Electric-Field-Induced Connectivity Switching in Single-Molecule Junctions
The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different...
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| Published in | iScience Vol. 23; no. 1; p. 100770 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
24.01.2020
Elsevier |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2589-0042 2589-0042 |
| DOI | 10.1016/j.isci.2019.100770 |
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| Abstract | The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction.
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•A strategy to in-situ switch the connectivity of single-molecule junctions•A concept to manipulate the molecule-electrode interaction•A molecular switch triggered by the varying of electric field•Experiments were combined with calculations to probe the switching mechanism
Molecular Electrochemistry; Quantum Electronics; Electronic Materials |
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| AbstractList | The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction.
[Display omitted]
•A strategy to in-situ switch the connectivity of single-molecule junctions•A concept to manipulate the molecule-electrode interaction•A molecular switch triggered by the varying of electric field•Experiments were combined with calculations to probe the switching mechanism
Molecular Electrochemistry; Quantum Electronics; Electronic Materials The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction.The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction. The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction. • A strategy to in-situ switch the connectivity of single-molecule junctions • A concept to manipulate the molecule-electrode interaction • A molecular switch triggered by the varying of electric field • Experiments were combined with calculations to probe the switching mechanism Molecular Electrochemistry; Quantum Electronics; Electronic Materials The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction. The manipulation of molecule-electrode interaction is essential for the fabrication of molecular devices and determines the connectivity from electrodes to molecular components. Although the connectivity of molecular devices could be controlled by molecular design to place anchor groups in different positions of molecule backbones, the reversible switching of such connectivities remains challenging. Here, we develop an electric-field-induced strategy to switch the connectivity of single-molecule junctions reversibly, leading to the manipulation of different connectivities in the same molecular backbone. Our results offer a new concept of single-molecule manipulation and provide a feasible strategy to regulate molecule-electrode interaction. : Molecular Electrochemistry; Quantum Electronics; Electronic Materials Subject Areas: Molecular Electrochemistry, Quantum Electronics, Electronic Materials |
| ArticleNumber | 100770 |
| Author | Xia, Haiping Chen, Lijue Liu, Junyang Chen, Zhixin Yan, Zhewei Shi, Jia Chen, Lichuan Huang, Xiaoyan Chen, Zhaobin Hong, Wenjing Zheng, Jueting Tang, Chun Ye, Yiling Bai, Jie |
| AuthorAffiliation | 1 State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China |
| AuthorAffiliation_xml | – name: 1 State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China |
| Author_xml | – sequence: 1 givenname: Chun surname: Tang fullname: Tang, Chun organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 2 givenname: Jueting surname: Zheng fullname: Zheng, Jueting organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 3 givenname: Yiling surname: Ye fullname: Ye, Yiling organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 4 givenname: Junyang surname: Liu fullname: Liu, Junyang organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 5 givenname: Lijue surname: Chen fullname: Chen, Lijue organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 6 givenname: Zhewei surname: Yan fullname: Yan, Zhewei organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 7 givenname: Zhixin surname: Chen fullname: Chen, Zhixin organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 8 givenname: Lichuan surname: Chen fullname: Chen, Lichuan organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 9 givenname: Xiaoyan surname: Huang fullname: Huang, Xiaoyan organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 10 givenname: Jie surname: Bai fullname: Bai, Jie organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 11 givenname: Zhaobin surname: Chen fullname: Chen, Zhaobin organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 12 givenname: Jia surname: Shi fullname: Shi, Jia organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 13 givenname: Haiping surname: Xia fullname: Xia, Haiping email: hpxia@xmu.edu.cn organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China – sequence: 14 givenname: Wenjing surname: Hong fullname: Hong, Wenjing email: whong@xmu.edu.cn organization: State Key Laboratory of Physical Chemistry of Solid Surfaces, College of Chemistry and Chemical Engineering, Collaborative Innovation Center of Chemistry for Energy Materials, Xiamen University, 361005 Xiamen, China |
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| Keywords | Quantum Electronics Molecular Electrochemistry Electronic Materials |
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| Title | Electric-Field-Induced Connectivity Switching in Single-Molecule Junctions |
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