Experimental and theoretical studies on induced ferromagnetism of new (1 − x)Na0.5Bi0.5TiO3 + xBaFeO3−δ solid solution

New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO 3− δ materials existed as a well solid solution and resulted in distortion the structure of host Na 0.5 Bi 0.5 TiO 3 materials. The rando...

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Published inScientific reports Vol. 11; no. 1; p. 8908
Main Authors Dung, Dang Duc, Lam, Nguyen Huu, Nguyen, Anh Duc, Trung, Nguyen Ngoc, Van Duc, Nguyen, Hung, Nguyen The, Kim, Yong Soo, Odkhuu, Dorj
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 26.04.2021
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Abstract New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO 3− δ materials existed as a well solid solution and resulted in distortion the structure of host Na 0.5 Bi 0.5 TiO 3 materials. The randomly incorporated Fe and Ba cations in the host Na 0.5 Bi 0.5 TiO 3 crystal decreased the optical band gap from 3.11 to 2.48 eV, and induced the room-temperature ferromagnetism. Our density-functional theory calculations further suggested that both Ba for Bi/Na-site and Fe dopant, regardless of the substitutional sites, in Na 0.5 Bi 0.5 TiO 3 lead to the induced magnetism, which is illustrated in terms of the exchange splitting between spin subbands through the crystal field theory and Jahn–Teller distortion effects. Our work proposes a simple method for fabricating lead-free ferroelectric materials with ferromagnetism property for multifunctional applications in smart electronic devices.
AbstractList New solid solution of Na0.5Bi0.5TiO3 with BaFeO3−δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO3−δ materials existed as a well solid solution and resulted in distortion the structure of host Na0.5Bi0.5TiO3 materials. The randomly incorporated Fe and Ba cations in the host Na0.5Bi0.5TiO3 crystal decreased the optical band gap from 3.11 to 2.48 eV, and induced the room-temperature ferromagnetism. Our density-functional theory calculations further suggested that both Ba for Bi/Na-site and Fe dopant, regardless of the substitutional sites, in Na0.5Bi0.5TiO3 lead to the induced magnetism, which is illustrated in terms of the exchange splitting between spin subbands through the crystal field theory and Jahn–Teller distortion effects. Our work proposes a simple method for fabricating lead-free ferroelectric materials with ferromagnetism property for multifunctional applications in smart electronic devices.
Abstract New solid solution of Na0.5Bi0.5TiO3 with BaFeO3−δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO3−δ materials existed as a well solid solution and resulted in distortion the structure of host Na0.5Bi0.5TiO3 materials. The randomly incorporated Fe and Ba cations in the host Na0.5Bi0.5TiO3 crystal decreased the optical band gap from 3.11 to 2.48 eV, and induced the room-temperature ferromagnetism. Our density-functional theory calculations further suggested that both Ba for Bi/Na-site and Fe dopant, regardless of the substitutional sites, in Na0.5Bi0.5TiO3 lead to the induced magnetism, which is illustrated in terms of the exchange splitting between spin subbands through the crystal field theory and Jahn–Teller distortion effects. Our work proposes a simple method for fabricating lead-free ferroelectric materials with ferromagnetism property for multifunctional applications in smart electronic devices.
Abstract New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO 3− δ materials existed as a well solid solution and resulted in distortion the structure of host Na 0.5 Bi 0.5 TiO 3 materials. The randomly incorporated Fe and Ba cations in the host Na 0.5 Bi 0.5 TiO 3 crystal decreased the optical band gap from 3.11 to 2.48 eV, and induced the room-temperature ferromagnetism. Our density-functional theory calculations further suggested that both Ba for Bi/Na-site and Fe dopant, regardless of the substitutional sites, in Na 0.5 Bi 0.5 TiO 3 lead to the induced magnetism, which is illustrated in terms of the exchange splitting between spin subbands through the crystal field theory and Jahn–Teller distortion effects. Our work proposes a simple method for fabricating lead-free ferroelectric materials with ferromagnetism property for multifunctional applications in smart electronic devices.
New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO 3− δ materials existed as a well solid solution and resulted in distortion the structure of host Na 0.5 Bi 0.5 TiO 3 materials. The randomly incorporated Fe and Ba cations in the host Na 0.5 Bi 0.5 TiO 3 crystal decreased the optical band gap from 3.11 to 2.48 eV, and induced the room-temperature ferromagnetism. Our density-functional theory calculations further suggested that both Ba for Bi/Na-site and Fe dopant, regardless of the substitutional sites, in Na 0.5 Bi 0.5 TiO 3 lead to the induced magnetism, which is illustrated in terms of the exchange splitting between spin subbands through the crystal field theory and Jahn–Teller distortion effects. Our work proposes a simple method for fabricating lead-free ferroelectric materials with ferromagnetism property for multifunctional applications in smart electronic devices.
ArticleNumber 8908
Author Van Duc, Nguyen
Nguyen, Anh Duc
Dung, Dang Duc
Lam, Nguyen Huu
Odkhuu, Dorj
Hung, Nguyen The
Kim, Yong Soo
Trung, Nguyen Ngoc
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– sequence: 2
  givenname: Nguyen Huu
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  fullname: Lam, Nguyen Huu
  organization: School of Engineering Physics, Ha Noi University of Science and Technology
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  fullname: Nguyen, Anh Duc
  organization: School of Engineering Physics, Ha Noi University of Science and Technology, Department of Physics, University of Ulsan
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  givenname: Nguyen Ngoc
  surname: Trung
  fullname: Trung, Nguyen Ngoc
  organization: School of Engineering Physics, Ha Noi University of Science and Technology
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  givenname: Nguyen
  surname: Van Duc
  fullname: Van Duc, Nguyen
  email: duc.nguyenvan1@hust.edu.vn
  organization: School of Electronics and Telecommunications, Ha Noi University of Science and Technology
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  fullname: Hung, Nguyen The
  organization: School of Engineering Physics, Ha Noi University of Science and Technology
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  givenname: Yong Soo
  surname: Kim
  fullname: Kim, Yong Soo
  email: yskim2@ulsan.ac.kr
  organization: Department of Physics, University of Ulsan
– sequence: 8
  givenname: Dorj
  surname: Odkhuu
  fullname: Odkhuu, Dorj
  email: odkhuu@inu.ac.kr
  organization: Department of Physics, Incheon National University
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Snippet New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that...
Abstract New solid solution of Na 0.5 Bi 0.5 TiO 3 with BaFeO 3− δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns...
New solid solution of Na0.5Bi0.5TiO3 with BaFeO3−δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that BaFeO3−δ...
Abstract New solid solution of Na0.5Bi0.5TiO3 with BaFeO3−δ materials were fabricated by sol–gel method. Analysis of X-ray diffraction patterns indicated that...
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SubjectTerms 639/301
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Cations
Electronic equipment
Humanities and Social Sciences
Magnetism
multidisciplinary
Science
Science (multidisciplinary)
Solid solutions
X-ray diffraction
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Title Experimental and theoretical studies on induced ferromagnetism of new (1 − x)Na0.5Bi0.5TiO3 + xBaFeO3−δ solid solution
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