A Chiral Metal—Organic Framework Prepared on Large-Scale for Sensitive and Enantioselective Fluorescence Recognition
MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s...
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| Published in | Molecules (Basel, Switzerland) Vol. 28; no. 12; p. 4593 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
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MDPI AG
07.06.2023
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| Online Access | Get full text |
| ISSN | 1420-3049 1420-3049 |
| DOI | 10.3390/molecules28124593 |
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| Abstract | MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s-L)](NO3)2 (MOF-1), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF-1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF-1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. |
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| AbstractList | MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s-L)](NO3)2 (MOF-1), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF-1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF-1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd( s - L )](NO 3 ) 2 (MOF- 1 ), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF- 1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF- 1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s-L)](NO3)2 (MOF-1), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF-1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF-1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol.MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s-L)](NO3)2 (MOF-1), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF-1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF-1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd(s-L)](NO[sub.3])[sub.2] (MOF-1), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF-1 has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF-1 exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. MOF-based luminescent sensors have garnered considerable attention due to their potential in recognition and discrimination with high sensitivity, selectivity, and fast response in the last decades. Herein, this work describes the bulk preparation of a novel luminescent homochiral MOF, namely, [Cd( - )](NO ) (MOF- ), from an enantiopure pyridyl-functionalized ligand with rigid binaphthol skeleton under mild synthetic condition. Except for the features of porosity and crystallinity, the MOF- has also been characterized with water-stability, luminescence, and homochirality. Most important, the MOF- exhibits highly sensitive molecular recognition toward the4-nitrobenzoic acid (NBC) and moderate enantioselective detection of proline, arginine, and 1-phenylethanol. |
| Audience | Academic |
| Author | Kang, Yan-Shang Wu, Fang-Hui Zhang, Xin-Mei Xu, Fan Luo, Li Chen, Kai Bai, Yan-Mei Ai, Lu-Lu Shan, Wei-Long |
| AuthorAffiliation | 2 School of Chemistry and Life Sciences, Suzhou University of Science and Technology, Suzhou 215009, China 3 Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Nanjing University of Information Science & Technology, Nanjing 210044, China; catqchen@163.com 4 SJTU SMSE—Mingguang Joint Research Center for Advanced Palygoskite Materials, Mingguang Mingyao Attapulgite Industry Technology Co., Ltd., Chuzhou 239400, China; xufan921222@163.com 1 School of Chemistry and Chemical Engineering, Anhui University of Technology, Maanshan 243002, China; zxm13295603905@163.com (X.-M.Z.); bym1101074898@163.com (Y.-M.B.); a8156162496158@163.com (L.-L.A.); wfhwfh@ahut.edu.cn (F.-H.W.); wlshan@ahut.edu.cn (W.-L.S.) |
| AuthorAffiliation_xml | – name: 2 School of Chemistry and Life Sciences, Suzhou University of Science and Technology, Suzhou 215009, China – name: 3 Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Nanjing University of Information Science & Technology, Nanjing 210044, China; catqchen@163.com – name: 1 School of Chemistry and Chemical Engineering, Anhui University of Technology, Maanshan 243002, China; zxm13295603905@163.com (X.-M.Z.); bym1101074898@163.com (Y.-M.B.); a8156162496158@163.com (L.-L.A.); wfhwfh@ahut.edu.cn (F.-H.W.); wlshan@ahut.edu.cn (W.-L.S.) – name: 4 SJTU SMSE—Mingguang Joint Research Center for Advanced Palygoskite Materials, Mingguang Mingyao Attapulgite Industry Technology Co., Ltd., Chuzhou 239400, China; xufan921222@163.com |
| Author_xml | – sequence: 1 givenname: Xin-Mei surname: Zhang fullname: Zhang, Xin-Mei – sequence: 2 givenname: Yan-Mei surname: Bai fullname: Bai, Yan-Mei – sequence: 3 givenname: Lu-Lu surname: Ai fullname: Ai, Lu-Lu – sequence: 4 givenname: Fang-Hui surname: Wu fullname: Wu, Fang-Hui – sequence: 5 givenname: Wei-Long surname: Shan fullname: Shan, Wei-Long – sequence: 6 givenname: Yan-Shang surname: Kang fullname: Kang, Yan-Shang – sequence: 7 givenname: Li surname: Luo fullname: Luo, Li – sequence: 8 givenname: Kai surname: Chen fullname: Chen, Kai – sequence: 9 givenname: Fan surname: Xu fullname: Xu, Fan |
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| CitedBy_id | crossref_primary_10_1016_j_microc_2024_110974 crossref_primary_10_1002_chem_202400071 crossref_primary_10_1002_chem_202401091 crossref_primary_10_1021_acs_inorgchem_4c05262 crossref_primary_10_1039_D4TC03506B |
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| Keywords | enantioselectivity chiral recognition luminescence chiral metal-organic framework amino acid |
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| SubjectTerms | amino acid Aqueous solutions chiral metal-organic framework chiral recognition Communication enantioselectivity Fluorescence Ligands luminescence Pollutants Single crystals Solvents Spectrum analysis Water pollution |
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| Title | A Chiral Metal—Organic Framework Prepared on Large-Scale for Sensitive and Enantioselective Fluorescence Recognition |
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