Lifetime over 10000 hours for organic solar cells with Ir/IrOx electron-transporting layer

The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrO x electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surfac...

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Published inNature communications Vol. 14; no. 1; pp. 1241 - 10
Main Authors Li, Yanxun, Huang, Bo, Zhang, Xuning, Ding, Jianwei, Zhang, Yingyu, Xiao, Linge, Wang, Boxin, Cheng, Qian, Huang, Gaosheng, Zhang, Hong, Yang, Yingguo, Qi, Xiaoying, Zheng, Qiang, Zhang, Yuan, Qiu, Xiaohui, Liang, Minghui, Zhou, Huiqiong
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 04.03.2023
Nature Publishing Group
Nature Portfolio
Subjects
140/133
140/146
147/143
147/3
639/301/1005
639/301/357/354
639/4077/909/4101/4096/946
639/925/357
Aging
Devices
Electron transport
Energy distribution
Humanities and Social Sciences
Iridium
Maximum power tracking
multidisciplinary
Nanoparticles
Photovoltaic cells
Recombination
Science
Science (multidisciplinary)
Solar cells
Stability
Surface energy
Surface properties
Work functions
Zinc oxide
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Abstract The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrO x electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrO x -based devices exhibit superior stabilities under shelf storing ( T 80  = 56696 h), thermal aging ( T 70  = 13920 h), and maximum power point tracking ( T 80  = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrO x -based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells. Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the electron-transporting material and realize enhanced device stabilities under thermal aging with T70 of over 10000 h.
AbstractList The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrO x electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrO x -based devices exhibit superior stabilities under shelf storing ( T 80  = 56696 h), thermal aging ( T 70  = 13920 h), and maximum power point tracking ( T 80  = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrO x -based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells. Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the electron-transporting material and realize enhanced device stabilities under thermal aging with T70 of over 10000 h.
Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the electron-transporting material and realize enhanced device stabilities under thermal aging with T70 of over 10000 h.
The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrOx electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrOx-based devices exhibit superior stabilities under shelf storing (T80 = 56696 h), thermal aging (T70 = 13920 h), and maximum power point tracking (T80 = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrOx-based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells.Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the electron-transporting material and realize enhanced device stabilities under thermal aging with T70 of over 10000 h.
The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrO x electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrO x -based devices exhibit superior stabilities under shelf storing ( T 80  = 56696 h), thermal aging ( T 70  = 13920 h), and maximum power point tracking ( T 80  = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrO x -based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells.
The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrOx electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrOx-based devices exhibit superior stabilities under shelf storing (T80 = 56696 h), thermal aging (T70 = 13920 h), and maximum power point tracking (T80 = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrOx-based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells.The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar cells is enhanced by an Ir/IrOx electron-transporting layer, benefiting from its suitable work function and heterogeneous distribution of surface energy in nanoscale. Notably, the champion Ir/IrOx-based devices exhibit superior stabilities under shelf storing (T80 = 56696 h), thermal aging (T70 = 13920 h), and maximum power point tracking (T80 = 1058 h), compared to the ZnO-based devices. It can be attributed to the stable morphology of photoactive layer resulting from the optimized molecular distribution of the donor and acceptor and the absence of photocatalysis in the Ir/IrOx-based devices, which helps to maintain the improved charge extraction and inhibited charge recombination in the aged devices. This work provides a reliable and efficient electron-transporting material toward stable organic solar cells.
ArticleNumber 1241
Author Cheng, Qian
Xiao, Linge
Huang, Gaosheng
Zhang, Hong
Wang, Boxin
Zhou, Huiqiong
Yang, Yingguo
Huang, Bo
Ding, Jianwei
Qi, Xiaoying
Qiu, Xiaohui
Zhang, Xuning
Zhang, Yingyu
Zheng, Qiang
Li, Yanxun
Zhang, Yuan
Liang, Minghui
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  orcidid: 0000-0002-1749-2799
  surname: Yang
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  organization: Shanghai Synchrotron Radiation Facility (SSRF), Zhangjiang Lab, Shanghai Advanced Research Institute, Chinese Academy of Sciences
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  email: zhouhq@nanoctr.cn
  organization: CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences
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Snippet The stability of organic solar cells is a key issue to promote practical applications. Herein, we demonstrate that the device performance of organic solar...
Long-term stability of organic solar cells is critical to promote practical applications. Here, the authors utilize iridium/iridium oxide nanoparticles as the...
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SubjectTerms 140/133
140/146
147/143
147/3
639/301/1005
639/301/357/354
639/4077/909/4101/4096/946
639/925/357
Aging
Devices
Electron transport
Energy distribution
Humanities and Social Sciences
Iridium
Maximum power tracking
multidisciplinary
Nanoparticles
Photovoltaic cells
Recombination
Science
Science (multidisciplinary)
Solar cells
Stability
Surface energy
Surface properties
Work functions
Zinc oxide
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Title Lifetime over 10000 hours for organic solar cells with Ir/IrOx electron-transporting layer
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Volume 14
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