Li‐ and Mn‐Rich Cathode Materials: Challenges to Commercialization

The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg−1) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initi...

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Published in	Advanced energy materials Vol. 7; no. 6; pp. np - n/a
Main Authors	Zheng, Jianming, Myeong, Seungjun, Cho, Woongrae, Yan, Pengfei, Xiao, Jie, Wang, Chongmin, Cho, Jaephil, Zhang, Ji‐Guang
Format	Journal Article
Language	English
Published	Weinheim Wiley Subscription Services, Inc 22.03.2017 Wiley
Subjects	Cathodes Commercialization doping/coating Electric potential Electrodes Environmental Molecular Sciences Laboratory full cell full cells Graphite initial capacity loss Li-rich Mn-rich cathode Lithium Li‐ and Mn‐rich cathode rate capability Specifications Strategy Voltage voltage fade
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Abstract	The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg−1) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progress and in depth understandings on the application of LMR cathode materials from a practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full‐cell operation are systematically analyzed. These factors include the first‐cycle capacity loss, voltage fade, powder tap density, and electrode density. New approaches to minimize the detrimental effects of these factors are highlighted in this work. We also provide perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while keeping practical considerations in mind. An overview of current research activities addressing the key challenges of LMR cathodes is presented, focusing on discussion of the facile strategies to improve the initial Coulombic efficiency, working voltage stability, and rate capability. Promising perspectives for LMR studies are suggested by providing full‐cell data of LMR electrodes with commercialization specifications.
AbstractList	The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg−1) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progress and in depth understandings on the application of LMR cathode materials from a practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full‐cell operation are systematically analyzed. These factors include the first‐cycle capacity loss, voltage fade, powder tap density, and electrode density. New approaches to minimize the detrimental effects of these factors are highlighted in this work. We also provide perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while keeping practical considerations in mind. An overview of current research activities addressing the key challenges of LMR cathodes is presented, focusing on discussion of the facile strategies to improve the initial Coulombic efficiency, working voltage stability, and rate capability. Promising perspectives for LMR studies are suggested by providing full‐cell data of LMR electrodes with commercialization specifications. The lithium- and manganese-rich (LMR) layered structure cathodes exhibit one of the highest specific energies ( approximately 900 W h kg super(-1)) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progress and in depth understandings on the application of LMR cathode materials from a practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full-cell operation are systematically analyzed. These factors include the first-cycle capacity loss, voltage fade, powder tap density, and electrode density. New approaches to minimize the detrimental effects of these factors are highlighted in this work. We also provide perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while keeping practical considerations in mind. An overview of current research activities addressing the key challenges of LMR cathodes is presented, focusing on discussion of the facile strategies to improve the initial Coulombic efficiency, working voltage stability, and rate capability. Promising perspectives for LMR studies are suggested by providing full-cell data of LMR electrodes with commercialization specifications. The lithium- and manganese-rich (LMR) layered structure cathodes exhibit one of the highest specific energies ([asymptotically =]900 W h kg-1) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progress and in depth understandings on the application of LMR cathode materials from a practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full-cell operation are systematically analyzed. These factors include the first-cycle capacity loss, voltage fade, powder tap density, and electrode density. New approaches to minimize the detrimental effects of these factors are highlighted in this work. We also provide perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while keeping practical considerations in mind. The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg −1 ) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges, including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progress and in depth understandings on the application of LMR cathode materials from a practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full‐cell operation are systematically analyzed. These factors include the first‐cycle capacity loss, voltage fade, powder tap density, and electrode density. New approaches to minimize the detrimental effects of these factors are highlighted in this work. We also provide perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while keeping practical considerations in mind. The lithium- and manganese-rich (LMR) layered structure cathode exhibit one of the highest specific energy (~900 Wh kg-1) among all the cathode materials. However, the practical applications of LMR cathodes are still hindered by several significant challenges including voltage fade, large initial capacity loss, poor rate capability and limited cycle life. Herein, we review the recent progresses and understandings on the application of LMR cathode materials from practical point of view. Several key parameters of LMR cathodes that affect the LMR/graphite full cell operation are systematically analysed. These factors include the first cycle capacity loss, voltage fade, powder tap density, electrode density of LMR based cathode etc. New approaches to minimize the detrimental effect of these factors are highlighted in this work. We also provided the perspectives for the future research on LMR cathode materials, focusing on addressing the fundamental problems of LMR cathodes while always keeping practical considerations in mind.
Author	Xiao, Jie Myeong, Seungjun Zheng, Jianming Cho, Jaephil Zhang, Ji‐Guang Yan, Pengfei Cho, Woongrae Wang, Chongmin
Author_xml	– sequence: 1 givenname: Jianming surname: Zheng fullname: Zheng, Jianming organization: Pacific Northwest National Laboratory – sequence: 2 givenname: Seungjun surname: Myeong fullname: Myeong, Seungjun organization: Ulsan National Institute of Science and Technology (UNIST) – sequence: 3 givenname: Woongrae surname: Cho fullname: Cho, Woongrae organization: Ulsan National Institute of Science and Technology (UNIST) – sequence: 4 givenname: Pengfei surname: Yan fullname: Yan, Pengfei organization: Pacific Northwest National Laboratory – sequence: 5 givenname: Jie surname: Xiao fullname: Xiao, Jie organization: Pacific Northwest National Laboratory – sequence: 6 givenname: Chongmin surname: Wang fullname: Wang, Chongmin organization: Pacific Northwest National Laboratory – sequence: 7 givenname: Jaephil surname: Cho fullname: Cho, Jaephil email: jpcho@unist.ac.kr organization: Ulsan National Institute of Science and Technology (UNIST) – sequence: 8 givenname: Ji‐Guang surname: Zhang fullname: Zhang, Ji‐Guang email: jiguang.zhang@pnnl.gov organization: Pacific Northwest National Laboratory
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Snippet	The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg−1) among all the cathode materials.... The lithium‐ and manganese‐rich (LMR) layered structure cathodes exhibit one of the highest specific energies (≈900 W h kg −1 ) among all the cathode... The lithium- and manganese-rich (LMR) layered structure cathodes exhibit one of the highest specific energies ([asymptotically =]900 W h kg-1) among all the... The lithium- and manganese-rich (LMR) layered structure cathodes exhibit one of the highest specific energies ( approximately 900 W h kg super(-1)) among all... The lithium- and manganese-rich (LMR) layered structure cathode exhibit one of the highest specific energy (~900 Wh kg-1) among all the cathode materials....
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SubjectTerms	Cathodes Commercialization doping/coating Electric potential Electrodes Environmental Molecular Sciences Laboratory full cell full cells Graphite initial capacity loss Li-rich Mn-rich cathode Lithium Li‐ and Mn‐rich cathode rate capability Specifications Strategy Voltage voltage fade
Title	Li‐ and Mn‐Rich Cathode Materials: Challenges to Commercialization
URI	https://onlinelibrary.wiley.com/doi/abs/10.1002%2Faenm.201601284 https://www.proquest.com/docview/1879721353 https://www.proquest.com/docview/1893910193 https://www.osti.gov/biblio/1373002
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