Removal of heavy metals from aqueous solution by biochars derived from anaerobically digested biomass
► Biochars from anaerobically digested biomass effectively removed heavy metals. ► Lead sorption capacities of the biochars were close to or higher than 200mmol/kg. ► Surface precipitation was the governing heavy metal removal mechanism. This study examined the ability of two biochars converted from...
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| Published in | Bioresource technology Vol. 110; pp. 50 - 56 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.04.2012
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| Subjects | |
| Online Access | Get full text |
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| Abstract | ► Biochars from anaerobically digested biomass effectively removed heavy metals. ► Lead sorption capacities of the biochars were close to or higher than 200mmol/kg. ► Surface precipitation was the governing heavy metal removal mechanism.
This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb2 +, Cu2+, Ni2+, and Cd2+) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM–EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons. |
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| AbstractList | This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb2 +, Cu2+, Ni2+, and Cd2+) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM-EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200 mmol/kg, which is comparable to that of commercial activated carbons. This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb² ⁺, Cu²⁺, Ni²⁺, and Cd²⁺) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM–EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons. ► Biochars from anaerobically digested biomass effectively removed heavy metals. ► Lead sorption capacities of the biochars were close to or higher than 200mmol/kg. ► Surface precipitation was the governing heavy metal removal mechanism. This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb2 +, Cu2+, Ni2+, and Cd2+) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM–EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons. This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb(2 +), Cu(2+), Ni(2+), and Cd(2+)) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM-EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons.This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb(2 +), Cu(2+), Ni(2+), and Cd(2+)) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM-EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons. This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and characterization experiments. Initial evaluation of DAWC (digested dairy waste biochar) and DWSBC (digested whole sugar beet biochar) showed that both biochars were effective in removing a mixture of four heavy metals (Pb(2 +), Cu(2+), Ni(2+), and Cd(2+)) from aqueous solutions. Compared to DAWC, DWSBC demonstrated a better ability to remove Ni and Cd. Further investigations of lead sorption by the two biochars indicated that the removal was mainly through a surface precipitation mechanism, which was confirmed by batch sorption experiments, mathematical modeling, and examinations of lead-laden biochars samples using SEM-EDS, XRD, and FTIR. The lead sorption capacity of the two biochars was close to or higher than 200mmol/kg, which is comparable to that of commercial activated carbons. |
| Author | Zimmerman, Andrew R. Xue, Yingwen Inyang, Mandu Yao, Ying Pullammanappallil, Pratap Cao, Xinde Gao, Bin |
| Author_xml | – sequence: 1 givenname: Mandu surname: Inyang fullname: Inyang, Mandu organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States – sequence: 2 givenname: Bin surname: Gao fullname: Gao, Bin email: bg55@ufl.edu organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States – sequence: 3 givenname: Ying surname: Yao fullname: Yao, Ying organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States – sequence: 4 givenname: Yingwen surname: Xue fullname: Xue, Yingwen organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States – sequence: 5 givenname: Andrew R. surname: Zimmerman fullname: Zimmerman, Andrew R. organization: Department of Geological Sciences, University of Florida, Gainesville, FL 32611, United States – sequence: 6 givenname: Pratap surname: Pullammanappallil fullname: Pullammanappallil, Pratap organization: Department of Agricultural and Biological Engineering, University of Florida, Gainesville, FL 32611, United States – sequence: 7 givenname: Xinde surname: Cao fullname: Cao, Xinde organization: School of Environmental Science and Engineering, Shanghai Jiaotong University, Shanghai 200240, China |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22325901$$D View this record in MEDLINE/PubMed |
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| Keywords | Sorption Biochar Wastewater Anaerobic digestion Heavy metal |
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| Snippet | ► Biochars from anaerobically digested biomass effectively removed heavy metals. ► Lead sorption capacities of the biochars were close to or higher than... This study examined the ability of two biochars converted from anaerobically digested biomass to sorb heavy metals using a range of laboratory sorption and... |
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| SubjectTerms | activated carbon Anaerobic digestion Anaerobiosis aqueous solutions Biochar Biomass dairies Fourier transform infrared spectroscopy Heavy metal heavy metals isolation & purification Kinetics lead mathematical models Metals, Heavy Metals, Heavy - isolation & purification Solutions Sorption sugar beet Wastewater Water |
| Title | Removal of heavy metals from aqueous solution by biochars derived from anaerobically digested biomass |
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