Ultrafast charge transfer and vibronic coupling in a laser-excited hybrid inorganic/organic interface

• Published in: Advances in physics: X Vol. 5; no. 1; p. 1749883
• Main Authors: Jacobs, Matheus, Krumland, Jannis, Valencia, Ana M., Wang, Haiyuan, Rossi, Mariana, Cocchi, Caterina
• Format: Journal Article
• Language: English
• Published: Abingdon Taylor & Francis 01.01.2020; Taylor & Francis Ltd; Taylor & Francis Group
• Subjects: Charge materials; Charge transfer; Coordination compounds; Coupling (molecular); Density functional theory; Electronic structure; hybrid materials; Interfaces; Lasers; Molecular dynamics; Organic chemistry; Organic semiconductors; Time dependence; time-dependent DFT; Ultrafast charge transfer; vibronic coupling; Windows (intervals)

Hybrid interfaces formed by inorganic semiconductors and organic molecules are intriguing materials for opto-electronics. Interfacial charge transfer is primarily responsible for their peculiar electronic structure and optical response. Hence, it is essential to gain insight into this fundamental pr...