Bond engineering of molecular ferroelectrics renders soft and high-performance piezoelectric energy harvesting materials

Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their appli...

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Published inNature communications Vol. 13; no. 1; pp. 5607 - 10
Main Authors Hu, Yuzhong, Parida, Kaushik, Zhang, Hao, Wang, Xin, Li, Yongxin, Zhou, Xinran, Morris, Samuel Alexander, Liew, Weng Heng, Wang, Haomin, Li, Tao, Jiang, Feng, Yang, Mingmin, Alexe, Marin, Du, Zehui, Gan, Chee Lip, Yao, Kui, Xu, Bin, Lee, Pooi See, Fan, Hong Jin
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 24.09.2022
Nature Publishing Group
Nature Portfolio
Subjects
119/118
142/136
639/301/119/1002
639/301/119/996
639/4077/4072/4062
639/638/298/917
Bonding strength
Chemical bonds
Crystal structure
Electric potential
Energy
Energy harvesting
Engineering
Ferroelectric materials
Ferroelectricity
Ferroelectrics
Humanities and Social Sciences
Laboratories
Metal halides
multidisciplinary
Phase transitions
Piezoelectricity
Science
Science (multidisciplinary)
Shear strain
Softness
Solid solutions
Strain
Voltage
Wearable computers
Wearable technology
Online AccessGet full text

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Abstract Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C 6 H 5 N(CH 3 ) 3 CdBr 2 Cl 0.75 I 0.25 exhibits excellent piezoelectric constants ( d 33  = 367 pm/V, g 33  = 3595 × 10 −3  Vm/N), energy harvesting property (power density is 11 W/m 2 ), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics. Improving piezoelectric strain and voltage constant generally compromises piezoelectric performance and mechanical softness. Here, the authors report a bond weakening strategy for organic-inorganic hybrid piezoelectrics and mitigated these issues.
AbstractList Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C6H5N(CH3)3CdBr2Cl0.75I0.25 exhibits excellent piezoelectric constants (d33 = 367 pm/V, g33 = 3595 × 10−3 Vm/N), energy harvesting property (power density is 11 W/m2), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics.Improving piezoelectric strain and voltage constant generally compromises piezoelectric performance and mechanical softness. Here, the authors report a bond weakening strategy for organic-inorganic hybrid piezoelectrics and mitigated these issues.
Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C 6 H 5 N(CH 3 ) 3 CdBr 2 Cl 0.75 I 0.25 exhibits excellent piezoelectric constants ( d 33  = 367 pm/V, g 33  = 3595 × 10 −3  Vm/N), energy harvesting property (power density is 11 W/m 2 ), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics. Improving piezoelectric strain and voltage constant generally compromises piezoelectric performance and mechanical softness. Here, the authors report a bond weakening strategy for organic-inorganic hybrid piezoelectrics and mitigated these issues.
Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C 6 H 5 N(CH 3 ) 3 CdBr 2 Cl 0.75 I 0.25 exhibits excellent piezoelectric constants ( d 33  = 367 pm/V, g 33  = 3595 × 10 −3  Vm/N), energy harvesting property (power density is 11 W/m 2 ), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics.
Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C6H5N(CH3)3CdBr2Cl0.75I0.25 exhibits excellent piezoelectric constants (d33 = 367 pm/V, g33 = 3595 × 10-3 Vm/N), energy harvesting property (power density is 11 W/m2), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics.Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the piezoelectric family, there are two pairs of properties that improving one of them will generally compromises the other, which limits their applications. The first pair is piezoelectric strain and voltage constant, and the second is piezoelectric performance and mechanical softness. Here, we report a molecular bond weakening strategy to mitigate these issues in organic-inorganic hybrid piezoelectrics. By introduction of large-size halide elements, the metal-halide bonds can be effectively weakened, leading to a softening effect on bond strength and reduction in polarization switching barrier. The obtained solid solution C6H5N(CH3)3CdBr2Cl0.75I0.25 exhibits excellent piezoelectric constants (d33 = 367 pm/V, g33 = 3595 × 10-3 Vm/N), energy harvesting property (power density is 11 W/m2), and superior mechanical softness (0.8 GPa), promising this hybrid as high-performance soft piezoelectrics.
Improving piezoelectric strain and voltage constant generally compromises piezoelectric performance and mechanical softness. Here, the authors report a bond weakening strategy for organic-inorganic hybrid piezoelectrics and mitigated these issues.
ArticleNumber 5607
Author Jiang, Feng
Morris, Samuel Alexander
Du, Zehui
Wang, Xin
Liew, Weng Heng
Gan, Chee Lip
Yang, Mingmin
Zhang, Hao
Yao, Kui
Xu, Bin
Wang, Haomin
Li, Tao
Zhou, Xinran
Hu, Yuzhong
Fan, Hong Jin
Alexe, Marin
Lee, Pooi See
Li, Yongxin
Parida, Kaushik
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  organization: School of Physical and Mathematical Sciences, Nanyang Technological University
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Grimme, S. Semiempirical GGA-type density functional constructed with a long-range dispersion correction. 27, 1787–1799, https://doi.org/10.1002/jcc.20495 (2006).
LingYDisruptive, soft, wearable sensorsAdv. Mater.20203219046641:CAS:528:DC%2BC1MXitFCjtrvJ10.1002/adma.201904664
SunSFactors influencing the mechanical properties of formamidinium lead halides and related hybrid perovskitesChemSusChem.201710374037451:CAS:528:DC%2BC2sXht1eksbnL2866607910.1002/cssc.201700991
KresseGHafnerJAb initio molecular dynamics for liquid metalsPhys. Rev. B1993475585611993PhRvB..47..558K1:CAS:528:DyaK3sXlt1Gnsr0%3D10.1103/PhysRevB.47.558
LimH-RAdvanced soft materials, sensor integrations, and applications of wearable flexible hybrid electronics in healthcare, energy, and environmentAdv. Mater.20203219019241:CAS:528:DC%2BC1MXhtlejtrvN10.1002/adma.201901924
LiuYFerroelectric polymers exhibiting behaviour reminiscent of a morphotropic phase boundaryNature2018562961002018Natur.562...96L1:CAS:528:DC%2BC1cXhvVOjsLfK3028310210.1038/s41586-018-0550-z
Sheppard, D., Terrell, R. & Henkelman, G. Optimization methods for finding minimum energy paths. 128, 134106, https://doi.org/10.1063/1.2841941 (2008).
ChenX-GTwo-dimensional layered perovskite ferroelectric with giant piezoelectric voltage coefficientJ. Am. Chem. Soc.2020142107710821:CAS:528:DC%2BC1MXisVekt73I3185149510.1021/jacs.9b12368
QiuCTransparent ferroelectric crystals with ultrahigh piezoelectricityNature20205773503542020Natur.577..350Q1:CAS:528:DC%2BB3cXjsVejsrk%3D3194205510.1038/s41586-019-1891-y
Uchino, K. Advanced piezoelectric materials: Science and technology. (Woodhead Publishing, 2017).
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LiuHGiant piezoelectricity in oxide thin films with nanopillar structureScience20203692922972020Sci...369..292L1:CAS:528:DC%2BB3cXhsVSjtLfN3267537010.1126/science.abb3209
SongH-CPiezoelectric energy harvesting design principles for materials and structures: Material figure-of-merit and self-resonance tuningAdv. Mater.20203220022081:CAS:528:DC%2BB3cXhvFyqtr%2FJ10.1002/adma.202002208
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FragaMAFurlanHPessoaRSMassiMWide bandgap semiconductor thin films for piezoelectric and piezoresistive MEMS sensors applied at high temperatures: an overviewMicrosyst. Technol.2014209211:CAS:528:DC%2BC3sXhvFyksr%2FI10.1007/s00542-013-2029-z
LiaoW-QA molecular perovskite solid solution with piezoelectricity stronger than lead zirconate titanateScience2019363120612102019Sci...363.1206L1:CAS:528:DC%2BC1MXks1yrsr4%3D3087252210.1126/science.aav3057
JiL-JSunS-JQinYLiKLiWMechanical properties of hybrid organic-inorganic perovskitesCoord. Chem. Rev.201939115291:CAS:528:DC%2BC1MXnsFGht7Y%3D10.1016/j.ccr.2019.03.020
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TuQExploring the factors affecting the mechanical properties of 2D hybrid organic–inorganic perovskitesACS Appl. Mater. Interfaces20201220440204471:CAS:528:DC%2BB3cXmvV2qtLk%3D3227513210.1021/acsami.0c02313
CoondooIEnhanced Piezoelectric Properties of Praseodymium-Modified Lead-Free (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3 CeramicsJ. Am. Ceram. Soc.201598312731351:CAS:528:DC%2BC2MXhtVOrsbzN10.1111/jace.13713
MaintzSDeringerVLTchougréeffALDronskowskiRLOBSTER: A tool to extract chemical bonding from plane-wave based DFTJ. Computational Chem.201637103010351:CAS:528:DC%2BC28XjsVamtrg%3D10.1002/jcc.24300
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FanXDingYLiuYLiangJChenYPlasmonic Ti3C2Tx MXene enables highly efficient photothermal conversion for healable and transparent wearable deviceACS Nano.201913812481341:CAS:528:DC%2BC1MXhtF2ksb%2FO3124404610.1021/acsnano.9b03161
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YangM-MPiezoelectric and pyroelectric effects induced by interface polar symmetryNature20205843773811:CAS:528:DC%2BB3cXhs1Cju7fP3281489010.1038/s41586-020-2602-4
HanMThree-dimensional piezoelectric polymer microsystems for vibrational energy harvesting, robotic interfaces and biomedical implantsNat. Electron.20192263510.1038/s41928-018-0189-7
HaoJLiWZhaiJChenHProgress in high-strain perovskite piezoelectric ceramicsMater. Sci. Eng.: R: Rep.201913515710.1016/j.mser.2018.08.001
KuiYTayFEHMeasurement of longitudinal piezoelectric coefficient of thin films by a laser-scanning vibrometerIEEE Trans. Ultrason., Ferroelectr., Frequency Control20035011311610.1109/TUFFC.2003.1182115
LiWMechanical tunability via hydrogen bonding in metal–organic frameworks with the perovskite architectureJ. Am. Chem. Soc.2014136780178041:CAS:528:DC%2BC2cXns12jtL4%3D2481531910.1021/ja500618z
LiTHigh-Performance Poly(vinylidene difluoride)/Dopamine Core/Shell Piezoelectric nanofiber and its application for biomedical sensorsAdv. Mater.20213320060931:CAS:528:DC%2BB3cXisVyitrnO10.1002/adma.202006093
PanMTriboelectric and Piezoelectric nanogenerators for future soft robots and machinesiScience2020231016822020iSci...23j1682P33163937760742410.1016/j.isci.2020.101682
SalvadoriMCBrownIGVazARMeloLLCattaniMMeasurement of the elastic modulus of nanostructured gold and platinum thin filmsPhys. Rev. B2003671534042003PhRvB..67o3404S10.1103/PhysRevB.67.153404
AizuKPossible Species of “Ferroelastic” crystals and of simultaneously ferroelectric and ferroelastic crystalsJ. Phys. Soc. Jpn.1969273873961969JPSJ...27..387A1:CAS:528:DyaF1MXltFOhurw%3D10.1143/JPSJ.27.387
YanMPorous ferroelectric materials for energy technologies: Current status and future perspectivesEnergy. Environ. Sci.202114615861901:CAS:528:DC%2BB3MXisVentb7I10.1039/D1EE03025F
DamjanovicDDemartinMThe Rayleigh law in piezoelectric ceramicsJ. Phys. D: Appl. Phys.199629205720601996JPhD...29.2057D1:CAS:528:DyaK28XksFCls7s%3D10.1088/0022-3727/29/7/046
ShuLPhotoflexoelectric effect in halide perovskitesNat. Mater.2020196056092020NatMa..19..605S1:CAS:528:DC%2BB3cXnsFarur8%3D3231326510.1038/s41563-020-0659-y
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SenguptaDCharacterization of single polyvinylidene fluoride (PVDF) nanofiber for flow sensing applicationsAIP Adv.201771052052017AIPA....7j5205S10.1063/1.4994968
FuD-WDiisopropylammonium bromide is a high-temperature molecular ferroelectric crystalScience20133394254282013Sci...339..425F1:CAS:528:DC%2BC3sXhtFynsb0%3D2334928510.1126/science.1229675
YouYMAn organic-inorganic perovskite ferroelectric with large piezoelectric responseScience20173573063092017Sci...357..306Y1:CAS:528:DC%2BC2sXhtFygs73L2872951110.1126/science.aai8535
DesirajuGRHydrogen bridges in crystal engineering:  Interactions without BordersAcc. Chem. Res.2002355655731:CAS:528:DC%2BD38Xjt1Ojsrs%3D1211899610.1021/ar010054t
LiFUltrahigh piezoelectricity in ferroelectric ceramics by designNat. Mater.2018173493542018JNuM..502..349L1:CAS:528:DC%2BC1cXlvFKnsLw%3D2955599910.1038/s41563-018-0034-4
Xu, R. & Kim, S. Figures of merits of piezoelectric materials in energy harvesters. Proceed. PowerMEMS, 464–467 (2012).
DeringerVLTchougréeffALDronskowskiRCrystal Orbital Hamilton Population (COHP) Analysis As Projected from Plane-Wave Basis SetsJ. Phys. Chem. A2011115546154661:CAS:528:DC%2BC3MXlslKitr8%3D2154859410.1021/jp202489s
PerdewJPBurkeKErnzerhofMGeneralized gradient approximation made simplePhys. Rev. Lett.199677386538681996PhRvL..77.3865P1:CAS:528:DyaK28XmsVCgsbs%3D1006232810.1103/PhysRevLett.77.3865
HuYFerroelastic-switching-driven large shear strain and piezoelectricity in a hybrid ferroelectricNat. Mater.2021206126172021NatMa..20..612H1:CAS:528:DC%2BB3MXhtF2qtr4%3D3343214710.1038/s41563-020-00875-3
YangZZhouSZuJInmanDHigh-performance piezoelectric energy harvesters and their applicationsJoule201826426971:CAS:528:DC%2BC1cXpsFOnur4%3D10.1016/j.joule.2018.03.011
Z Yang (33325_CR6) 2018; 2
Y Kui (33325_CR31) 2003; 50
S Maintz (33325_CR50) 2016; 37
X Fan (33325_CR43) 2019; 13
M Pan (33325_CR3) 2020; 23
L Orgéas (33325_CR26) 1998; 46
J Hao (33325_CR29) 2019; 135
S Sun (33325_CR38) 2017; 10
D-W Fu (33325_CR35) 2013; 339
H-C Song (33325_CR14) 2020; 32
Y Hu (33325_CR23) 2021; 20
GR Desiraju (33325_CR41) 2002; 35
K Aizu (33325_CR25) 1969; 27
33325_CR47
C Qiu (33325_CR42) 2020; 577
J Merker (33325_CR36) 2001; 45
G Kresse (33325_CR44) 1993; 47
33325_CR48
W-Q Liao (33325_CR22) 2019; 363
L Bellaiche (33325_CR34) 1999; 83
Q Tu (33325_CR40) 2020; 12
MC Salvadori (33325_CR37) 2003; 67
L Shu (33325_CR20) 2020; 19
YM You (33325_CR18) 2017; 357
Y Liu (33325_CR13) 2018; 562
D Damjanovic (33325_CR28) 1997; 82
D Viehland (33325_CR30) 2004; 95
D Sengupta (33325_CR12) 2017; 7
MA Fraga (33325_CR10) 2014; 20
PK Panda (33325_CR9) 2015; 474
D Damjanovic (33325_CR33) 1996; 29
G Kresse (33325_CR45) 1996; 54
L-J Ji (33325_CR24) 2019; 391
I Coondoo (33325_CR15) 2015; 98
Y Ling (33325_CR7) 2020; 32
W Li (33325_CR39) 2014; 136
VL Deringer (33325_CR49) 2011; 115
H-R Lim (33325_CR8) 2020; 32
M Han (33325_CR4) 2019; 2
H Liu (33325_CR32) 2020; 369
X Liu (33325_CR19) 2019; 58
M-M Yang (33325_CR27) 2020; 584
T Someya (33325_CR5) 2016; 540
X-G Chen (33325_CR21) 2020; 142
T Li (33325_CR11) 2021; 33
F Li (33325_CR16) 2018; 17
JP Perdew (33325_CR46) 1996; 77
M Yan (33325_CR2) 2021; 14
33325_CR1
33325_CR17
References_xml – reference: LiuHGiant piezoelectricity in oxide thin films with nanopillar structureScience20203692922972020Sci...369..292L1:CAS:528:DC%2BB3cXhsVSjtLfN3267537010.1126/science.abb3209
– reference: PandaPKSahooBPZT to lead free piezo ceramics: A ReviewFerroelectrics20154741281431:CAS:528:DC%2BC2MXjslOqtL8%3D10.1080/00150193.2015.997146
– reference: DeringerVLTchougréeffALDronskowskiRCrystal Orbital Hamilton Population (COHP) Analysis As Projected from Plane-Wave Basis SetsJ. Phys. Chem. A2011115546154661:CAS:528:DC%2BC3MXlslKitr8%3D2154859410.1021/jp202489s
– reference: SunSFactors influencing the mechanical properties of formamidinium lead halides and related hybrid perovskitesChemSusChem.201710374037451:CAS:528:DC%2BC2sXht1eksbnL2866607910.1002/cssc.201700991
– reference: ChenX-GTwo-dimensional layered perovskite ferroelectric with giant piezoelectric voltage coefficientJ. Am. Chem. Soc.2020142107710821:CAS:528:DC%2BC1MXisVekt73I3185149510.1021/jacs.9b12368
– reference: FragaMAFurlanHPessoaRSMassiMWide bandgap semiconductor thin films for piezoelectric and piezoresistive MEMS sensors applied at high temperatures: an overviewMicrosyst. Technol.2014209211:CAS:528:DC%2BC3sXhvFyksr%2FI10.1007/s00542-013-2029-z
– reference: OrgéasLFavierDStress-induced martensitic transformation of a NiTi alloy in isothermal shear, tension and compressionActa. Mater.199846557955911998AcMat..46.5579O10.1016/S1359-6454(98)00167-0
– reference: YangZZhouSZuJInmanDHigh-performance piezoelectric energy harvesters and their applicationsJoule201826426971:CAS:528:DC%2BC1cXpsFOnur4%3D10.1016/j.joule.2018.03.011
– reference: LiuXPolarization-driven self-powered photodetection in a single-phase biaxial hybrid perovskite ferroelectricAngew. Chem. Int. Ed.20195814504145081:CAS:528:DC%2BC1MXhslWkurjF10.1002/anie.201907660
– reference: HaoJLiWZhaiJChenHProgress in high-strain perovskite piezoelectric ceramicsMater. Sci. Eng.: R: Rep.201913515710.1016/j.mser.2018.08.001
– reference: JiL-JSunS-JQinYLiKLiWMechanical properties of hybrid organic-inorganic perovskitesCoord. Chem. Rev.201939115291:CAS:528:DC%2BC1MXnsFGht7Y%3D10.1016/j.ccr.2019.03.020
– reference: SongH-CPiezoelectric energy harvesting design principles for materials and structures: Material figure-of-merit and self-resonance tuningAdv. Mater.20203220022081:CAS:528:DC%2BB3cXhvFyqtr%2FJ10.1002/adma.202002208
– reference: TuQExploring the factors affecting the mechanical properties of 2D hybrid organic–inorganic perovskitesACS Appl. Mater. Interfaces20201220440204471:CAS:528:DC%2BB3cXmvV2qtLk%3D3227513210.1021/acsami.0c02313
– reference: AizuKPossible Species of “Ferroelastic” crystals and of simultaneously ferroelectric and ferroelastic crystalsJ. Phys. Soc. Jpn.1969273873961969JPSJ...27..387A1:CAS:528:DyaF1MXltFOhurw%3D10.1143/JPSJ.27.387
– reference: Grimme, S. Semiempirical GGA-type density functional constructed with a long-range dispersion correction. 27, 1787–1799, https://doi.org/10.1002/jcc.20495 (2006).
– reference: FuD-WDiisopropylammonium bromide is a high-temperature molecular ferroelectric crystalScience20133394254282013Sci...339..425F1:CAS:528:DC%2BC3sXhtFynsb0%3D2334928510.1126/science.1229675
– reference: YouYMAn organic-inorganic perovskite ferroelectric with large piezoelectric responseScience20173573063092017Sci...357..306Y1:CAS:528:DC%2BC2sXhtFygs73L2872951110.1126/science.aai8535
– reference: MerkerJLuptonDTopferMKnakeHHigh temperature mechanical properties of the platinum group metalsPlatin. Met. Rev.(UK)20014574821:CAS:528:DC%2BD3MXltVOgsLg%3D
– reference: LiTHigh-Performance Poly(vinylidene difluoride)/Dopamine Core/Shell Piezoelectric nanofiber and its application for biomedical sensorsAdv. Mater.20213320060931:CAS:528:DC%2BB3cXisVyitrnO10.1002/adma.202006093
– reference: Xu, R. & Kim, S. Figures of merits of piezoelectric materials in energy harvesters. Proceed. PowerMEMS, 464–467 (2012).
– reference: PanMTriboelectric and Piezoelectric nanogenerators for future soft robots and machinesiScience2020231016822020iSci...23j1682P33163937760742410.1016/j.isci.2020.101682
– reference: PerdewJPBurkeKErnzerhofMGeneralized gradient approximation made simplePhys. Rev. Lett.199677386538681996PhRvL..77.3865P1:CAS:528:DyaK28XmsVCgsbs%3D1006232810.1103/PhysRevLett.77.3865
– reference: KresseGFurthmüllerJEfficient iterative schemes for ab initio total-energy calculations using a plane-wave basis setPhys. Rev. B19965411169111861996PhRvB..5411169K1:CAS:528:DyaK28Xms1Whu7Y%3D10.1103/PhysRevB.54.11169
– reference: HanMThree-dimensional piezoelectric polymer microsystems for vibrational energy harvesting, robotic interfaces and biomedical implantsNat. Electron.20192263510.1038/s41928-018-0189-7
– reference: DamjanovicDStress and frequency dependence of the direct piezoelectric effect in ferroelectric ceramicsJ. Appl. Phys.199782178817971997JAP....82.1788D1:CAS:528:DyaK2sXlsFSjsLc%3D10.1063/1.365981
– reference: HuYFerroelastic-switching-driven large shear strain and piezoelectricity in a hybrid ferroelectricNat. Mater.2021206126172021NatMa..20..612H1:CAS:528:DC%2BB3MXhtF2qtr4%3D3343214710.1038/s41563-020-00875-3
– reference: SomeyaTBaoZMalliarasGGThe rise of plastic bioelectronicsNature20165403793852016Natur.540..379S1:CAS:528:DC%2BC28XitVyru7%2FO2797476910.1038/nature21004
– reference: KresseGHafnerJAb initio molecular dynamics for liquid metalsPhys. Rev. B1993475585611993PhRvB..47..558K1:CAS:528:DyaK3sXlt1Gnsr0%3D10.1103/PhysRevB.47.558
– reference: DamjanovicDDemartinMThe Rayleigh law in piezoelectric ceramicsJ. Phys. D: Appl. Phys.199629205720601996JPhD...29.2057D1:CAS:528:DyaK28XksFCls7s%3D10.1088/0022-3727/29/7/046
– reference: MaintzSDeringerVLTchougréeffALDronskowskiRLOBSTER: A tool to extract chemical bonding from plane-wave based DFTJ. Computational Chem.201637103010351:CAS:528:DC%2BC28XjsVamtrg%3D10.1002/jcc.24300
– reference: QiuCTransparent ferroelectric crystals with ultrahigh piezoelectricityNature20205773503542020Natur.577..350Q1:CAS:528:DC%2BB3cXjsVejsrk%3D3194205510.1038/s41586-019-1891-y
– reference: YangM-MPiezoelectric and pyroelectric effects induced by interface polar symmetryNature20205843773811:CAS:528:DC%2BB3cXhs1Cju7fP3281489010.1038/s41586-020-2602-4
– reference: LingYDisruptive, soft, wearable sensorsAdv. Mater.20203219046641:CAS:528:DC%2BC1MXitFCjtrvJ10.1002/adma.201904664
– reference: DesirajuGRHydrogen bridges in crystal engineering:  Interactions without BordersAcc. Chem. Res.2002355655731:CAS:528:DC%2BD38Xjt1Ojsrs%3D1211899610.1021/ar010054t
– reference: ShuLPhotoflexoelectric effect in halide perovskitesNat. Mater.2020196056092020NatMa..19..605S1:CAS:528:DC%2BB3cXnsFarur8%3D3231326510.1038/s41563-020-0659-y
– reference: SalvadoriMCBrownIGVazARMeloLLCattaniMMeasurement of the elastic modulus of nanostructured gold and platinum thin filmsPhys. Rev. B2003671534042003PhRvB..67o3404S10.1103/PhysRevB.67.153404
– reference: LiuYFerroelectric polymers exhibiting behaviour reminiscent of a morphotropic phase boundaryNature2018562961002018Natur.562...96L1:CAS:528:DC%2BC1cXhvVOjsLfK3028310210.1038/s41586-018-0550-z
– reference: YanMPorous ferroelectric materials for energy technologies: Current status and future perspectivesEnergy. Environ. Sci.202114615861901:CAS:528:DC%2BB3MXisVentb7I10.1039/D1EE03025F
– reference: Sheppard, D., Terrell, R. & Henkelman, G. Optimization methods for finding minimum energy paths. 128, 134106, https://doi.org/10.1063/1.2841941 (2008).
– reference: Uchino, K. Advanced piezoelectric materials: Science and technology. (Woodhead Publishing, 2017).
– reference: KuiYTayFEHMeasurement of longitudinal piezoelectric coefficient of thin films by a laser-scanning vibrometerIEEE Trans. Ultrason., Ferroelectr., Frequency Control20035011311610.1109/TUFFC.2003.1182115
– reference: CoondooIEnhanced Piezoelectric Properties of Praseodymium-Modified Lead-Free (Ba0.85Ca0.15)(Ti0.90Zr0.10)O3 CeramicsJ. Am. Ceram. Soc.201598312731351:CAS:528:DC%2BC2MXhtVOrsbzN10.1111/jace.13713
– reference: LiaoW-QA molecular perovskite solid solution with piezoelectricity stronger than lead zirconate titanateScience2019363120612102019Sci...363.1206L1:CAS:528:DC%2BC1MXks1yrsr4%3D3087252210.1126/science.aav3057
– reference: LiWMechanical tunability via hydrogen bonding in metal–organic frameworks with the perovskite architectureJ. Am. Chem. Soc.2014136780178041:CAS:528:DC%2BC2cXns12jtL4%3D2481531910.1021/ja500618z
– reference: SenguptaDCharacterization of single polyvinylidene fluoride (PVDF) nanofiber for flow sensing applicationsAIP Adv.201771052052017AIPA....7j5205S10.1063/1.4994968
– reference: FanXDingYLiuYLiangJChenYPlasmonic Ti3C2Tx MXene enables highly efficient photothermal conversion for healable and transparent wearable deviceACS Nano.201913812481341:CAS:528:DC%2BC1MXhtF2ksb%2FO3124404610.1021/acsnano.9b03161
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Snippet Piezoelectric materials convert mechanical stress to electrical energy and thus are widely used in energy harvesting and wearable devices. However, in the...
Improving piezoelectric strain and voltage constant generally compromises piezoelectric performance and mechanical softness. Here, the authors report a bond...
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SubjectTerms 119/118
142/136
639/301/119/1002
639/301/119/996
639/4077/4072/4062
639/638/298/917
Bonding strength
Chemical bonds
Crystal structure
Electric potential
Energy
Energy harvesting
Engineering
Ferroelectric materials
Ferroelectricity
Ferroelectrics
Humanities and Social Sciences
Laboratories
Metal halides
multidisciplinary
Phase transitions
Piezoelectricity
Science
Science (multidisciplinary)
Shear strain
Softness
Solid solutions
Strain
Voltage
Wearable computers
Wearable technology
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Title Bond engineering of molecular ferroelectrics renders soft and high-performance piezoelectric energy harvesting materials
URI https://link.springer.com/article/10.1038/s41467-022-33325-6
https://www.proquest.com/docview/2717360389
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https://pubmed.ncbi.nlm.nih.gov/PMC9509372
https://doaj.org/article/5270b427ae8b4360805a5f095f4c2fd8
Volume 13
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