A Long Life Moisture‐Enabled Electric Generator Based on Ionic Diode Rectification and Electrode Chemistry Regulation
Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy ef...
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| Published in | Advanced science Vol. 11; no. 15; pp. e2305530 - n/a |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Germany
John Wiley & Sons, Inc
01.04.2024
John Wiley and Sons Inc Wiley |
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| Online Access | Get full text |
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| Abstract | Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode‐type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl−. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion‐electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion‐to‐electron current conversion. A single device can deliver an open‐circuit voltage of about 1 V and a peak short‐circuit current density of 350 µA cm−2. Finally, the first‐principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance.
A moisture‐enabled electric generator for power generation at high humidity for 1240 h is presented. The device simultaneously meets the requirements of fast capture of moisture molecules, high rectification ratio transport of ions, and sustained ion‐electron current conversion, and also provides a reliable solution for ultra‐long‐time humidity power generation. |
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| AbstractList | Considerable efforts have recently been made to augment the power density of moisture-enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion-directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode-type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl-. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion-electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion-to-electron current conversion. A single device can deliver an open-circuit voltage of about 1 V and a peak short-circuit current density of 350 µA cm-2. Finally, the first-principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance.Considerable efforts have recently been made to augment the power density of moisture-enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion-directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode-type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl-. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion-electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion-to-electron current conversion. A single device can deliver an open-circuit voltage of about 1 V and a peak short-circuit current density of 350 µA cm-2. Finally, the first-principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode‐type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl−. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion‐electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion‐to‐electron current conversion. A single device can deliver an open‐circuit voltage of about 1 V and a peak short‐circuit current density of 350 µA cm−2. Finally, the first‐principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. A moisture‐enabled electric generator for power generation at high humidity for 1240 h is presented. The device simultaneously meets the requirements of fast capture of moisture molecules, high rectification ratio transport of ions, and sustained ion‐electron current conversion, and also provides a reliable solution for ultra‐long‐time humidity power generation. Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode‐type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl − . The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion‐electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion‐to‐electron current conversion. A single device can deliver an open‐circuit voltage of about 1 V and a peak short‐circuit current density of 350 µA cm −2 . Finally, the first‐principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode‐type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl − . The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion‐electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion‐to‐electron current conversion. A single device can deliver an open‐circuit voltage of about 1 V and a peak short‐circuit current density of 350 µA cm −2 . Finally, the first‐principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. A moisture‐enabled electric generator for power generation at high humidity for 1240 h is presented. The device simultaneously meets the requirements of fast capture of moisture molecules, high rectification ratio transport of ions, and sustained ion‐electron current conversion, and also provides a reliable solution for ultra‐long‐time humidity power generation. Abstract Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion‐directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode‐type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl−. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion‐electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion‐to‐electron current conversion. A single device can deliver an open‐circuit voltage of about 1 V and a peak short‐circuit current density of 350 µA cm−2. Finally, the first‐principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. Considerable efforts have recently been made to augment the power density of moisture-enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion-directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode-type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl−. The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion-electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion-to-electron current conversion. A single device can deliver an open-circuit voltage of about 1 V and a peak short-circuit current density of 350 µA cm−2. Finally, the first-principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. Considerable efforts have recently been made to augment the power density of moisture-enabled electric generators. However, due to the unsustainable ion/water molecule concentration gradients, the ion-directed transport gradually diminishes, which largely affects the operating lifetime and energy efficiency of generators. This work introduces an electrode chemistry regulation strategy into the ionic diode-type energy conversion structure, which demonstrates 1240 h power generation in ambient humidity. The electrode chemical regulation can be achieved by adding Cl . The purpose is to destroy the passivation film on the electrode interface and provide a continuous path for ion-electron coupling conduction. Moreover, this device simultaneously satisfies the requirements of fast trapping of moisture molecules, high rectification ratio transport of ions, and sustained ion-to-electron current conversion. A single device can deliver an open-circuit voltage of about 1 V and a peak short-circuit current density of 350 µA cm . Finally, the first-principle calculations are carried out to reveal the mechanism by which the electrode surface chemistry affects the power generation performance. |
| Author | Fu, Chunqiao Lu, Xulei He, Qi‐Chang Zhou, Jian Yao, Yuming Feng, Haochen Shang, Kedong Zhang, Yong Jiang, Zhongbao Yang, Tingting |
| AuthorAffiliation | 1 Tribology Research Institute School of Mechanical Engineering Southwest Jiaotong University Chengdu 610031 P. R. China 2 Univ Gustave Eiffel MSME CNRS UMR 8208 Marne‐la‐Vallée F‐77454 France |
| AuthorAffiliation_xml | – name: 1 Tribology Research Institute School of Mechanical Engineering Southwest Jiaotong University Chengdu 610031 P. R. China – name: 2 Univ Gustave Eiffel MSME CNRS UMR 8208 Marne‐la‐Vallée F‐77454 France |
| Author_xml | – sequence: 1 givenname: Chunqiao surname: Fu fullname: Fu, Chunqiao organization: Southwest Jiaotong University – sequence: 2 givenname: Jian surname: Zhou fullname: Zhou, Jian organization: Southwest Jiaotong University – sequence: 3 givenname: Xulei surname: Lu fullname: Lu, Xulei organization: Southwest Jiaotong University – sequence: 4 givenname: Haochen surname: Feng fullname: Feng, Haochen organization: Southwest Jiaotong University – sequence: 5 givenname: Yong surname: Zhang fullname: Zhang, Yong organization: Southwest Jiaotong University – sequence: 6 givenname: Kedong surname: Shang fullname: Shang, Kedong organization: Southwest Jiaotong University – sequence: 7 givenname: Zhongbao surname: Jiang fullname: Jiang, Zhongbao organization: Southwest Jiaotong University – sequence: 8 givenname: Yuming surname: Yao fullname: Yao, Yuming organization: Southwest Jiaotong University – sequence: 9 givenname: Qi‐Chang surname: He fullname: He, Qi‐Chang email: qichang.he@u-pem.fr organization: MSME – sequence: 10 givenname: Tingting orcidid: 0000-0001-6773-8438 surname: Yang fullname: Yang, Tingting email: yangtingting@swjtu.edu.cn organization: Southwest Jiaotong University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/38353337$$D View this record in MEDLINE/PubMed |
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| CitedBy_id | crossref_primary_10_1016_j_isci_2025_112026 crossref_primary_10_1088_1402_4896_ad911f crossref_primary_10_1016_j_nanoen_2024_110291 crossref_primary_10_1038_s41467_024_55516_z crossref_primary_10_1039_D4EE02252A |
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| Keywords | long lifetime electrode chemistry regulation ionic diode hydrovoltaic moisture |
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| Snippet | Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable ion/water... Considerable efforts have recently been made to augment the power density of moisture-enabled electric generators. However, due to the unsustainable ion/water... Abstract Considerable efforts have recently been made to augment the power density of moisture‐enabled electric generators. However, due to the unsustainable... |
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| SubjectTerms | Alternative energy sources Carbon Chemical vapor deposition Chloride Electric fields Electricity electrode chemistry regulation Electrodes Energy resources Generators Humidity hydrovoltaic ionic diode long lifetime moisture Moisture absorption Nanostructured materials Renewable resources |
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| Title | A Long Life Moisture‐Enabled Electric Generator Based on Ionic Diode Rectification and Electrode Chemistry Regulation |
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