Bandgap control in two-dimensional semiconductors via coherent doping of plasmonic hot electrons
Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimens...
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| Published in | Nature communications Vol. 12; no. 1; pp. 4332 - 8 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
15.07.2021
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-021-24667-8 |
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| Abstract | Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS
2
) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS
2
conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices.
The established means of bandgap control in semiconductors are based on chemical, electrical or optical doping. Here, the authors report wide bandgap modulations in monolayer WS2 at room temperature by coupling the 2D semiconductor to a self-assembled plasmonic crystal inducing coherent hot electron doping. |
|---|---|
| AbstractList | Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS
2
) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS
2
conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices. Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS2) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS2 conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices.Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS2) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS2 conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices. Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS 2 ) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS 2 conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices. The established means of bandgap control in semiconductors are based on chemical, electrical or optical doping. Here, the authors report wide bandgap modulations in monolayer WS2 at room temperature by coupling the 2D semiconductor to a self-assembled plasmonic crystal inducing coherent hot electron doping. The established means of bandgap control in semiconductors are based on chemical, electrical or optical doping. Here, the authors report wide bandgap modulations in monolayer WS2 at room temperature by coupling the 2D semiconductor to a self-assembled plasmonic crystal inducing coherent hot electron doping. Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or optically with charge carriers. Here, we demonstrate a widely tunable bandgap (renormalisation up to 550 meV at room-temperature) in two-dimensional (2D) semiconductors by coherently doping the lattice with plasmonic hot electrons. In particular, we integrate tungsten-disulfide (WS2) monolayers into a self-assembled plasmonic crystal, which enables coherent coupling between semiconductor excitons and plasmon resonances. Accompanying this process, the plasmon-induced hot electrons can repeatedly fill the WS2 conduction band, leading to population inversion and a significant reconstruction in band structures and exciton relaxations. Our findings provide an effective measure to engineer optical responses of 2D semiconductors, allowing flexibilities in design and optimisation of photonic and optoelectronic devices.The established means of bandgap control in semiconductors are based on chemical, electrical or optical doping. Here, the authors report wide bandgap modulations in monolayer WS2 at room temperature by coupling the 2D semiconductor to a self-assembled plasmonic crystal inducing coherent hot electron doping. |
| ArticleNumber | 4332 |
| Author | Liu, Fengjiang Hodgkiss, Justin M. Qiu, Min Blaikie, Richard J. Ding, Boyang Chen, Yu-Hui Zhang, Yanfeng Chen, Kai Zhang, Zhepeng Tamming, Ronnie R. |
| Author_xml | – sequence: 1 givenname: Yu-Hui surname: Chen fullname: Chen, Yu-Hui organization: Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements of Ministry of Education, Beijing Key Laboratory of Nanophotonics & Ultrafine Optoelectronic Systems, School of Physics, Beijing Institute of Technology – sequence: 2 givenname: Ronnie R. surname: Tamming fullname: Tamming, Ronnie R. organization: Dodd-Walls Centre for Photonic and Quantum Technologies, MacDiarmid Institute for Advanced Materials and Nanotechnology, School of Chemical and Physical Sciences, Victoria University of Wellington – sequence: 3 givenname: Kai surname: Chen fullname: Chen, Kai organization: Dodd-Walls Centre for Photonic and Quantum Technologies, MacDiarmid Institute for Advanced Materials and Nanotechnology, School of Chemical and Physical Sciences, Victoria University of Wellington – sequence: 4 givenname: Zhepeng surname: Zhang fullname: Zhang, Zhepeng organization: Department of Materials Science and Engineering, College of Engineering, Center for Nanochemistry (CNC), College of Chemistry and Molecular Engineering, Academy for Advanced Interdisciplinary Studies, Peking University – sequence: 5 givenname: Fengjiang orcidid: 0000-0002-0161-2290 surname: Liu fullname: Liu, Fengjiang organization: Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province, School of Engineering, Westlake University, Institute of Advanced Technology, Westlake Institute for Advanced Study – sequence: 6 givenname: Yanfeng orcidid: 0000-0003-1319-3270 surname: Zhang fullname: Zhang, Yanfeng organization: Department of Materials Science and Engineering, College of Engineering, Center for Nanochemistry (CNC), College of Chemistry and Molecular Engineering, Academy for Advanced Interdisciplinary Studies, Peking University – sequence: 7 givenname: Justin M. surname: Hodgkiss fullname: Hodgkiss, Justin M. organization: Dodd-Walls Centre for Photonic and Quantum Technologies, MacDiarmid Institute for Advanced Materials and Nanotechnology, School of Chemical and Physical Sciences, Victoria University of Wellington – sequence: 8 givenname: Richard J. orcidid: 0000-0002-6991-835X surname: Blaikie fullname: Blaikie, Richard J. organization: Dodd-Walls Centre for Photonic and Quantum Technologies, MacDiarmid Institute for Advanced Materials and Nanotechnology, Department of Physics, University of Otago – sequence: 9 givenname: Boyang orcidid: 0000-0002-6299-5010 surname: Ding fullname: Ding, Boyang email: boyang.ding@otago.ac.nz organization: Dodd-Walls Centre for Photonic and Quantum Technologies, MacDiarmid Institute for Advanced Materials and Nanotechnology, Department of Physics, University of Otago – sequence: 10 givenname: Min orcidid: 0000-0002-4613-5125 surname: Qiu fullname: Qiu, Min email: qiu_lab@westlake.edu.cn organization: Key Laboratory of 3D Micro/Nano Fabrication and Characterization of Zhejiang Province, School of Engineering, Westlake University, Institute of Advanced Technology, Westlake Institute for Advanced Study |
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| Snippet | Bandgap control is of central importance for semiconductor technologies. The traditional means of control is to dope the lattice chemically, electrically or... The established means of bandgap control in semiconductors are based on chemical, electrical or optical doping. Here, the authors report wide bandgap... |
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| SubjectTerms | 639/301/357/1018 639/624/400/1021 639/624/400/2797 Coherence Conduction bands Coupling Current carriers Design optimization Doping Energy gap Excitons Hot electrons Humanities and Social Sciences Monolayers multidisciplinary Optoelectronic devices Plasmonics Population inversion Room temperature Science Science (multidisciplinary) Self-assembly Semiconductors Tungsten Tungsten disulfide |
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| Title | Bandgap control in two-dimensional semiconductors via coherent doping of plasmonic hot electrons |
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