The NH Functional Group in Organometallic Catalysis
The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various benef...
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| Published in | Angewandte Chemie International Edition Vol. 52; no. 18; pp. 4744 - 4788 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
26.04.2013
WILEY‐VCH Verlag |
| Subjects | |
| Online Access | Get full text |
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| Abstract | The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst–substrate, ligand–ligand, ligand–catalyst, and catalyst–catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety.
The “magic” effects of NH moieties in organometallic catalysis have been observed in various reaction systems. Recent advances are presented in the development of organometallic catalysts based on the concept of cooperative catalysis by taking the beneficial effect of the NH moiety in the catalyst by catalyst–substrate, ligand–ligand, and catalyst–catalyst interactions. |
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| AbstractList | The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst-substrate, ligand-ligand, ligand-catalyst, and catalyst-catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety. The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst-substrate, ligand-ligand, ligand-catalyst, and catalyst-catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety.The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst-substrate, ligand-ligand, ligand-catalyst, and catalyst-catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety. The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst–substrate, ligand–ligand, ligand–catalyst, and catalyst–catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety. The “magic” effects of NH moieties in organometallic catalysis have been observed in various reaction systems. Recent advances are presented in the development of organometallic catalysts based on the concept of cooperative catalysis by taking the beneficial effect of the NH moiety in the catalyst by catalyst–substrate, ligand–ligand, and catalyst–catalyst interactions. The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an important and attractive concept in catalyst design. NH moieties in the modifiers of organometallic catalysts have been shown to have various beneficial functions in catalysis by molecular recognition through hydrogen bonding to give catalyst-substrate, ligand-ligand, ligand-catalyst, and catalyst-catalyst interactions. This Review summarizes recent progress in the development of the organometallic catalysts based on the concept of cooperative catalysis by focusing on the NH moiety. The "magic" effects of N--H moieties in organometallic catalysis have been observed in various reaction systems. Recent advances are presented in the development of organometallic catalysts based on the concept of cooperative catalysis by taking the beneficial effect of the NH moiety in the catalyst by catalyst-substrate, ligand-ligand, and catalyst-catalyst interactions. |
| Author | Ding, Kuiling Zhao, Baoguo Han, Zhaobin |
| Author_xml | – sequence: 1 givenname: Baoguo surname: Zhao fullname: Zhao, Baoguo organization: Key Laboratory of Resource Chemistry of Ministry of Education, Shanghai Key Laboratory of Rare Earth Functional Materials, Shanghai Normal University, Shanghai 200234 (P.R. China) – sequence: 2 givenname: Zhaobin surname: Han fullname: Han, Zhaobin organization: State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, 345 Lingling Road, Shanghai 200032 (P.R. China) – sequence: 3 givenname: Kuiling surname: Ding fullname: Ding, Kuiling email: kding@mail.sioc.ac.cn organization: State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, 345 Lingling Road, Shanghai 200032 (P.R. China) |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23471875$$D View this record in MEDLINE/PubMed |
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| Snippet | The organometallic approach is one of the most active topics in catalysis. The application of NH functionality in organometallic catalysis has become an... |
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| SubjectTerms | Catalysis Catalysts cooperative catalysis Design engineering Functional groups Hydrogen bonding Metalorganic compounds NH effect organometallic catalysis Recognition self-assembly supramolecular catalysis |
| Title | The NH Functional Group in Organometallic Catalysis |
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