Polyester Stereocomplexes Beyond PLA: Could Synthetic Opportunities Revolutionize Established Material Blending?

This review summarizes the current literature regarding stereocomplexation of different polyesters based on α‐ as well as β‐hydroxy acids beyond the well‐known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic poly...

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Published inMacromolecular rapid communications. Vol. 41; no. 1; pp. e1900560 - n/a
Main Authors Bandelli, Damiano, Alex, Julien, Weber, Christine, Schubert, Ulrich S.
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.01.2020
Subjects
Biocompatible Materials - chemistry
Chemical synthesis
Cycloaddition Reaction
Hydroxy acids
Hydroxy Acids - chemistry
Literature reviews
Macromolecules
Material properties
Materials science
Mechanical properties
Organic chemistry
poly(α‐hydroxyacid)s
poly(β‐hydroxyacid)s
Polyester resins
Polyesters
Polyesters - chemical synthesis
Polyesters - chemistry
Polylactic acid
Polymerization
ring‐opening polymerization
Stereocomplexes
Stereoisomerism
Stereoselectivity
poly(β-hydroxyacid)s
stereocomplexes
polyesters
ring-opening polymerization
poly(α-hydroxyacid)s
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Abstract This review summarizes the current literature regarding stereocomplexation of different polyesters based on α‐ as well as β‐hydroxy acids beyond the well‐known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic polyesters are summarized. The basic technologies for the preparation and characterization of the respective stereocomplexes (SCs) are described, and published material properties are related to the structure of the respective polyesters. The variety of available SC materials is very limited despite the multiple options provided by state‐of‐the‐art stereoselective monomer synthesis and polymerization methods. A combination of knowledge from the three scientific areas (i.e., organic chemistry, synthetic macromolecular chemistry, and materials science) thus has enormous potential to create novel materials with additional features enabled by the introduction of functional moieties to such materials besides the adjustment of thermal as well as mechanical properties. This review provides an overview of polyester stereocomplexes reported to date, complemented by the methods for preparation as well as for analysis. To encourage the scientific community to further exploit the range of functional monomers and polymers available for this purpose, synthetic methods are discussed, pointing out promising opportunities that have not yet been considered for stereocomplexation.
AbstractList This review summarizes the current literature regarding stereocomplexation of different polyesters based on α‐ as well as β‐hydroxy acids beyond the well‐known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic polyesters are summarized. The basic technologies for the preparation and characterization of the respective stereocomplexes (SCs) are described, and published material properties are related to the structure of the respective polyesters. The variety of available SC materials is very limited despite the multiple options provided by state‐of‐the‐art stereoselective monomer synthesis and polymerization methods. A combination of knowledge from the three scientific areas (i.e., organic chemistry, synthetic macromolecular chemistry, and materials science) thus has enormous potential to create novel materials with additional features enabled by the introduction of functional moieties to such materials besides the adjustment of thermal as well as mechanical properties.
This review summarizes the current literature regarding stereocomplexation of different polyesters based on α- as well as β-hydroxy acids beyond the well-known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic polyesters are summarized. The basic technologies for the preparation and characterization of the respective stereocomplexes (SCs) are described, and published material properties are related to the structure of the respective polyesters. The variety of available SC materials is very limited despite the multiple options provided by state-of-the-art stereoselective monomer synthesis and polymerization methods. A combination of knowledge from the three scientific areas (i.e., organic chemistry, synthetic macromolecular chemistry, and materials science) thus has enormous potential to create novel materials with additional features enabled by the introduction of functional moieties to such materials besides the adjustment of thermal as well as mechanical properties.This review summarizes the current literature regarding stereocomplexation of different polyesters based on α- as well as β-hydroxy acids beyond the well-known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic polyesters are summarized. The basic technologies for the preparation and characterization of the respective stereocomplexes (SCs) are described, and published material properties are related to the structure of the respective polyesters. The variety of available SC materials is very limited despite the multiple options provided by state-of-the-art stereoselective monomer synthesis and polymerization methods. A combination of knowledge from the three scientific areas (i.e., organic chemistry, synthetic macromolecular chemistry, and materials science) thus has enormous potential to create novel materials with additional features enabled by the introduction of functional moieties to such materials besides the adjustment of thermal as well as mechanical properties.
This review summarizes the current literature regarding stereocomplexation of different polyesters based on α‐ as well as β‐hydroxy acids beyond the well‐known poly(lactic acid). Representing the initial step toward stereocomplexation, synthetic approaches needed to obtain and analyze isotactic polyesters are summarized. The basic technologies for the preparation and characterization of the respective stereocomplexes (SCs) are described, and published material properties are related to the structure of the respective polyesters. The variety of available SC materials is very limited despite the multiple options provided by state‐of‐the‐art stereoselective monomer synthesis and polymerization methods. A combination of knowledge from the three scientific areas (i.e., organic chemistry, synthetic macromolecular chemistry, and materials science) thus has enormous potential to create novel materials with additional features enabled by the introduction of functional moieties to such materials besides the adjustment of thermal as well as mechanical properties. This review provides an overview of polyester stereocomplexes reported to date, complemented by the methods for preparation as well as for analysis. To encourage the scientific community to further exploit the range of functional monomers and polymers available for this purpose, synthetic methods are discussed, pointing out promising opportunities that have not yet been considered for stereocomplexation.
Author Alex, Julien
Weber, Christine
Schubert, Ulrich S.
Bandelli, Damiano
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  fullname: Alex, Julien
  organization: Friedrich Schiller University Jena
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  surname: Weber
  fullname: Weber, Christine
  organization: Friedrich Schiller University Jena
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  givenname: Ulrich S.
  surname: Schubert
  fullname: Schubert, Ulrich S.
  email: ulrich.schubert@uni-jena.de
  organization: Friedrich Schiller University Jena
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31793732$$D View this record in MEDLINE/PubMed
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Issue 1
Keywords poly(β-hydroxyacid)s
stereocomplexes
polyesters
ring-opening polymerization
poly(α-hydroxyacid)s
Language English
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2019 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
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PublicationTitle Macromolecular rapid communications.
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Snippet This review summarizes the current literature regarding stereocomplexation of different polyesters based on α‐ as well as β‐hydroxy acids beyond the well‐known...
This review summarizes the current literature regarding stereocomplexation of different polyesters based on α- as well as β-hydroxy acids beyond the well-known...
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StartPage e1900560
SubjectTerms Biocompatible Materials - chemistry
Chemical synthesis
Cycloaddition Reaction
Hydroxy acids
Hydroxy Acids - chemistry
Literature reviews
Macromolecules
Material properties
Materials science
Mechanical properties
Organic chemistry
poly(α‐hydroxyacid)s
poly(β‐hydroxyacid)s
Polyester resins
Polyesters
Polyesters - chemical synthesis
Polyesters - chemistry
Polylactic acid
Polymerization
ring‐opening polymerization
Stereocomplexes
Stereoisomerism
Stereoselectivity
Title Polyester Stereocomplexes Beyond PLA: Could Synthetic Opportunities Revolutionize Established Material Blending?
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fmarc.201900560
https://www.ncbi.nlm.nih.gov/pubmed/31793732
https://www.proquest.com/docview/2333939028
https://www.proquest.com/docview/2320875076
Volume 41
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