrid cavity – van der Waals heterostructure systems. |
| ArticleNumber | 3697 |
| Author | Lindlau, Jessica Mohite, Aditya D. Högele, Alexander Patel, Robin K. Yamaguchi, Hisato Hunger, David Förg, Michael Colombier, Léo Glazov, Mikhail M. |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/31420540$$D View this record in MEDLINE/PubMed |
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| Snippet | Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling... Abstract Monolayer transition metal dichalcogenides integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter... Cavity-enhanced light-matter interaction in the weak-coupling regime is known to result in Purcell enhancement. Here the authors demonstrate Purcell... |
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| SubjectTerms | 639/766/119/1000/1018 639/925/357/1018 Chemical vapor deposition Condensates Coupling Crystals Dipole moments Electric dipoles Excitons Gases Heterostructures Humanities and Social Sciences Hybrid systems Interlayers Laboratories Light Microcavities multidisciplinary Photonics Polaritons Science Science (multidisciplinary) Spectrum analysis Transition metal compounds |
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| Title | Cavity-control of interlayer excitons in van der Waals heterostructures |
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