Polyhydride CeH9 with an atomic-like hydrogen clathrate structure
Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors. However, it remains a challenge to get access to these states by synthesizing novel polyhydrides with unusually high hydrogen-to-metal ratio...
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Published in | Nature communications Vol. 10; no. 1; pp. 1 - 7 |
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Main Authors | , , , , , , , , , , |
Format | Journal Article |
Language | English |
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Nature Publishing Group UK
01.08.2019
Nature Publishing Group Nature Portfolio |
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Abstract | Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors. However, it remains a challenge to get access to these states by synthesizing novel polyhydrides with unusually high hydrogen-to-metal ratios. Here we synthesize a series of cerium (Ce) polyhydrides by a direct reaction of Ce and H
2
at high pressures. We discover that cerium polyhydride CeH
9
, formed above 100 GPa, presents a three-dimensional hydrogen network composed of clathrate H
29
cages. The electron localization function together with band structure calculations elucidate the weak electron localization between H-H atoms and confirm its metallic character. By means of Ce atom doping, metallic hydrogen structure can be realized via the existence of CeH
9
. Particularly, Ce atoms play a positive role to stabilize the sublattice of hydrogen cages similar to the recently discovered near-room-temperature lanthanum hydride superconductors.
Obtainment of hydrogen-rich metal hydrides that are high-temperature superconductors has been demonstrated under very high pressure, but is still largely unexplored. Here the authors synthesize CeH
9
, with a structure related to solid metallic hydrogen, at relatively low pressure and without need for heating. |
---|---|
AbstractList | Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors. However, it remains a challenge to get access to these states by synthesizing novel polyhydrides with unusually high hydrogen-to-metal ratios. Here we synthesize a series of cerium (Ce) polyhydrides by a direct reaction of Ce and H2 at high pressures. We discover that cerium polyhydride CeH9, formed above 100 GPa, presents a three-dimensional hydrogen network composed of clathrate H29 cages. The electron localization function together with band structure calculations elucidate the weak electron localization between H-H atoms and confirm its metallic character. By means of Ce atom doping, metallic hydrogen structure can be realized via the existence of CeH9. Particularly, Ce atoms play a positive role to stabilize the sublattice of hydrogen cages similar to the recently discovered near-room-temperature lanthanum hydride superconductors. Abstract Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors. However, it remains a challenge to get access to these states by synthesizing novel polyhydrides with unusually high hydrogen-to-metal ratios. Here we synthesize a series of cerium (Ce) polyhydrides by a direct reaction of Ce and H 2 at high pressures. We discover that cerium polyhydride CeH 9 , formed above 100 GPa, presents a three-dimensional hydrogen network composed of clathrate H 29 cages. The electron localization function together with band structure calculations elucidate the weak electron localization between H-H atoms and confirm its metallic character. By means of Ce atom doping, metallic hydrogen structure can be realized via the existence of CeH 9 . Particularly, Ce atoms play a positive role to stabilize the sublattice of hydrogen cages similar to the recently discovered near-room-temperature lanthanum hydride superconductors. Obtainment of hydrogen-rich metal hydrides that are high-temperature superconductors has been demonstrated under very high pressure, but is still largely unexplored. Here the authors synthesize CeH9, with a structure related to solid metallic hydrogen, at relatively low pressure and without need for heating. Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors. However, it remains a challenge to get access to these states by synthesizing novel polyhydrides with unusually high hydrogen-to-metal ratios. Here we synthesize a series of cerium (Ce) polyhydrides by a direct reaction of Ce and H 2 at high pressures. We discover that cerium polyhydride CeH 9 , formed above 100 GPa, presents a three-dimensional hydrogen network composed of clathrate H 29 cages. The electron localization function together with band structure calculations elucidate the weak electron localization between H-H atoms and confirm its metallic character. By means of Ce atom doping, metallic hydrogen structure can be realized via the existence of CeH 9 . Particularly, Ce atoms play a positive role to stabilize the sublattice of hydrogen cages similar to the recently discovered near-room-temperature lanthanum hydride superconductors. Obtainment of hydrogen-rich metal hydrides that are high-temperature superconductors has been demonstrated under very high pressure, but is still largely unexplored. Here the authors synthesize CeH 9 , with a structure related to solid metallic hydrogen, at relatively low pressure and without need for heating. |
ArticleNumber | 3461 |
Author | Duan, Defang Pickard, Chris J. Zhuang, Quan Huang, Yanping Huang, Xiaoli Zhou, Di Zhou, Qiang Liu, Bingbing Cui, Tian Li, Xin Xie, Hui |
Author_xml | – sequence: 1 givenname: Xin orcidid: 0000-0002-9613-2221 surname: Li fullname: Li, Xin organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 2 givenname: Xiaoli surname: Huang fullname: Huang, Xiaoli email: huangxiaoli@jlu.edu.cn organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 3 givenname: Defang surname: Duan fullname: Duan, Defang organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Department of Materials Science & Metallurgy, University of Cambridge – sequence: 4 givenname: Chris J. orcidid: 0000-0002-9684-5432 surname: Pickard fullname: Pickard, Chris J. organization: Department of Materials Science & Metallurgy, University of Cambridge – sequence: 5 givenname: Di surname: Zhou fullname: Zhou, Di organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 6 givenname: Hui surname: Xie fullname: Xie, Hui organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 7 givenname: Quan surname: Zhuang fullname: Zhuang, Quan organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 8 givenname: Yanping surname: Huang fullname: Huang, Yanping organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 9 givenname: Qiang surname: Zhou fullname: Zhou, Qiang organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 10 givenname: Bingbing surname: Liu fullname: Liu, Bingbing organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University – sequence: 11 givenname: Tian surname: Cui fullname: Cui, Tian email: cuitian@jlu.edu.cn organization: State Key Laboratory of Superhard Materials, College of Physics, Jilin University |
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Snippet | Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature superconductors.... Abstract Compression of hydrogen-rich hydrides has been proposed as an alternative way to attain the atomic metallic hydrogen state or high-temperature... Obtainment of hydrogen-rich metal hydrides that are high-temperature superconductors has been demonstrated under very high pressure, but is still largely... |
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SubjectTerms | 119/118 639/638/263/915 639/638/440/94 Cages Cerium Clathrates Compression High temperature superconductors Humanities and Social Sciences Hydrides Hydrogen Hydrogen storage Lanthanum Localization Metallic hydrogen multidisciplinary Science Science (multidisciplinary) |
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Title | Polyhydride CeH9 with an atomic-like hydrogen clathrate structure |
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