Mesoporous Carbon Nanocube Architecture for High-Performance Lithium-Oxygen Batteries
One of the major challenges to develop high‐performance lithium–oxygen (Li–O2) battery is to find effective cathode catalysts and design porous architecture for the promotion of both oxygen reduction reactions and oxygen evolution reactions. Herein, the synthesis of mesoporous carbon nanocubes as a...
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| Published in | Advanced functional materials Vol. 25; no. 28; pp. 4436 - 4444 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Blackwell Publishing Ltd
01.07.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | One of the major challenges to develop high‐performance lithium–oxygen (Li–O2) battery is to find effective cathode catalysts and design porous architecture for the promotion of both oxygen reduction reactions and oxygen evolution reactions. Herein, the synthesis of mesoporous carbon nanocubes as a new cathode nanoarchitecture for Li–O2 batteries is reported. The oxygen electrodes made of mesoporous carbon nanocubes contain numerously hierarchical mesopores and macropores, which can facilitate oxygen diffusion and electrolyte impregnation throughout the electrode, and provide sufficient spaces to accommodate insoluble discharge products. When they are applied as cathode catalysts, the Li–O2 cells deliver discharge capacities of 26 100 mA h g−1 at 200 mA g−1, which is much higher than that of commercial carbon black catalysts. Furthermore, the mesoporous nanocube architecture can also serve as a conductive host structure for other highly efficient catalysts. For instance, the Ru functionalized mesoporous carbon nanocubes show excellent catalytic activities toward oxygen evolution reactions. Li–O2 batteries with Ru functionalized mesoporous carbon nanocube catalysts demonstrate a high charge/discharge electrical energy efficiency of 86.2% at 200 mA g−1 under voltage limitation and a good cycling performance up to 120 cycles at 400 mA g−1 with the curtaining capacity of 1000 mA h g−1.
Mesoporous carbon nanocubes (MCCs) are synthesized by a chemical vapor deposition method. Oxygen electrode made of MCCs contains a hierarchical porous structure, which can facilitate oxygen diffusion, electrolyte impregnation, and accommodation of discharge products during the charge and discharge processes. |
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| AbstractList | One of the major challenges to develop high-performance lithium-oxygen (Li-O sub(2)) battery is to find effective cathode catalysts and design porous architecture for the promotion of both oxygen reduction reactions and oxygen evolution reactions. Herein, the synthesis of mesoporous carbon nanocubes as a new cathode nanoarchitecture for Li-O sub(2) batteries is reported. The oxygen electrodes made of mesoporous carbon nanocubes contain numerously hierarchical mesopores and macropores, which can facilitate oxygen diffusion and electrolyte impregnation throughout the electrode, and provide sufficient spaces to accommodate insoluble discharge products. When they are applied as cathode catalysts, the Li-O sub(2) cells deliver discharge capacities of 26 100 mA h g super(-1) at 200 mA g super(-1), which is much higher than that of commercial carbon black catalysts. Furthermore, the mesoporous nanocube architecture can also serve as a conductive host structure for other highly efficient catalysts. For instance, the Ru functionalized mesoporous carbon nanocubes show excellent catalytic activities toward oxygen evolution reactions. Li-O sub(2) batteries with Ru functionalized mesoporous carbon nanocube catalysts demonstrate a high charge/discharge electrical energy efficiency of 86.2% at 200 mA g super(-1) under voltage limitation and a good cycling performance up to 120 cycles at 400 mA g super(-1) with the curtaining capacity of 1000 mA h g super(-1). Mesoporous carbon nanocubes (MCCs) are synthesized by a chemical vapor deposition method. Oxygen electrode made of MCCs contains a hierarchical porous structure, which can facilitate oxygen diffusion, electrolyte impregnation, and accommodation of discharge products during the charge and discharge processes. One of the major challenges to develop high‐performance lithium–oxygen (Li–O2) battery is to find effective cathode catalysts and design porous architecture for the promotion of both oxygen reduction reactions and oxygen evolution reactions. Herein, the synthesis of mesoporous carbon nanocubes as a new cathode nanoarchitecture for Li–O2 batteries is reported. The oxygen electrodes made of mesoporous carbon nanocubes contain numerously hierarchical mesopores and macropores, which can facilitate oxygen diffusion and electrolyte impregnation throughout the electrode, and provide sufficient spaces to accommodate insoluble discharge products. When they are applied as cathode catalysts, the Li–O2 cells deliver discharge capacities of 26 100 mA h g−1 at 200 mA g−1, which is much higher than that of commercial carbon black catalysts. Furthermore, the mesoporous nanocube architecture can also serve as a conductive host structure for other highly efficient catalysts. For instance, the Ru functionalized mesoporous carbon nanocubes show excellent catalytic activities toward oxygen evolution reactions. Li–O2 batteries with Ru functionalized mesoporous carbon nanocube catalysts demonstrate a high charge/discharge electrical energy efficiency of 86.2% at 200 mA g−1 under voltage limitation and a good cycling performance up to 120 cycles at 400 mA g−1 with the curtaining capacity of 1000 mA h g−1. Mesoporous carbon nanocubes (MCCs) are synthesized by a chemical vapor deposition method. Oxygen electrode made of MCCs contains a hierarchical porous structure, which can facilitate oxygen diffusion, electrolyte impregnation, and accommodation of discharge products during the charge and discharge processes. One of the major challenges to develop high‐performance lithium–oxygen (Li–O 2 ) battery is to find effective cathode catalysts and design porous architecture for the promotion of both oxygen reduction reactions and oxygen evolution reactions. Herein, the synthesis of mesoporous carbon nanocubes as a new cathode nanoarchitecture for Li–O 2 batteries is reported. The oxygen electrodes made of mesoporous carbon nanocubes contain numerously hierarchical mesopores and macropores, which can facilitate oxygen diffusion and electrolyte impregnation throughout the electrode, and provide sufficient spaces to accommodate insoluble discharge products. When they are applied as cathode catalysts, the Li–O 2 cells deliver discharge capacities of 26 100 mA h g −1 at 200 mA g −1 , which is much higher than that of commercial carbon black catalysts. Furthermore, the mesoporous nanocube architecture can also serve as a conductive host structure for other highly efficient catalysts. For instance, the Ru functionalized mesoporous carbon nanocubes show excellent catalytic activities toward oxygen evolution reactions. Li–O 2 batteries with Ru functionalized mesoporous carbon nanocube catalysts demonstrate a high charge/discharge electrical energy efficiency of 86.2% at 200 mA g −1 under voltage limitation and a good cycling performance up to 120 cycles at 400 mA g −1 with the curtaining capacity of 1000 mA h g −1 . |
| Author | Liu, Hao Chen, Shuangqiang Wang, Guoxiu Sun, Bing |
| Author_xml | – sequence: 1 givenname: Bing surname: Sun fullname: Sun, Bing organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway, NSW, 2007, Sydney, Australia – sequence: 2 givenname: Shuangqiang surname: Chen fullname: Chen, Shuangqiang organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway, NSW, 2007, Sydney, Australia – sequence: 3 givenname: Hao surname: Liu fullname: Liu, Hao organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway, NSW, 2007, Sydney, Australia – sequence: 4 givenname: Guoxiu surname: Wang fullname: Wang, Guoxiu email: guoxiu.wang@uts.edu.au organization: Centre for Clean Energy Technology, University of Technology Sydney, Broadway, 2007, Sydney, NSW, Australia |
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| Snippet | One of the major challenges to develop high‐performance lithium–oxygen (Li–O2) battery is to find effective cathode catalysts and design porous architecture... One of the major challenges to develop high‐performance lithium–oxygen (Li–O 2 ) battery is to find effective cathode catalysts and design porous architecture... One of the major challenges to develop high-performance lithium-oxygen (Li-O sub(2)) battery is to find effective cathode catalysts and design porous... |
| SourceID | proquest crossref wiley istex |
| SourceType | Aggregation Database Enrichment Source Index Database Publisher |
| StartPage | 4436 |
| SubjectTerms | Architecture Carbon Catalysis Catalysts cathode catalysts Cathodes Discharge Electrodes lithium-oxygen batteries mesoporous carbon nanocubes Nanostructure ruthenium nanocrystals |
| Title | Mesoporous Carbon Nanocube Architecture for High-Performance Lithium-Oxygen Batteries |
| URI | https://api.istex.fr/ark:/67375/WNG-K6SHLTMP-L/fulltext.pdf https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadfm.201500863 https://www.proquest.com/docview/1718974814 |
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