From nanoscale interface characterization to sustainable energy storage using all-solid-state batteries
The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challen...
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| Published in | Nature nanotechnology Vol. 15; no. 3; pp. 170 - 180 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
01.03.2020
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1748-3387 1748-3395 1748-3395 |
| DOI | 10.1038/s41565-020-0657-x |
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| Abstract | The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model.
This Review summarizes the current nanoscale understanding of the interface chemistries between solid state electrolytes and electrodes for future all solid state batteries. |
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| AbstractList | The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model.This Review summarizes the current nanoscale understanding of the interface chemistries between solid state electrolytes and electrodes for future all solid state batteries. The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model. The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model. This Review summarizes the current nanoscale understanding of the interface chemistries between solid state electrolytes and electrodes for future all solid state batteries. The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model.The recent discovery of highly conductive solid-state electrolytes (SSEs) has led to tremendous progress in the development of all-solid-state batteries (ASSBs). Though promising, they still face barriers that limit their practical application, such as poor interfacial stability, scalability challenges and production safety. Additionally, efforts to develop sustainable manufacturing of lithium ion batteries are still lacking, with no prevailing strategy developed yet to handle recyclability of ASSBs. To date, most SSE research has been largely focused on the discovery of novel electrolytes. Recent review articles have extensively examined a broad spectrum of these SSEs using evaluation factors such as conductivity and chemical stability. Recognizing this, in this Review we seek to evaluate SSEs beyond conventional factors and offer a perspective on various bulk, interface and nanoscale phenomena that require urgent attention within the scientific community. We provide a realistic assessment of the current state-of-the-art characterization techniques and evaluate future full cell ASSB prototyping strategies. We hope to offer rational solutions to overcome some major fundamental obstacles faced by the ASSB community, as well as potential strategies toward a sustainable ASSB recycling model. |
| Author | Meng, Ying Shirley Tan, Darren H. S. Chen, Zheng Banerjee, Abhik |
| Author_xml | – sequence: 1 givenname: Darren H. S. surname: Tan fullname: Tan, Darren H. S. organization: Department of NanoEngineering, University of California San Diego – sequence: 2 givenname: Abhik surname: Banerjee fullname: Banerjee, Abhik organization: Department of NanoEngineering, University of California San Diego – sequence: 3 givenname: Zheng orcidid: 0000-0002-9186-4298 surname: Chen fullname: Chen, Zheng email: zhengchen@eng.ucsd.edu organization: Department of NanoEngineering, University of California San Diego, Program of Chemical Engineering, University of California San Diego, Sustainable Power & Energy Center (SPEC), University of California San Diego – sequence: 4 givenname: Ying Shirley orcidid: 0000-0001-8936-8845 surname: Meng fullname: Meng, Ying Shirley email: shmeng@ucsd.edu organization: Department of NanoEngineering, University of California San Diego, Sustainable Power & Energy Center (SPEC), University of California San Diego |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32157239$$D View this record in MEDLINE/PubMed |
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| Title | From nanoscale interface characterization to sustainable energy storage using all-solid-state batteries |
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