Molybdenum Disulfide/Nitrogen-Doped Reduced Graphene Oxide Nanocomposite with Enlarged Interlayer Spacing for Electrocatalytic Hydrogen Evolution
Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enl...
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| Published in | Advanced energy materials Vol. 6; no. 12; pp. np - n/a |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Blackwell Publishing Ltd
01.06.2016
Wiley Subscription Services, Inc |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å by a one‐step hydrothermal method is reported. The synergistic effects between the layered MoS2 nanosheets and N‐doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS2/N‐RGO‐180 exhibits the excellent catalytic activity with a low onset potential of −5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec−1, a high exchange current density of 7.4 × 10−4 A cm−2, and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS2/N‐RGO‐180 nanocomposite is superior to the most reported MoS2‐based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low‐cost MoS2‐based electrocatalysts with the extraordinary HER performance is presented.
A simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å is reported. MoS2/N‐RGO‐180 exhibits excellent hydrogen evolution reaction (HER) catalytic activity with a low onset potential of −5 mV versus RHE, a small Tafel slope of 41.3 mV dec−1 and good stability over 5000 cycles. |
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| AbstractList | Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS
2
/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å by a one‐step hydrothermal method is reported. The synergistic effects between the layered MoS
2
nanosheets and N‐doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS
2
/N‐RGO‐180 exhibits the excellent catalytic activity with a low onset potential of −5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec
−1
, a high exchange current density of 7.4 × 10
−4
A cm
−2
, and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS
2
/N‐RGO‐180 nanocomposite is superior to the most reported MoS
2
‐based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low‐cost MoS
2
‐based electrocatalysts with the extraordinary HER performance is presented. Facile design of low-cost and highly active catalysts from earth-abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen-doped reduced graphene oxide (MoS2/N-RGO-180) nanocomposite with the enlarged interlayer spacing of 9.5 Å by a one-step hydrothermal method is reported. The synergistic effects between the layered MoS2 nanosheets and N-doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS2/N-RGO-180 exhibits the excellent catalytic activity with a low onset potential of -5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec-1, a high exchange current density of 7.4 × 10-4 A cm-2, and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS2/N-RGO-180 nanocomposite is superior to the most reported MoS2-based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low-cost MoS2-based electrocatalysts with the extraordinary HER performance is presented. Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å by a one‐step hydrothermal method is reported. The synergistic effects between the layered MoS2 nanosheets and N‐doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS2/N‐RGO‐180 exhibits the excellent catalytic activity with a low onset potential of −5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec−1, a high exchange current density of 7.4 × 10−4 A cm−2, and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS2/N‐RGO‐180 nanocomposite is superior to the most reported MoS2‐based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low‐cost MoS2‐based electrocatalysts with the extraordinary HER performance is presented. A simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å is reported. MoS2/N‐RGO‐180 exhibits excellent hydrogen evolution reaction (HER) catalytic activity with a low onset potential of −5 mV versus RHE, a small Tafel slope of 41.3 mV dec−1 and good stability over 5000 cycles. Facile design of low-cost and highly active catalysts from earth-abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen-doped reduced graphene oxide (MoS sub(2)/N-RGO-180) nanocomposite with the enlarged interlayer spacing of 9.5 Aa by a one-step hydrothermal method is reported. The synergistic effects between the layered MoS sub(2) nanosheets and N-doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS sub(2)/N-RGO-180 exhibits the excellent catalytic activity with a low onset potential of -5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec super(-1), a high exchange current density of 7.4 10 super(-4) A cm super(-2), and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS sub(2)/N-RGO-180 nanocomposite is superior to the most reported MoS sub(2)-based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low-cost MoS sub(2)-based electrocatalysts with the extraordinary HER performance is presented. A simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen-doped reduced graphene oxide (MoS sub(2)/N-RGO-180) nanocomposite with the enlarged interlayer spacing of 9.5 Aa is reported. MoS sub(2)/N-RGO-180 exhibits excellent hydrogen evolution reaction (HER) catalytic activity with a low onset potential of -5 mV versus RHE, a small Tafel slope of 41.3 mV dec super(-1) and good stability over 5000 cycles. Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a simple strategy to synthesize an ultrathin molybdenum disulfide/nitrogen‐doped reduced graphene oxide (MoS2/N‐RGO‐180) nanocomposite with the enlarged interlayer spacing of 9.5 Å by a one‐step hydrothermal method is reported. The synergistic effects between the layered MoS2 nanosheets and N‐doped RGO films contribute to the high activity for hydrogen evolution reaction (HER). MoS2/N‐RGO‐180 exhibits the excellent catalytic activity with a low onset potential of −5 mV versus reversible hydrogen elelctrode (RHE), a small Tafel slope of 41.3 mV dec−1, a high exchange current density of 7.4 × 10−4 A cm−2, and good stability over 5 000 cycles under acidic conditions. The HER performance of MoS2/N‐RGO‐180 nanocomposite is superior to the most reported MoS2‐based catalysts, especially its onset potential and exchange current density. In this work, a novel and simple method to the preparation of low‐cost MoS2‐based electrocatalysts with the extraordinary HER performance is presented. |
| Author | Lan, Ya-Qian Tang, Yu-Jia Dong, Long-Zhang Li, Ya-Fei Wang, Yu Li, Shun-Li Huang, Wei Wang, Xiao-Li Liu, Chun-Hui |
| Author_xml | – sequence: 1 givenname: Yu-Jia surname: Tang fullname: Tang, Yu-Jia organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 2 givenname: Yu surname: Wang fullname: Wang, Yu organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 3 givenname: Xiao-Li surname: Wang fullname: Wang, Xiao-Li organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 4 givenname: Shun-Li surname: Li fullname: Li, Shun-Li organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 5 givenname: Wei surname: Huang fullname: Huang, Wei organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 6 givenname: Long-Zhang surname: Dong fullname: Dong, Long-Zhang organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 7 givenname: Chun-Hui surname: Liu fullname: Liu, Chun-Hui organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 8 givenname: Ya-Fei surname: Li fullname: Li, Ya-Fei email: liyafei.abc@gmail.com organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China – sequence: 9 givenname: Ya-Qian surname: Lan fullname: Lan, Ya-Qian email: liyafei.abc@gmail.com organization: Jiangsu Key Laboratory of Biofunctional Materials College of Chemistry and Materials Science, Nanjing Normal University, 210023, Nanjing, P. R. China |
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| Snippet | Facile design of low‐cost and highly active catalysts from earth‐abundant elements is favorable for the industrial application of water splitting. Here, a... Facile design of low-cost and highly active catalysts from earth-abundant elements is favorable for the industrial application of water splitting. Here, a... |
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| SubjectTerms | Catalysts Catalytic activity Current density Electrocatalysts enlarged interlayer spacing Expansion Graphene Hydrogen evolution hydrogen evolution reaction Hydrogen evolution reactions Industrial applications Interlayers Molybdenum Molybdenum disulfide MoS2/RGO Nanocomposites Nitrogen nitrogen-doped species Oxides Synergistic effect Water splitting |
| Title | Molybdenum Disulfide/Nitrogen-Doped Reduced Graphene Oxide Nanocomposite with Enlarged Interlayer Spacing for Electrocatalytic Hydrogen Evolution |
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