Ultrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature

Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly...

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Published in	Nature communications Vol. 15; no. 1; pp. 3295 - 9
Main Authors	Wu, Tingting, Wang, Chongwu, Hu, Guangwei, Wang, Zhixun, Zhao, Jiaxin, Wang, Zhe, Chaykun, Ksenia, Liu, Lin, Chen, Mengxiao, Li, Dong, Zhu, Song, Xiong, Qihua, Shen, Zexiang, Gao, Huajian, Garcia-Vidal, Francisco J., Wei, Lei, Wang, Qi Jie, Luo, Yu
Format	Journal Article
Language	English
Published	London Nature Publishing Group UK 17.04.2024 Nature Publishing Group Nature Portfolio
Subjects	140/125 140/133 147/135 639/301/1019/1021 639/301/357/1018 639/624/399/1015 639/624/399/1098 639/624/400/2797 Couplings Excitons Heavy metals Humanities and Social Sciences Low dimensional semiconductors Metasurfaces multidisciplinary Multilayers Optoelectronic devices Plasmonics Plasmons Polymers Room temperature Science Science (multidisciplinary) Semiconductors Substrates Transition metal compounds Tungsten Tungsten disulfide
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Abstract	Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS 2 ) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS 2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS 2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors. Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS 2 excitons, achieving ultrastrong exciton-plasmon coupling.
AbstractList	Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS 2 ) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS 2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS 2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors. Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS 2 excitons, achieving ultrastrong exciton-plasmon coupling. Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS 2 ) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS 2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS 2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors. Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS2) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors.Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS2) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors. Abstract Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS2) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors. Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics. Boosting their interaction with light is vital for practical applications, especially in the quantum regime where ultrastrong coupling is highly demanded but not yet realized. Here we report ultrastrong exciton-plasmon coupling at room temperature in tungsten disulfide (WS2) layers loaded with a random multi-singular plasmonic metasurface deposited on a flexible polymer substrate. Different from seeking perfect metals or high-quality resonators, we create a unique type of metasurface with a dense array of singularities that can support nanometre-sized plasmonic hotspots to which several WS2 excitons coherently interact. The associated normalized coupling strength is 0.12 for monolayer WS2 and can be up to 0.164 for quadrilayers, showcasing the ultrastrong exciton-plasmon coupling that is important for practical optoelectronic devices based on low-dimensional semiconductors.Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS2 excitons, achieving ultrastrong exciton-plasmon coupling.
ArticleNumber	3295
Author	Wang, Zhe Shen, Zexiang Chen, Mengxiao Wei, Lei Luo, Yu Chaykun, Ksenia Garcia-Vidal, Francisco J. Hu, Guangwei Gao, Huajian Liu, Lin Wang, Chongwu Zhu, Song Wu, Tingting Wang, Zhixun Li, Dong Xiong, Qihua Wang, Qi Jie Zhao, Jiaxin
Author_xml	– sequence: 1 givenname: Tingting surname: Wu fullname: Wu, Tingting organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 2 givenname: Chongwu orcidid: 0000-0002-8749-196X surname: Wang fullname: Wang, Chongwu organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 3 givenname: Guangwei orcidid: 0000-0002-3023-9632 surname: Hu fullname: Hu, Guangwei organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 4 givenname: Zhixun orcidid: 0000-0001-9918-9939 surname: Wang fullname: Wang, Zhixun organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 5 givenname: Jiaxin surname: Zhao fullname: Zhao, Jiaxin organization: School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 6 givenname: Zhe surname: Wang fullname: Wang, Zhe organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 7 givenname: Ksenia surname: Chaykun fullname: Chaykun, Ksenia organization: School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 8 givenname: Lin surname: Liu fullname: Liu, Lin organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 9 givenname: Mengxiao orcidid: 0000-0001-5853-4791 surname: Chen fullname: Chen, Mengxiao organization: Zhejiang Provincial Key Laboratory of Cardio-Cerebral Vascular Detection Technology and Medicinal Effectiveness Appraisal, Zhejiang University – sequence: 10 givenname: Dong orcidid: 0000-0002-4484-8738 surname: Li fullname: Li, Dong organization: School of Mechanical and Aerospace Engineering, Nanyang Technological University – sequence: 11 givenname: Song surname: Zhu fullname: Zhu, Song organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 12 givenname: Qihua orcidid: 0000-0002-2555-4363 surname: Xiong fullname: Xiong, Qihua organization: State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University – sequence: 13 givenname: Zexiang orcidid: 0000-0001-7432-7936 surname: Shen fullname: Shen, Zexiang organization: School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 14 givenname: Huajian orcidid: 0000-0002-8656-846X surname: Gao fullname: Gao, Huajian organization: School of Mechanical and Aerospace Engineering, Nanyang Technological University – sequence: 15 givenname: Francisco J. orcidid: 0000-0003-4354-0982 surname: Garcia-Vidal fullname: Garcia-Vidal, Francisco J. email: fj.garcia@uam.es organization: Departamento de Física Teorica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Institute of High Performance Computing, Agency for Science, Technology and Research (ASTAR) – sequence: 16 givenname: Lei orcidid: 0000-0003-0819-8325 surname: Wei fullname: Wei, Lei email: wei.lei@ntu.edu.sg organization: School of Electrical and Electronic Engineering, Nanyang Technological University – sequence: 17 givenname: Qi Jie orcidid: 0000-0002-9910-1455 surname: Wang fullname: Wang, Qi Jie email: qjwang@ntu.edu.sg organization: School of Electrical and Electronic Engineering, Nanyang Technological University, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 18 givenname: Yu orcidid: 0000-0003-2925-682X surname: Luo fullname: Luo, Yu email: yu.luo@nuaa.edu.cn organization: National Key Laboratory of Microwave Photonics, Nanjing University of Aeronautics and Astronautics
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Snippet	Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin optoelectronics.... Abstract Van der Waals semiconductors exemplified by two-dimensional transition-metal dichalcogenides have promised next-generation atomically thin...
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SubjectTerms	140/125 140/133 147/135 639/301/1019/1021 639/301/357/1018 639/624/399/1015 639/624/399/1098 639/624/400/2797 Couplings Excitons Heavy metals Humanities and Social Sciences Low dimensional semiconductors Metasurfaces multidisciplinary Multilayers Optoelectronic devices Plasmonics Plasmons Polymers Room temperature Science Science (multidisciplinary) Semiconductors Substrates Transition metal compounds Tungsten Tungsten disulfide
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Title	Ultrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature
URI	https://link.springer.com/article/10.1038/s41467-024-47610-z https://www.proquest.com/docview/3040144572 https://www.proquest.com/docview/3041234846 https://pubmed.ncbi.nlm.nih.gov/PMC11024105 https://doaj.org/article/d6e1caff6d03478eb4968d4b265fb6ca
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