Renewable resource-based composites of recycled natural fibers and maleated polylactide bioplastic: Characterization and biodegradability

The thermal properties of composite materials composed of polylactide (PLA) and green coconut fiber (GCF) were evaluated. Blends containing maleic anhydride-grafted PLA (PLA-g-MA/GCF) exhibited noticeably superior thermal properties due to greater compatibility between the two components. The disper...

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Published in	Polymer degradation and stability Vol. 94; no. 7; pp. 1076 - 1084
Main Author	Wu, Chin-San
Format	Journal Article
Language	English
Published	Kidlington Elsevier Ltd 01.07.2009 Elsevier
Subjects	Applied sciences Biodegradation Blend Burkholderia cepacia Coconut Exact sciences and technology Fibers and threads Forms of application and semi-finished materials Polylactide Polymer industry, paints, wood Technology of polymers Biodegradation Blend Polylactide Coconut Biological properties Lactone copolymer Biodegradability Lactic acid copolymer Intrinsic viscosity Fiber reinforced material Plant fiber Coconut fiber Organic anhydride Experimental study Lactone polymer Functional polymer Composite material Thermal properties Lactic acid polymer Natural fiber Aliphatic polymer Concentration effect Water absorption Rheological properties
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Abstract	The thermal properties of composite materials composed of polylactide (PLA) and green coconut fiber (GCF) were evaluated. Blends containing maleic anhydride-grafted PLA (PLA-g-MA/GCF) exhibited noticeably superior thermal properties due to greater compatibility between the two components. The dispersion of GCF in the PLA-g-MA matrix was highly homogeneous as a result of ester formation, and the consequent creation of branched and cross-linked macromolecules, between the carboxyl groups of PLA-g-MA and the hydroxyl groups in GCF. In addition, the PLA-g-MA/GCF blend was more easily processed due to a lower melt viscosity. Each composite was subject to biodegradation tests in a Burkholderia cepacia BCRC 14253 compost. The bacterium completely degraded both the PLA and the PLA-g-MA/GCF composite films. Morphological observations indicated severe disruption of the film structure after 9–12 days of incubation. The PLA-g-MA/GCF (10 wt%) films were not only more biodegradable than those made of PLA, but also exhibited lower molecular weight and intrinsic viscosity, implying a strong connection between these characteristics and biodegradability.
AbstractList	The thermal properties of composite materials composed of polylactide (PLA) and green coconut fiber (GCF) were evaluated. Blends containing maleic anhydride-grafted PLA (PLA-g-MA/GCF) exhibited noticeably superior thermal properties due to greater compatibility between the two components. The dispersion of GCF in the PLA-g-MA matrix was highly homogeneous as a result of ester formation, and the consequent creation of branched and cross-linked macromolecules, between the carboxyl groups of PLA-g-MA and the hydroxyl groups in GCF. In addition, the PLA-g-MA/GCF blend was more easily processed due to a lower melt viscosity. Each composite was subject to biodegradation tests in a Burkholderia cepacia BCRC 14253 compost. The bacterium completely degraded both the PLA and the PLA-g-MA/GCF composite films. Morphological observations indicated severe disruption of the film structure after 9–12 days of incubation. The PLA-g-MA/GCF (10 wt%) films were not only more biodegradable than those made of PLA, but also exhibited lower molecular weight and intrinsic viscosity, implying a strong connection between these characteristics and biodegradability. The thermal properties of composite materials composed of polylactide (PLA) and green coconut fiber (GCF) were evaluated. Blends containing maleic anhydride-grafted PLA (PLA-g-MA/GCF) exhibited noticeably superior thermal properties due to greater compatibility between the two components. The dispersion of GCF in the PLA-g-MA matrix was highly homogeneous as a result of ester formation, and the consequent creation of branched and cross-linked macromolecules, between the carboxyl groups of PLA-g-MA and the hydroxyl groups in GCF. In addition, the PLA-g-MA/GCF blend was more easily processed due to a lower melt viscosity. Each composite was subject to biodegradation tests in a Burkholderia cepacia BCRC 14253 compost. The bacterium completely degraded both the PLA and the PLA-g-MA/GCF composite films. Morphological observations indicated severe disruption of the film structure after 9-12 days of incubation. The PLA-g-MA/GCF (10 wt%) films were not only more biodegradable than those made of PLA, but also exhibited lower molecular weight and intrinsic viscosity, implying a strong connection between these characteristics and biodegradability.
Author	Wu, Chin-San
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Keywords	Biodegradation Blend Polylactide Coconut Biological properties Lactone copolymer Biodegradability Lactic acid copolymer Intrinsic viscosity Fiber reinforced material Plant fiber Coconut fiber Organic anhydride Experimental study Lactone polymer Functional polymer Composite material Thermal properties Lactic acid polymer Natural fiber Aliphatic polymer Concentration effect Water absorption Rheological properties
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Snippet	The thermal properties of composite materials composed of polylactide (PLA) and green coconut fiber (GCF) were evaluated. Blends containing maleic...
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SubjectTerms	Applied sciences Biodegradation Blend Burkholderia cepacia Coconut Exact sciences and technology Fibers and threads Forms of application and semi-finished materials Polylactide Polymer industry, paints, wood Technology of polymers
Title	Renewable resource-based composites of recycled natural fibers and maleated polylactide bioplastic: Characterization and biodegradability
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