Recent Advances in Visible-Light-Driven Photoelectrochemical Water Splitting: Catalyst Nanostructures and Reaction Systems
Photoelectrochemical(PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint, while there are enormous challenges that still remain for improving solar energy water splitting efficiency, due to limited light harvesting, en...
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Published in | Nano-micro letters Vol. 8; no. 1; pp. 1 - 12 |
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Main Authors | , , , , , |
Format | Journal Article |
Language | English |
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Springer Berlin Heidelberg
01.01.2016
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Abstract | Photoelectrochemical(PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint, while there are enormous challenges that still remain for improving solar energy water splitting efficiency, due to limited light harvesting, energy loss associated to fast recombination of photogenerated charge carriers, as well as electrode degradation. This overview focuses on the recent development about catalyst nanomaterials and nanostructures in different PEC water splitting systems. As photoanode, Au nanoparticle-decorated TiO2 nanowire electrodes exhibited enhanced photoactivity in both the UV and the visible regions due to surface plasmon resonance of Au and showed the largest photocurrent generation of up to 710 nm. Pt/Cd S/CGSe electrodes were developed as photocathode. With the role of p–n heterojunction, the photoelectrode showed high stability and evolved hydrogen continuously for more than 10 days. Further, in the Z-scheme system(Bi2S3/TNA as photoanode and Pt/Si PVC as photocathode at the same time), a self-bias(open-circuit voltage Voc= 0.766 V) was formed between two photoelectrodes, which could facilitate photogenerated charge transfers and enhance the photoelectrochemical performance, and which might provide new hints for PEC water splitting. Meanwhile, the existing problems and prospective solutions have also been reviewed. |
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AbstractList | Photoelectrochemical (PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint, while there are enormous challenges that still remain for improving solar energy water splitting efficiency, due to limited light harvesting, energy loss associated to fast recombination of photogenerated charge carriers, as well as electrode degradation. This overview focuses on the recent development about catalyst nanomaterials and nanostructures in different PEC water splitting systems. As photoanode, Au nanoparticle-decorated TiO
2
nanowire electrodes exhibited enhanced photoactivity in both the UV and the visible regions due to surface plasmon resonance of Au and showed the largest photocurrent generation of up to 710 nm. Pt/CdS/CGSe electrodes were developed as photocathode. With the role of p–n heterojunction, the photoelectrode showed high stability and evolved hydrogen continuously for more than 10 days. Further, in the Z-scheme system (Bi
2
S
3
/TNA as photoanode and Pt/SiPVC as photocathode at the same time), a self-bias (open-circuit voltage
V
oc
= 0.766 V) was formed between two photoelectrodes, which could facilitate photogenerated charge transfers and enhance the photoelectrochemical performance, and which might provide new hints for PEC water splitting. Meanwhile, the existing problems and prospective solutions have also been reviewed. Photoelectrochemical(PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint, while there are enormous challenges that still remain for improving solar energy water splitting efficiency, due to limited light harvesting, energy loss associated to fast recombination of photogenerated charge carriers, as well as electrode degradation. This overview focuses on the recent development about catalyst nanomaterials and nanostructures in different PEC water splitting systems. As photoanode, Au nanoparticle-decorated TiO2 nanowire electrodes exhibited enhanced photoactivity in both the UV and the visible regions due to surface plasmon resonance of Au and showed the largest photocurrent generation of up to 710 nm. Pt/Cd S/CGSe electrodes were developed as photocathode. With the role of p–n heterojunction, the photoelectrode showed high stability and evolved hydrogen continuously for more than 10 days. Further, in the Z-scheme system(Bi2S3/TNA as photoanode and Pt/Si PVC as photocathode at the same time), a self-bias(open-circuit voltage Voc= 0.766 V) was formed between two photoelectrodes, which could facilitate photogenerated charge transfers and enhance the photoelectrochemical performance, and which might provide new hints for PEC water splitting. Meanwhile, the existing problems and prospective solutions have also been reviewed. Photoelectrochemical (PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint, while there are enormous challenges that still remain for improving solar energy water splitting efficiency, due to limited light harvesting, energy loss associated to fast recombination of photogenerated charge carriers, as well as electrode degradation. This overview focuses on the recent development about catalyst nanomaterials and nanostructures in different PEC water splitting systems. As photoanode, Au nanoparticle-decorated TiO nanowire electrodes exhibited enhanced photoactivity in both the UV and the visible regions due to surface plasmon resonance of Au and showed the largest photocurrent generation of up to 710 nm. Pt/CdS/CGSe electrodes were developed as photocathode. With the role of p-n heterojunction, the photoelectrode showed high stability and evolved hydrogen continuously for more than 10 days. Further, in the Z-scheme system (Bi S /TNA as photoanode and Pt/SiPVC as photocathode at the same time), a self-bias (open-circuit voltage = 0.766 V) was formed between two photoelectrodes, which could facilitate photogenerated charge transfers and enhance the photoelectrochemical performance, and which might provide new hints for PEC water splitting. Meanwhile, the existing problems and prospective solutions have also been reviewed. |
Author | Xiaoping Chen Zhixiang Zhang Lina Chi Aathira Krishnadas Nair Wenfeng Shangguan Zheng Jiang |
AuthorAffiliation | Research Center for Combustion and Environment Technology, Shanghai Jiao Tong University;Faculty of Engineering and the Environment, University of Southampton;School of Environmental Science and Technology, Shanghai Jiao Tong University |
Author_xml | – sequence: 1 givenname: Xiaoping surname: Chen fullname: Chen, Xiaoping organization: Research Center for Combustion and Environment Technology, Shanghai Jiao Tong University, Faculty of Engineering and the Environment, University of Southampton – sequence: 2 givenname: Zhixiang surname: Zhang fullname: Zhang, Zhixiang organization: Research Center for Combustion and Environment Technology, Shanghai Jiao Tong University, Faculty of Engineering and the Environment, University of Southampton – sequence: 3 givenname: Lina surname: Chi fullname: Chi, Lina organization: Faculty of Engineering and the Environment, University of Southampton, School of Environmental Science and Technology, Shanghai Jiao Tong University – sequence: 4 givenname: Aathira Krishnadas surname: Nair fullname: Nair, Aathira Krishnadas organization: Faculty of Engineering and the Environment, University of Southampton – sequence: 5 givenname: Wenfeng surname: Shangguan fullname: Shangguan, Wenfeng email: shangguang@sjtu.edu.cn organization: Research Center for Combustion and Environment Technology, Shanghai Jiao Tong University – sequence: 6 givenname: Zheng surname: Jiang fullname: Jiang, Zheng email: Z.Jiang@soton.ac.uk organization: Faculty of Engineering and the Environment, University of Southampton |
BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30464988$$D View this record in MEDLINE/PubMed |
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Keywords | Hybrid systems Heterojuction Photoelectrochemical water splitting Nanostructures Reaction system |
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Notes | 31-2103/TB Xiaoping Chen;Zhixiang Zhang;Lina Chi;Aathira Krishnadas Nair;Wenfeng Shangguan;Zheng Jiang;Research Center for Combustion and Environment Technology, Shanghai Jiao Tong University;Faculty of Engineering and the Environment, University of Southampton;School of Environmental Science and Technology, Shanghai Jiao Tong University ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-3 content type line 23 ObjectType-Review-1 |
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Snippet | Photoelectrochemical(PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint,... Photoelectrochemical (PEC) water splitting using solar energy has attracted great attention for generation of renewable hydrogen with less carbon footprint,... |
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SubjectTerms | Engineering Nanoscale Science and Technology Nanotechnology Nanotechnology and Microengineering Photoelectrochemical Review splitting;Nanostructures;Reaction system;Heterojuction;Hybrid systems water |
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Title | Recent Advances in Visible-Light-Driven Photoelectrochemical Water Splitting: Catalyst Nanostructures and Reaction Systems |
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