Small reorganization energy acceptors enable low energy losses in non-fullerene organic solar cells
Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy...
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| Published in | Nature communications Vol. 13; no. 1; pp. 3256 - 10 |
|---|---|
| Main Authors | , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
07.06.2022
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells.
Minimising energy loss is important for achieving high-performance organic solar cells. Here, the authors design and synthesise two acceptors with small reorganisation energies and reveal the relationship between reorganisation energy and energy losses. |
|---|---|
| AbstractList | Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells.Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells. Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells. Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells. Minimising energy loss is important for achieving high-performance organic solar cells. Here, the authors design and synthesise two acceptors with small reorganisation energies and reveal the relationship between reorganisation energy and energy losses. Minimising energy loss is important for achieving high-performance organic solar cells. Here, the authors design and synthesise two acceptors with small reorganisation energies and reveal the relationship between reorganisation energy and energy losses. Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a crucial role in photoelectric conversion processes. However, the understanding of the relationship between reorganization energy and energy losses has rarely been studied. Here, two acceptors, Qx-1 and Qx-2, were developed. The reorganization energies of these two acceptors during photoelectric conversion processes are substantially smaller than the conventional Y6 acceptor, which is beneficial for improving the exciton lifetime and diffusion length, promoting charge transport, and reducing the energy loss originating from exciton dissociation and non-radiative recombination. So, a high efficiency of 18.2% with high open circuit voltage above 0.93 V in the PM6:Qx-2 blend, accompanies a significantly reduced energy loss of 0.48 eV. This work underlines the importance of the reorganization energy in achieving small energy losses and paves a way to obtain high-performance organic solar cells.Minimising energy loss is important for achieving high-performance organic solar cells. Here, the authors design and synthesise two acceptors with small reorganisation energies and reveal the relationship between reorganisation energy and energy losses. |
| ArticleNumber | 3256 |
| Author | Hao, Xiaotao Liu, Yanan Adil, Muhammad Abdullah Shi, Yanan Ma, Wei Zhang, Jianqi Chang, Yilin Yan, Yangjun Zhu, Lingyun Lu, Kun Wei, Zhixiang Chen, Zhihao Qiu, Dingding |
| Author_xml | – sequence: 1 givenname: Yanan surname: Shi fullname: Shi, Yanan organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology, University of Chinese Academy of Sciences – sequence: 2 givenname: Yilin surname: Chang fullname: Chang, Yilin organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology, University of Chinese Academy of Sciences – sequence: 3 givenname: Kun orcidid: 0000-0002-3403-2516 surname: Lu fullname: Lu, Kun email: lvk@nanoctr.cn organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology, University of Chinese Academy of Sciences – sequence: 4 givenname: Zhihao surname: Chen fullname: Chen, Zhihao organization: School of Physics, State Key Laboratory of Crystal Materials, Shandong University – sequence: 5 givenname: Jianqi orcidid: 0000-0002-3549-1482 surname: Zhang fullname: Zhang, Jianqi organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology – sequence: 6 givenname: Yangjun surname: Yan fullname: Yan, Yangjun organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology – sequence: 7 givenname: Dingding surname: Qiu fullname: Qiu, Dingding organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology, University of Chinese Academy of Sciences – sequence: 8 givenname: Yanan surname: Liu fullname: Liu, Yanan organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology – sequence: 9 givenname: Muhammad Abdullah orcidid: 0000-0002-7658-5370 surname: Adil fullname: Adil, Muhammad Abdullah organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology – sequence: 10 givenname: Wei orcidid: 0000-0002-7239-2010 surname: Ma fullname: Ma, Wei organization: State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University – sequence: 11 givenname: Xiaotao orcidid: 0000-0002-0197-6545 surname: Hao fullname: Hao, Xiaotao email: haoxt@sdu.edu.cn organization: School of Physics, State Key Laboratory of Crystal Materials, Shandong University – sequence: 12 givenname: Lingyun orcidid: 0000-0001-7391-1866 surname: Zhu fullname: Zhu, Lingyun email: zhuly@nanoctr.cn organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology – sequence: 13 givenname: Zhixiang orcidid: 0000-0001-6188-3634 surname: Wei fullname: Wei, Zhixiang email: weizx@nanoctr.cn organization: Chinese Academy of Sciences (CAS) key laboratory of nanosystem and hierarchical fabrication, National Center for Nanoscience and Technology, University of Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/35672325$$D View this record in MEDLINE/PubMed |
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| Snippet | Minimizing energy loss is of critical importance in the pursuit of attaining high-performance organic solar cells. Interestingly, reorganization energy plays a... Minimising energy loss is important for achieving high-performance organic solar cells. Here, the authors design and synthesise two acceptors with small... |
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| SubjectTerms | 119/118 140/131 140/58 147/143 147/3 639/301/299/946 639/638/675 Charge transport Conversion Diffusion length Energy Energy loss Excitons Fullerenes Humanities and Social Sciences multidisciplinary Open circuit voltage Photoelectricity Photovoltaic cells Radiative recombination Recombination Science Science (multidisciplinary) Solar cells Solar energy |
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| Title | Small reorganization energy acceptors enable low energy losses in non-fullerene organic solar cells |
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