Noble metal-modified octahedral anatase titania particles with enhanced activity for decomposition of chemical and microbiological pollutants

[Display omitted] •Enhancement of titania activity by modification with Au, Pt, Ag and Cu.•Significant change of properties by metal photodeposition in the presence of oxygen.•Correlation of antimicrobial and photocatalytic properties for octahedral anatase.•Zero-valent Pt and Au and positively char...

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Published inChemical engineering journal (Lausanne, Switzerland : 1996) Vol. 318; pp. 121 - 134
Main Authors Wei, Z., Endo, M., Wang, K., Charbit, E., Markowska-Szczupak, A., Ohtani, B., Kowalska, E.
Format Journal Article
LanguageEnglish
Published Switzerland Elsevier B.V 15.06.2017
Elsevier
Subjects
Antimicrobial activity
Modified titania
Octahedral anatase particles
Photocatalytic activity
Plasmonic nanoparticles
Visible light-responsive photocatalysts
Photocatalytic activity
Antimicrobial activity
Visible light-responsive photocatalysts
Modified titania
Octahedral anatase particles
Plasmonic nanoparticles
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Abstract [Display omitted] •Enhancement of titania activity by modification with Au, Pt, Ag and Cu.•Significant change of properties by metal photodeposition in the presence of oxygen.•Correlation of antimicrobial and photocatalytic properties for octahedral anatase.•Zero-valent Pt and Au and positively charged Cu and Ag in the ambient environment.•Visible activity of Au/OAPs and Ag/OAPs, due to activation of plasmon resonance. Octahedral anatase particles (OAPs) were prepared by hydrothermal (HT) reaction of titanate nanowires (TNWs). OAPs were modified with noble metals (Au, Ag, Cu and Pt) by two photodeposition methods: in the absence and in the initial presence of oxygen in the system. Photocatalytic activities for oxidative decomposition of acetic acid and anaerobic dehydrogenation of methanol under UV/vis irradiation and for oxidation of 2-propanol under visible light irradiation were investigated. Antibacterial activities for bacteria (Escherichia coli) and fungi (Candida albicans) were investigated in the dark and under UV irradiation and/or visible light irradiation. It was found that the kind of metal deposition significantly influenced the properties of photocatalysts obtained and thus their photocatalytic and antimicrobial activities. Modification of OAPs with metallic deposits resulted in enhanced photocatalytic activities for all tested systems. Pt-modified OAPs showed the highest activity for dehydrogenation of methanol due to their highest work function and lowest activation overpotential of hydrogen evolution. Cu-modified OAPs exhibited the highest activity for oxidative decomposition of acetic acid under UV/vis irradiation, probably due to the heterojunction between Cu oxides and TiO2. On the other hand, Au-modified OAPs showed the highest photocatalytic activity under visible light irradiation due to their plasmonic properties. Bare OAPs, prepared with various durations of the HT reaction, did not have any antibacterial properties in the dark, while their activity under UV/vis irradiation was correlated with their photocatalytic activities for dehydrogenation of methanol and decomposition of acetic acid. Antimicrobial activity of modified OAPs in the dark and under visible light irradiation was the highest for Ag-modified OAPs. Under UV irradiation, Cu-modified OAPs showed the highest activity for inactivation of both bacteria and fungi.
AbstractList Octahedral anatase particles (OAPs) were prepared by hydrothermal (HT) reaction of titanate nanowires (TNWs). OAPs were modified with noble metals (Au, Ag, Cu and Pt) by two photodeposition methods: in the absence and in the initial presence of oxygen in the system. Photocatalytic activities for oxidative decomposition of acetic acid and anaerobic dehydrogenation of methanol under UV/vis irradiation and for oxidation of 2-propanol under visible light irradiation were investigated. Antibacterial activities for bacteria ( ) and fungi ( ) were investigated in the dark and under UV irradiation and/or visible light irradiation. It was found that the kind of metal deposition significantly influenced the properties of photocatalysts obtained and thus their photocatalytic and antimicrobial activities. Modification of OAPs with metallic deposits resulted in enhanced photocatalytic activities for all tested systems. Pt-modified OAPs showed the highest activity for dehydrogenation of methanol due to their highest work function and lowest activation overpotential of hydrogen evolution. Cu-modified OAPs exhibited the highest activity for oxidative decomposition of acetic acid under UV/vis irradiation, probably due to the heterojunction between Cu oxides and TiO . On the other hand, Au-modified OAPs showed the highest photocatalytic activity under visible light irradiation due to their plasmonic properties. Bare OAPs, prepared with various durations of the HT reaction, did not have any antibacterial properties in the dark, while their activity under UV/vis irradiation was correlated with their photocatalytic activities for dehydrogenation of methanol and decomposition of acetic acid. Antimicrobial activity of modified OAPs in the dark and under visible light irradiation was the highest for Ag-modified OAPs. Under UV irradiation, Cu-modified OAPs showed the highest activity for inactivation of both bacteria and fungi.
• Enhancement of titania activity by modification with Au, Pt, Ag and Cu. • Significant change of properties by metal photodeposition in the presence of oxygen. • Correlation of antimicrobial and photocatalytic properties for octahedral anatase. • Zero-valent Pt and Au and positively charged Cu and Ag in the ambient environment. • Visible activity of Au/OAPs and Ag/OAPs, due to activation of plasmon resonance. Octahedral anatase particles (OAPs) were prepared by hydrothermal (HT) reaction of titanate nanowires (TNWs). OAPs were modified with noble metals (Au, Ag, Cu and Pt) by two photodeposition methods: in the absence and in the initial presence of oxygen in the system. Photocatalytic activities for oxidative decomposition of acetic acid and anaerobic dehydrogenation of methanol under UV/vis irradiation and for oxidation of 2-propanol under visible light irradiation were investigated. Antibacterial activities for bacteria ( Escherichia coli ) and fungi ( Candida albicans ) were investigated in the dark and under UV irradiation and/or visible light irradiation. It was found that the kind of metal deposition significantly influenced the properties of photocatalysts obtained and thus their photocatalytic and antimicrobial activities. Modification of OAPs with metallic deposits resulted in enhanced photocatalytic activities for all tested systems. Pt-modified OAPs showed the highest activity for dehydrogenation of methanol due to their highest work function and lowest activation overpotential of hydrogen evolution. Cu-modified OAPs exhibited the highest activity for oxidative decomposition of acetic acid under UV/vis irradiation, probably due to the heterojunction between Cu oxides and TiO 2 . On the other hand, Au-modified OAPs showed the highest photocatalytic activity under visible light irradiation due to their plasmonic properties. Bare OAPs, prepared with various durations of the HT reaction, did not have any antibacterial properties in the dark, while their activity under UV/vis irradiation was correlated with their photocatalytic activities for dehydrogenation of methanol and decomposition of acetic acid. Antimicrobial activity of modified OAPs in the dark and under visible light irradiation was the highest for Ag-modified OAPs. Under UV irradiation, Cu-modified OAPs showed the highest activity for inactivation of both bacteria and fungi.
[Display omitted] •Enhancement of titania activity by modification with Au, Pt, Ag and Cu.•Significant change of properties by metal photodeposition in the presence of oxygen.•Correlation of antimicrobial and photocatalytic properties for octahedral anatase.•Zero-valent Pt and Au and positively charged Cu and Ag in the ambient environment.•Visible activity of Au/OAPs and Ag/OAPs, due to activation of plasmon resonance. Octahedral anatase particles (OAPs) were prepared by hydrothermal (HT) reaction of titanate nanowires (TNWs). OAPs were modified with noble metals (Au, Ag, Cu and Pt) by two photodeposition methods: in the absence and in the initial presence of oxygen in the system. Photocatalytic activities for oxidative decomposition of acetic acid and anaerobic dehydrogenation of methanol under UV/vis irradiation and for oxidation of 2-propanol under visible light irradiation were investigated. Antibacterial activities for bacteria (Escherichia coli) and fungi (Candida albicans) were investigated in the dark and under UV irradiation and/or visible light irradiation. It was found that the kind of metal deposition significantly influenced the properties of photocatalysts obtained and thus their photocatalytic and antimicrobial activities. Modification of OAPs with metallic deposits resulted in enhanced photocatalytic activities for all tested systems. Pt-modified OAPs showed the highest activity for dehydrogenation of methanol due to their highest work function and lowest activation overpotential of hydrogen evolution. Cu-modified OAPs exhibited the highest activity for oxidative decomposition of acetic acid under UV/vis irradiation, probably due to the heterojunction between Cu oxides and TiO2. On the other hand, Au-modified OAPs showed the highest photocatalytic activity under visible light irradiation due to their plasmonic properties. Bare OAPs, prepared with various durations of the HT reaction, did not have any antibacterial properties in the dark, while their activity under UV/vis irradiation was correlated with their photocatalytic activities for dehydrogenation of methanol and decomposition of acetic acid. Antimicrobial activity of modified OAPs in the dark and under visible light irradiation was the highest for Ag-modified OAPs. Under UV irradiation, Cu-modified OAPs showed the highest activity for inactivation of both bacteria and fungi.
Author Wei, Z.
Endo, M.
Markowska-Szczupak, A.
Ohtani, B.
Kowalska, E.
Wang, K.
Charbit, E.
AuthorAffiliation b Institute of Chemical and Environmental Engineering, West Pomeranian University of Technology in Szczecin, ul. Pulaskiego 10, 70-322 Szczecin, Poland
a Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
AuthorAffiliation_xml – name: b Institute of Chemical and Environmental Engineering, West Pomeranian University of Technology in Szczecin, ul. Pulaskiego 10, 70-322 Szczecin, Poland
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Author_xml – sequence: 1
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  fullname: Wei, Z.
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
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  givenname: M.
  surname: Endo
  fullname: Endo, M.
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
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  surname: Wang
  fullname: Wang, K.
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
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  givenname: E.
  surname: Charbit
  fullname: Charbit, E.
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
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  givenname: A.
  surname: Markowska-Szczupak
  fullname: Markowska-Szczupak, A.
  organization: Institute of Chemical and Environmental Engineering, West Pomeranian University of Technology in Szczecin, ul. Pulaskiego 10, 70-322 Szczecin, Poland
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  givenname: B.
  surname: Ohtani
  fullname: Ohtani, B.
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
– sequence: 7
  givenname: E.
  surname: Kowalska
  fullname: Kowalska, E.
  email: kowalska@cat.hokudai.ac.jp
  organization: Institute for Catalysis, Hokkaido University, N21, W10, 001-0021 Sapporo, Japan
BackLink https://www.ncbi.nlm.nih.gov/pubmed/28626359$$D View this record in MEDLINE/PubMed
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Keywords Photocatalytic activity
Antimicrobial activity
Visible light-responsive photocatalysts
Modified titania
Octahedral anatase particles
Plasmonic nanoparticles
Language English
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This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
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Snippet [Display omitted] •Enhancement of titania activity by modification with Au, Pt, Ag and Cu.•Significant change of properties by metal photodeposition in the...
Octahedral anatase particles (OAPs) were prepared by hydrothermal (HT) reaction of titanate nanowires (TNWs). OAPs were modified with noble metals (Au, Ag, Cu...
• Enhancement of titania activity by modification with Au, Pt, Ag and Cu. • Significant change of properties by metal photodeposition in the presence of...
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StartPage 121
SubjectTerms Antimicrobial activity
Modified titania
Octahedral anatase particles
Photocatalytic activity
Plasmonic nanoparticles
Visible light-responsive photocatalysts
Title Noble metal-modified octahedral anatase titania particles with enhanced activity for decomposition of chemical and microbiological pollutants
URI https://dx.doi.org/10.1016/j.cej.2016.05.138
https://www.ncbi.nlm.nih.gov/pubmed/28626359
https://pubmed.ncbi.nlm.nih.gov/PMC5391806
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