0D/2D Heterojunctions of Vanadate Quantum Dots/Graphitic Carbon Nitride Nanosheets for Enhanced Visible‐Light‐Driven Photocatalysis
0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO3, BiVO4, InVO4 and CuV2O6) QDs/graphitic carbon nitride (g‐C3N4)...
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| Published in | Angewandte Chemie International Edition Vol. 56; no. 29; pp. 8407 - 8411 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
10.07.2017
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO3, BiVO4, InVO4 and CuV2O6) QDs/graphitic carbon nitride (g‐C3N4) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up‐conversion absorption, and nitrogen coordinating sites of g‐C3N4 NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible‐light‐driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto‐electronic applications, not limited in photocatalysis.
Vanadate quantum dots including AgVO3, BiVO4, InVO4, and CuV2O6 were strongly coupled with graphitic carbon nitride nanosheets using an in situ growth strategy. These quantum dots displayed a much better visible‐light‐driven photoelectrochemical activity and photocatalytic degradation efficiency than single vanadate quantum dots, carbon nitride nanosheets or previously reported highly active photocatalysts. |
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| AbstractList | 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO3, BiVO4, InVO4 and CuV2O6) QDs/graphitic carbon nitride (g-C3N4) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up-conversion absorption, and nitrogen coordinating sites of g-C3N4 NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible-light-driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto-electronic applications, not limited in photocatalysis. 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO , BiVO , InVO and CuV O ) QDs/graphitic carbon nitride (g-C N ) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up-conversion absorption, and nitrogen coordinating sites of g-C N NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible-light-driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto-electronic applications, not limited in photocatalysis. 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO3, BiVO4, InVO4 and CuV2O6) QDs/graphitic carbon nitride (g‐C3N4) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up‐conversion absorption, and nitrogen coordinating sites of g‐C3N4 NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible‐light‐driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto‐electronic applications, not limited in photocatalysis. Vanadate quantum dots including AgVO3, BiVO4, InVO4, and CuV2O6 were strongly coupled with graphitic carbon nitride nanosheets using an in situ growth strategy. These quantum dots displayed a much better visible‐light‐driven photoelectrochemical activity and photocatalytic degradation efficiency than single vanadate quantum dots, carbon nitride nanosheets or previously reported highly active photocatalysts. 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO3 , BiVO4 , InVO4 and CuV2 O6 ) QDs/graphitic carbon nitride (g-C3 N4 ) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up-conversion absorption, and nitrogen coordinating sites of g-C3 N4 NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible-light-driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto-electronic applications, not limited in photocatalysis. 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their high charge mobility. Herein, unprecedent heterojunctions of vanadate (AgVO 3 , BiVO 4 , InVO 4 and CuV 2 O 6 ) QDs/graphitic carbon nitride (g‐C 3 N 4 ) NSs exhibiting multiple unique advances beyond traditional 0D/2D composites have been developed. The photoactive contribution, up‐conversion absorption, and nitrogen coordinating sites of g‐C 3 N 4 NSs, highly dispersed vanadate nanocrystals, as well as the strong coupling and band alignment between them lead to superior visible‐light‐driven photoelectrochemical (PEC) and photocatalytic performance, competing with the best reported photocatalysts. This work is expected to provide a new concept to construct multifunctional 0D/2D nanocomposites for a large variety of opto‐electronic applications, not limited in photocatalysis. |
| Author | Liu, Le‐Quan Ye, Meng‐Yang Zhao, Zhi‐Hao Hu, Zhuo‐Feng Ji, Hui‐Ming Ma, Tian‐Yi Shen, Zhu‐Rui |
| Author_xml | – sequence: 1 givenname: Meng‐Yang surname: Ye fullname: Ye, Meng‐Yang organization: Tianjin University – sequence: 2 givenname: Zhi‐Hao surname: Zhao fullname: Zhao, Zhi‐Hao organization: Tianjin University – sequence: 3 givenname: Zhuo‐Feng surname: Hu fullname: Hu, Zhuo‐Feng organization: The Chinese University of Hong Kong – sequence: 4 givenname: Le‐Quan surname: Liu fullname: Liu, Le‐Quan organization: Tianjin University – sequence: 5 givenname: Hui‐Ming surname: Ji fullname: Ji, Hui‐Ming organization: Tianjin University – sequence: 6 givenname: Zhu‐Rui surname: Shen fullname: Shen, Zhu‐Rui email: shenzhurui@tju.edu.cn organization: Tianjin University – sequence: 7 givenname: Tian‐Yi orcidid: 0000-0002-1042-8700 surname: Ma fullname: Ma, Tian‐Yi email: tian-yi.ma@adelaide.edu.au organization: The University of Adelaide |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28052568$$D View this record in MEDLINE/PubMed |
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| Snippet | 0D/2D heterojunctions, especially quantum dots (QDs)/nanosheets (NSs) have attracted significant attention for use of photoexcited electrons/holes due to their... |
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| SubjectTerms | Carbon nitride Crystals graphitic carbon nitride Heterojunctions Nanocomposites Nanocrystals Nanosheets Optoelectronics Photocatalysis Quantum dots Two dimensional composites Upconversion Vanadate vanadates |
| Title | 0D/2D Heterojunctions of Vanadate Quantum Dots/Graphitic Carbon Nitride Nanosheets for Enhanced Visible‐Light‐Driven Photocatalysis |
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