Beyond the Phase Segregation: Probing the Irreversible Phase Reconstruction of Mixed‐Halide Perovskites
Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the pha...
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| Published in | Advanced science Vol. 9; no. 5; pp. e2103948 - n/a |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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John Wiley & Sons, Inc
01.02.2022
John Wiley and Sons Inc Wiley |
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| Abstract | Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I1−xBrx)3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3. The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution.
Photoluminescence imaging microscopy is employed to investigate the phase transformation of MAPb(I1−xBrx)3 under continuous irradiation. Due to the charge injection from Br‐rich to I‐rich domains, an irreversible reconstruction of MAPbBr3 is induced. This work reveals the mechanisms of photo‐induced phase reconstruction, and deepens the understanding of the stability of mixed‐halide perovskites. |
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| AbstractList | Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I1−xBrx)3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3. The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution.
Photoluminescence imaging microscopy is employed to investigate the phase transformation of MAPb(I1−xBrx)3 under continuous irradiation. Due to the charge injection from Br‐rich to I‐rich domains, an irreversible reconstruction of MAPbBr3 is induced. This work reveals the mechanisms of photo‐induced phase reconstruction, and deepens the understanding of the stability of mixed‐halide perovskites. Abstract Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I1−xBrx)3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3. The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution. Mixed-halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite-based devices are still open questions. Here, the phase transformation of MAPb(I Br ) after phase segregation and probe an irreversible phase reconstruction of MAPbBr is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type-I band alignment of segregated I-rich and Br-rich domains can enhance the emission of the I-rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br-rich to I-rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr . The work highlights the significance of ion movements in mixed-halide perovskites and provides new perspectives to understand the property evolution. Mixed-halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite-based devices are still open questions. Here, the phase transformation of MAPb(I1- x Brx )3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type-I band alignment of segregated I-rich and Br-rich domains can enhance the emission of the I-rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br-rich to I-rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3 . The work highlights the significance of ion movements in mixed-halide perovskites and provides new perspectives to understand the property evolution.Mixed-halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite-based devices are still open questions. Here, the phase transformation of MAPb(I1- x Brx )3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type-I band alignment of segregated I-rich and Br-rich domains can enhance the emission of the I-rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br-rich to I-rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3 . The work highlights the significance of ion movements in mixed-halide perovskites and provides new perspectives to understand the property evolution. Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I 1− x Br x ) 3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr 3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr 3 . The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution. Photoluminescence imaging microscopy is employed to investigate the phase transformation of MAPb(I 1− x Br x ) 3 under continuous irradiation. Due to the charge injection from Br‐rich to I‐rich domains, an irreversible reconstruction of MAPbBr 3 is induced. This work reveals the mechanisms of photo‐induced phase reconstruction, and deepens the understanding of the stability of mixed‐halide perovskites. Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I1−xBrx)3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr3. The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution. Abstract Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is reversible, what happens after phase segregation and its impact on the performance of perovskite‐based devices are still open questions. Here, the phase transformation of MAPb(I 1− x Br x ) 3 after phase segregation and probe an irreversible phase reconstruction of MAPbBr 3 is investigated. The photoluminescence imaging microscopy technique is introduced to in situ record the whole process. It is proposed that the type‐I band alignment of segregated I‐rich and Br‐rich domains can enhance the emission of the I‐rich domains by suppressing the nonradiative recombination channels. At the same time, the charge injection from Br‐rich to I‐rich domains drives the expulsion of iodide from the lattice, and thus triggers the reconstruction of MAPbBr 3 . The work highlights the significance of ion movements in mixed‐halide perovskites and provides new perspectives to understand the property evolution. |
| Author | Wang, Yanbo An, Yongkang Cheacharoen, Rongrong Li, Zhe Xiao, Xuan Li, Xiong An, Qinyou Huang, Qingyi Zheng, Xin Wang, Ti Rong, Yaoguang Xu, Hongxing |
| AuthorAffiliation | 1 School of Physics and Technology and Key Laboratory of Artificial Micro‐ and Nanostructures of Ministry of Education Wuhan University Wuhan 430072 China 2 Wuhan National Laboratory for Optoelectronics Huazhong University of Science and Technology Wuhan 430074 China 3 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan Hubei 430070 China 4 State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong University Shanghai 200240 China 5 Metallurgy and Materials Science Research Institute Chulalongkorn University Bangkok 10330 Thailand |
| AuthorAffiliation_xml | – name: 2 Wuhan National Laboratory for Optoelectronics Huazhong University of Science and Technology Wuhan 430074 China – name: 3 State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan Hubei 430070 China – name: 1 School of Physics and Technology and Key Laboratory of Artificial Micro‐ and Nanostructures of Ministry of Education Wuhan University Wuhan 430072 China – name: 4 State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong University Shanghai 200240 China – name: 5 Metallurgy and Materials Science Research Institute Chulalongkorn University Bangkok 10330 Thailand |
| Author_xml | – sequence: 1 givenname: Zhe surname: Li fullname: Li, Zhe organization: Wuhan University – sequence: 2 givenname: Xin surname: Zheng fullname: Zheng, Xin organization: Huazhong University of Science and Technology – sequence: 3 givenname: Xuan surname: Xiao fullname: Xiao, Xuan organization: Huazhong University of Science and Technology – sequence: 4 givenname: Yongkang surname: An fullname: An, Yongkang organization: Wuhan University of Technology – sequence: 5 givenname: Yanbo surname: Wang fullname: Wang, Yanbo organization: Shanghai Jiao Tong University – sequence: 6 givenname: Qingyi surname: Huang fullname: Huang, Qingyi organization: Huazhong University of Science and Technology – sequence: 7 givenname: Xiong surname: Li fullname: Li, Xiong organization: Huazhong University of Science and Technology – sequence: 8 givenname: Rongrong surname: Cheacharoen fullname: Cheacharoen, Rongrong organization: Chulalongkorn University – sequence: 9 givenname: Qinyou surname: An fullname: An, Qinyou organization: Wuhan University of Technology – sequence: 10 givenname: Yaoguang orcidid: 0000-0003-4794-8213 surname: Rong fullname: Rong, Yaoguang email: ygrong@hust.edu.cn organization: Huazhong University of Science and Technology – sequence: 11 givenname: Ti surname: Wang fullname: Wang, Ti email: wangti@whu.edu.cn organization: Wuhan University – sequence: 12 givenname: Hongxing surname: Xu fullname: Xu, Hongxing email: hxxu@whu.edu.cn organization: Wuhan University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34923773$$D View this record in MEDLINE/PubMed |
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| CitedBy_id | crossref_primary_10_1021_acs_jpcc_3c04708 crossref_primary_10_1021_acs_jpcc_3c05919 crossref_primary_10_1038_s41570_023_00492_z crossref_primary_10_1021_acssuschemeng_2c05752 crossref_primary_10_1021_acsanm_3c02399 crossref_primary_10_1126_science_add8786 crossref_primary_10_1002_aenm_202203911 crossref_primary_10_1016_j_chempr_2022_07_005 crossref_primary_10_1002_adma_202210834 crossref_primary_10_1039_D3QM00970J crossref_primary_10_1021_acssuschemeng_3c01873 crossref_primary_10_1039_D3TC01362F crossref_primary_10_1002_smtd_202200161 crossref_primary_10_1002_adom_202202118 crossref_primary_10_1016_j_cej_2022_140142 crossref_primary_10_1002_solr_202400216 crossref_primary_10_1039_D2QM01341J |
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| Keywords | mixed-halide perovskite phase reconstruction photoluminescence imaging stability |
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| Snippet | Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is... Mixed-halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is... Abstract Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is... Abstract Mixed‐halide perovskites can undergo a photoinduced phase segregation. Even though many reports have claimed that such a phase segregation process is... |
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| SubjectTerms | Glass substrates Grain boundaries Light Microscopy mixed‐halide perovskite phase reconstruction Phase transitions photoluminescence imaging stability Thin films |
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| Title | Beyond the Phase Segregation: Probing the Irreversible Phase Reconstruction of Mixed‐Halide Perovskites |
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