Efficient single-component white light emitting diodes enabled by lanthanide ions doped lead halide perovskites via controlling Förster energy transfer and specific defect clearance
Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion segregation. Herein, we report a promising method to fabricate white perovskite LEDs using lanthanide (Ln 3+ ) ions doped CsPbCl 3 perovskit...
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Published in | Light, science & applications Vol. 11; no. 1; p. 340 |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
Published |
London
Nature Publishing Group UK
06.12.2022
Springer Nature B.V Nature Publishing Group |
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Abstract | Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion segregation. Herein, we report a promising method to fabricate white perovskite LEDs using lanthanide (Ln
3+
) ions doped CsPbCl
3
perovskite nanocrystals (PeNCs). First, K
+
ions are doped into the lattice to tune the perovskite bandgap by partially substituting Cs
+
ions, which are well matched to the transition energy of some Ln
3+
ions from the ground state to the excited state, thereby greatly improving the Förster energy transfer efficiency from excitons to Ln
3+
ions. Then, creatine phosphate (CP), a phospholipid widely found in organisms, serves as a tightly binding surface-capping multi-functional ligand which regulates the film formation and enhances the optical and electrical properties of PeNC film. Consequently, the Eu
3+
doped PeNCs based-white LEDs show a peak luminance of 1678 cd m
-2
and a maximum external quantum efficiency (EQE) of 5.4%, demonstrating excellent performance among existing white PeNC LEDs from a single chip. Furthermore, the method of bandgap modulation and the defect passivation were generalized to other Ln
3+
ions doped perovskite LEDs and successfully obtained improved electroluminescence (EL). This work demonstrates the comprehensive and universal strategies in the realization of highly efficient and stable white LEDs via single-component Ln
3+
ions doped PeNCs, which provides an optimal solution for the development of low-cost and simple white perovskite LEDs.
Highly efficient and stable white LEDs were fabricated based on Eu
3+
doped Cs
x
K
1-x
PbCl
3
PeNCs, in which the PeNC film experienced the band engineering and defect passivation treatment. |
---|---|
AbstractList | Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion segregation. Herein, we report a promising method to fabricate white perovskite LEDs using lanthanide (Ln
3+
) ions doped CsPbCl
3
perovskite nanocrystals (PeNCs). First, K
+
ions are doped into the lattice to tune the perovskite bandgap by partially substituting Cs
+
ions, which are well matched to the transition energy of some Ln
3+
ions from the ground state to the excited state, thereby greatly improving the Förster energy transfer efficiency from excitons to Ln
3+
ions. Then, creatine phosphate (CP), a phospholipid widely found in organisms, serves as a tightly binding surface-capping multi-functional ligand which regulates the film formation and enhances the optical and electrical properties of PeNC film. Consequently, the Eu
3+
doped PeNCs based-white LEDs show a peak luminance of 1678 cd m
-2
and a maximum external quantum efficiency (EQE) of 5.4%, demonstrating excellent performance among existing white PeNC LEDs from a single chip. Furthermore, the method of bandgap modulation and the defect passivation were generalized to other Ln
3+
ions doped perovskite LEDs and successfully obtained improved electroluminescence (EL). This work demonstrates the comprehensive and universal strategies in the realization of highly efficient and stable white LEDs via single-component Ln
3+
ions doped PeNCs, which provides an optimal solution for the development of low-cost and simple white perovskite LEDs.
Highly efficient and stable white LEDs were fabricated based on Eu
3+
doped Cs
x
K
1-x
PbCl
3
PeNCs, in which the PeNC film experienced the band engineering and defect passivation treatment. Abstract Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion segregation. Herein, we report a promising method to fabricate white perovskite LEDs using lanthanide (Ln 3+ ) ions doped CsPbCl 3 perovskite nanocrystals (PeNCs). First, K + ions are doped into the lattice to tune the perovskite bandgap by partially substituting Cs + ions, which are well matched to the transition energy of some Ln 3+ ions from the ground state to the excited state, thereby greatly improving the Förster energy transfer efficiency from excitons to Ln 3+ ions. Then, creatine phosphate (CP), a phospholipid widely found in organisms, serves as a tightly binding surface-capping multi-functional ligand which regulates the film formation and enhances the optical and electrical properties of PeNC film. Consequently, the Eu 3+ doped PeNCs based-white LEDs show a peak luminance of 1678 cd m -2 and a maximum external quantum efficiency (EQE) of 5.4%, demonstrating excellent performance among existing white PeNC LEDs from a single chip. Furthermore, the method of bandgap modulation and the defect passivation were generalized to other Ln 3+ ions doped perovskite LEDs and successfully obtained improved electroluminescence (EL). This work demonstrates the comprehensive and universal strategies in the realization of highly efficient and stable white LEDs via single-component Ln 3+ ions doped PeNCs, which provides an optimal solution for the development of low-cost and simple white perovskite LEDs. Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion segregation. Herein, we report a promising method to fabricate white perovskite LEDs using lanthanide (Ln3+) ions doped CsPbCl3 perovskite nanocrystals (PeNCs). First, K+ ions are doped into the lattice to tune the perovskite bandgap by partially substituting Cs+ ions, which are well matched to the transition energy of some Ln3+ ions from the ground state to the excited state, thereby greatly improving the Förster energy transfer efficiency from excitons to Ln3+ ions. Then, creatine phosphate (CP), a phospholipid widely found in organisms, serves as a tightly binding surface-capping multi-functional ligand which regulates the film formation and enhances the optical and electrical properties of PeNC film. Consequently, the Eu3+ doped PeNCs based-white LEDs show a peak luminance of 1678 cd m-2 and a maximum external quantum efficiency (EQE) of 5.4%, demonstrating excellent performance among existing white PeNC LEDs from a single chip. Furthermore, the method of bandgap modulation and the defect passivation were generalized to other Ln3+ ions doped perovskite LEDs and successfully obtained improved electroluminescence (EL). This work demonstrates the comprehensive and universal strategies in the realization of highly efficient and stable white LEDs via single-component Ln3+ ions doped PeNCs, which provides an optimal solution for the development of low-cost and simple white perovskite LEDs.Highly efficient and stable white LEDs were fabricated based on Eu3+ doped CsxK1-xPbCl3 PeNCs, in which the PeNC film experienced the band engineering and defect passivation treatment. Highly efficient and stable white LEDs were fabricated based on Eu3+ doped CsxK1-xPbCl3 PeNCs, in which the PeNC film experienced the band engineering and defect passivation treatment. |
ArticleNumber | 340 |
Author | Liu, Shuainan Wang, Yue Wang, Yuqi Song, Hongwei Xu, Wen Zhou, Donglei Ding, Yujiao Wang, Tianyuan Zhuang, Xinmeng Ding, Nan Sun, Rui |
Author_xml | – sequence: 1 givenname: Rui surname: Sun fullname: Sun, Rui organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 2 givenname: Donglei surname: Zhou fullname: Zhou, Donglei email: zhoudl@jlu.edu.cn organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 3 givenname: Yujiao surname: Ding fullname: Ding, Yujiao organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 4 givenname: Yue surname: Wang fullname: Wang, Yue organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 5 givenname: Yuqi surname: Wang fullname: Wang, Yuqi organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 6 givenname: Xinmeng surname: Zhuang fullname: Zhuang, Xinmeng organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 7 givenname: Shuainan surname: Liu fullname: Liu, Shuainan organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 8 givenname: Nan surname: Ding fullname: Ding, Nan organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 9 givenname: Tianyuan surname: Wang fullname: Wang, Tianyuan organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 10 givenname: Wen surname: Xu fullname: Xu, Wen organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University – sequence: 11 givenname: Hongwei surname: Song fullname: Song, Hongwei email: songhw@jlu.edu.cn organization: State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University |
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Snippet | Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to halide ion... Abstract Currently, a major challenge for metal-halide perovskite light emitting diodes (LEDs) is to achieve stable and efficient white light emission due to... Highly efficient and stable white LEDs were fabricated based on Eu3+ doped CsxK1-xPbCl3 PeNCs, in which the PeNC film experienced the band engineering and... |
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Title | Efficient single-component white light emitting diodes enabled by lanthanide ions doped lead halide perovskites via controlling Förster energy transfer and specific defect clearance |
URI | https://link.springer.com/article/10.1038/s41377-022-01027-9 https://www.proquest.com/docview/2746829633 https://search.proquest.com/docview/2747277163 https://pubmed.ncbi.nlm.nih.gov/PMC9722690 https://doaj.org/article/2117bf45cffd4997a76310eb39425ff8 |
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