High energy resolution CsPbBr3 alpha particle detector with a full-customized readout application specific integrated circuit
α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr 3 crystal...
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| Published in | Nature communications Vol. 15; no. 1; pp. 6333 - 9 |
|---|---|
| Main Authors | , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
27.07.2024
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-024-50746-7 |
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| Abstract | α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr
3
crystal exhibits a low and stable dark current (34.6 nA·cm
−2
at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb
2
Br
5
phase near the surface. The introduction of the Schottky electrode for the CsPbBr
3
detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr
3
detector by reducing the parasitic capacitance and electronic noise.
By developing a synergistic strategy of thinning the perovskite crystal, employing Schottky electrode and full-customised readout application specific integrated circuit to supress dark current and electronic noise, the authors report an energy resolution of 1.1% for perovskite α-particle detector. |
|---|---|
| AbstractList | α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr
3
crystal exhibits a low and stable dark current (34.6 nA·cm
−2
at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb
2
Br
5
phase near the surface. The introduction of the Schottky electrode for the CsPbBr
3
detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr
3
detector by reducing the parasitic capacitance and electronic noise.
By developing a synergistic strategy of thinning the perovskite crystal, employing Schottky electrode and full-customised readout application specific integrated circuit to supress dark current and electronic noise, the authors report an energy resolution of 1.1% for perovskite α-particle detector. Abstract α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr3 crystal exhibits a low and stable dark current (34.6 nA·cm−2 at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb2Br5 phase near the surface. The introduction of the Schottky electrode for the CsPbBr3 detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr3 detector by reducing the parasitic capacitance and electronic noise. α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr3 crystal exhibits a low and stable dark current (34.6 nA·cm-2 at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb2Br5 phase near the surface. The introduction of the Schottky electrode for the CsPbBr3 detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr3 detector by reducing the parasitic capacitance and electronic noise.α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr3 crystal exhibits a low and stable dark current (34.6 nA·cm-2 at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb2Br5 phase near the surface. The introduction of the Schottky electrode for the CsPbBr3 detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr3 detector by reducing the parasitic capacitance and electronic noise. α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer from limited energy resolution, which affects spectroscopy and imaging applications. Here, we report that the solution-grown CsPbBr3 crystal exhibits a low and stable dark current (34.6 nA·cm−2 at 200 V) by thinning the as-grown crystal to decrease the high concentration CsPb2Br5 phase near the surface. The introduction of the Schottky electrode for the CsPbBr3 detector further reduces the dark current and improves the high-temperature stability. An energy resolution of 6.9% is achieved with the commercial electronic system, while the effects of air scattering and absorption are investigated. Moreover, 1.1% energy resolution is recognized by a full-customized readout application-specific integrated circuit without any additional signal processing, which matches well with the given parameters of the CsPbBr3 detector by reducing the parasitic capacitance and electronic noise.By developing a synergistic strategy of thinning the perovskite crystal, employing Schottky electrode and full-customised readout application specific integrated circuit to supress dark current and electronic noise, the authors report an energy resolution of 1.1% for perovskite α-particle detector. |
| ArticleNumber | 6333 |
| Author | Zhang, Xin Ge, Bangzhi Hu, Yongcai Jie, Wanqi Wang, Jia Liu, Jianxi Ouyang, Xiaoping Xu, Yadong Hao, Yingying Fu, Yuhao Bai, Ruichen Peng, Xinkai |
| Author_xml | – sequence: 1 givenname: Xin orcidid: 0000-0001-6972-3184 surname: Zhang fullname: Zhang, Xin organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 2 givenname: Ruichen surname: Bai fullname: Bai, Ruichen organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 3 givenname: Yuhao surname: Fu fullname: Fu, Yuhao organization: School of Electronics and Information, Northwestern Polytechnical University – sequence: 4 givenname: Yingying surname: Hao fullname: Hao, Yingying organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 5 givenname: Xinkai surname: Peng fullname: Peng, Xinkai organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 6 givenname: Jia surname: Wang fullname: Wang, Jia email: jwang@nwpu.edu.cn organization: Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology, School of Electronics and Information, Northwestern Polytechnical University – sequence: 7 givenname: Bangzhi surname: Ge fullname: Ge, Bangzhi organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 8 givenname: Jianxi orcidid: 0000-0002-6394-600X surname: Liu fullname: Liu, Jianxi organization: School of Materials Science and Engineering, Northwestern Polytechnical University – sequence: 9 givenname: Yongcai surname: Hu fullname: Hu, Yongcai organization: Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology, School of Computer Science, Northwestern Polytechnical University – sequence: 10 givenname: Xiaoping surname: Ouyang fullname: Ouyang, Xiaoping email: oyxp2003@aliyun.com organization: Northwest Institute of Nuclear Technology – sequence: 11 givenname: Wanqi surname: Jie fullname: Jie, Wanqi organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology – sequence: 12 givenname: Yadong orcidid: 0000-0002-1017-9337 surname: Xu fullname: Xu, Yadong email: xyd220@nwpu.edu.cn organization: School of Materials Science and Engineering, Northwestern Polytechnical University, Key Laboratory of Radiation Detection Materials and Devices, Ministry of Industry and Information Technology |
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| CitedBy_id | crossref_primary_10_1016_j_ceramint_2025_01_270 crossref_primary_10_1021_acsami_4c21983 crossref_primary_10_1007_s10853_025_10727_7 crossref_primary_10_1002_ifm2_29 crossref_primary_10_1002_adfm_202422522 crossref_primary_10_1021_acs_jpcc_4c07924 crossref_primary_10_3390_ma17215360 crossref_primary_10_1021_acsmaterialslett_4c01559 |
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| Snippet | α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite detectors suffer... Abstract α particles must be monitored to be managed as radioactive diagnostic agents or nuclear activity indicators. The new generation of perovskite... |
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| SubjectTerms | 147/135 147/3 639/301/1005 639/624/1075/1083 Air temperature Alpha particles Alpha rays Application specific integrated circuits Capacitance Crystal growth Customization Dark current Diagnostic agents Electrodes Electronic systems Energy resolution High temperature Humanities and Social Sciences Integrated circuits multidisciplinary Parasitics (electronics) Perovskites Radiation counters Rocket launches Science Science (multidisciplinary) Sensors Signal processing Spectroscopy Surface stability Thinning |
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| Title | High energy resolution CsPbBr3 alpha particle detector with a full-customized readout application specific integrated circuit |
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