Seawater-Mediated Solar-to-Sodium Conversion by Bismuth Vanadate Photoanode- Photovoltaic Tandem Cell: Solar Rechargeable Seawater Battery
Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural...
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| Published in | iScience Vol. 19; pp. 232 - 243 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Inc
27.09.2019
Elsevier |
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| Abstract | Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery.
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•Solar rechargeable battery using natural seawater as a medium was realized•Solar charge was achieved by metal oxide-based photoelectrodes, especially BiVO4•BiVO4-c-Si tandem cell achieved unbiased charge with a high efficiency up to 8%
Electrochemical Energy Conversion; Energy Storage; Materials Characterization |
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| AbstractList | Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery.Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery. Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery. • Solar rechargeable battery using natural seawater as a medium was realized • Solar charge was achieved by metal oxide-based photoelectrodes, especially BiVO 4 • BiVO 4 -c-Si tandem cell achieved unbiased charge with a high efficiency up to 8% Electrochemical Energy Conversion; Energy Storage; Materials Characterization Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery. : Electrochemical Energy Conversion; Energy Storage; Materials Characterization Subject Areas: Electrochemical Energy Conversion, Energy Storage, Materials Characterization Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery. [Display omitted] •Solar rechargeable battery using natural seawater as a medium was realized•Solar charge was achieved by metal oxide-based photoelectrodes, especially BiVO4•BiVO4-c-Si tandem cell achieved unbiased charge with a high efficiency up to 8% Electrochemical Energy Conversion; Energy Storage; Materials Characterization Conversion of sunlight to chemical energy based on photoelectrochemical (PEC) processes has been considered as a promising strategy for solar energy harvesting. Here, we propose a novel platform that converts solar energy into sodium (Na) as a solid-state solar fuel via the PEC oxidation of natural seawater, for which a Na ion-selective ceramic membrane is employed together with photoelectrode (PE)-photovoltaic (PV) tandem cell. Using an elaborately modified bismuth vanadate-based PE in tandem with crystalline silicon PV, we demonstrate unassisted solar-to-Na conversion (equivalent to solar charge of seawater battery) with an unprecedentedly high efficiency of 8% (expected operating point under 1 sun) and measured operation efficiency of 5.7% (0.2 sun) and long-term stability, suggesting a new benchmark for low-cost, efficient, and scalable solid solar fuel production. The sodium turns easily into electricity on demand making the device a nature-friendly, monolithic solar rechargeable seawater battery. |
| Author | Hwang, Inchan Kim, Jeong Hun Kim, Jin Hyun Lee, Jae Sung Hwang, Soo Min Jo, Yim Hyun Seo, Kwanyong Han, Jinhyup Kim, Youngsik |
| AuthorAffiliation | 1 Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea 2 Advanced Center for Energy, Korea Institute of Energy Research (KIER), Ulsan 44919, Republic of Korea 3 Energy Materials and Devices Lab, 4TOONE Corporation, 50 UNIST-gil, Ulsan 44919, Republic of Korea |
| AuthorAffiliation_xml | – name: 1 Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – name: 2 Advanced Center for Energy, Korea Institute of Energy Research (KIER), Ulsan 44919, Republic of Korea – name: 3 Energy Materials and Devices Lab, 4TOONE Corporation, 50 UNIST-gil, Ulsan 44919, Republic of Korea |
| Author_xml | – sequence: 1 givenname: Jin Hyun surname: Kim fullname: Kim, Jin Hyun email: kihi6783@unist.ac.kr organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 2 givenname: Soo Min surname: Hwang fullname: Hwang, Soo Min organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 3 givenname: Inchan surname: Hwang fullname: Hwang, Inchan organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 4 givenname: Jinhyup surname: Han fullname: Han, Jinhyup organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 5 givenname: Jeong Hun surname: Kim fullname: Kim, Jeong Hun organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 6 givenname: Yim Hyun surname: Jo fullname: Jo, Yim Hyun organization: Advanced Center for Energy, Korea Institute of Energy Research (KIER), Ulsan 44919, Republic of Korea – sequence: 7 givenname: Kwanyong surname: Seo fullname: Seo, Kwanyong organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 8 givenname: Youngsik surname: Kim fullname: Kim, Youngsik email: ykim@unist.ac.kr organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea – sequence: 9 givenname: Jae Sung orcidid: 0000-0001-6432-9073 surname: Lee fullname: Lee, Jae Sung email: jlee1234@unist.ac.kr organization: Department of Energy Engineering, School of Energy and Chemical Engineering, Ulsan National Institute of Science & Technology (UNIST), Ulsan 44919, Republic of Korea |
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| Title | Seawater-Mediated Solar-to-Sodium Conversion by Bismuth Vanadate Photoanode- Photovoltaic Tandem Cell: Solar Rechargeable Seawater Battery |
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