Silicon-based materials as high capacity anodes for next generation lithium ion batteries

Silicon (Si)-based materials have the highest capacity among the investigated anode materials and have been recognized as one of the most promising materials for lithium-ion batteries. However, it is still a significant challenge to obtain good performance for practical applications due to the huge...

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Published in	Journal of power sources Vol. 267; pp. 469 - 490
Main Authors	Liang, Bo, Liu, Yanping, Xu, Yunhua
Format	Journal Article
Language	English
Published	Amsterdam Elsevier B.V 01.12.2014 Elsevier
Subjects	Anode Anodes Applied sciences Composite Design engineering Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Exact sciences and technology Lithium batteries Lithium-ion batteries Materials Nano-structure Nanostructure Recognition Silicon Strategy Synthesis Lithium-ion batteries Silicon Anode Composite Nano-structure Lithium ion batteries Capacitance Secondary cell Nanostructure Electrode material Composite material
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Abstract	Silicon (Si)-based materials have the highest capacity among the investigated anode materials and have been recognized as one of the most promising materials for lithium-ion batteries. However, it is still a significant challenge to obtain good performance for practical applications due to the huge volume change during the electrochemical process. To date, the most successful strategy is to introduce other components into Si to form composite or alloy materials. In this review, the recent progress in Si-based materials utilized in lithium-ion batteries is reviewed in terms of composite systems, nano-structure designs, material synthesis methods, and electrochemical performances. The merits and disadvantages of different Si-based materials, the understanding of the mechanisms behind the performance enhancement as well as the challenges faced in Si anodes are also discussed. We are trying to present a full scope of the Si-based materials, and help understand and design future structures of Si anodes in lithium-ion batteries. •The paper reviewed the merits of silicon-based anodes in lithium ion batteries.•The mechanisms were discussed from in-situ TEM and first-principles simulation.•The challenges faced in silicon-based anodes were analyzed and forecast.
AbstractList	Silicon (Si)-based materials have the highest capacity among the investigated anode materials and have been recognized as one of the most promising materials for lithium-ion batteries. However, it is still a significant challenge to obtain good performance for practical applications due to the huge volume change during the electrochemical process. To date, the most successful strategy is to introduce other components into Si to form composite or alloy materials. In this review, the recent progress in Si-based materials utilized in lithium-ion batteries is reviewed in terms of composite systems, nano-structure designs, material synthesis methods, and electrochemical performances. The merits and disadvantages of different Si-based materials, the understanding of the mechanisms behind the performance enhancement as well as the challenges faced in Si anodes are also discussed. We are trying to present a full scope of the Si-based materials, and help understand and design future structures of Si anodes in lithium-ion batteries. Silicon (Si)-based materials have the highest capacity among the investigated anode materials and have been recognized as one of the most promising materials for lithium-ion batteries. However, it is still a significant challenge to obtain good performance for practical applications due to the huge volume change during the electrochemical process. To date, the most successful strategy is to introduce other components into Si to form composite or alloy materials. In this review, the recent progress in Si-based materials utilized in lithium-ion batteries is reviewed in terms of composite systems, nano-structure designs, material synthesis methods, and electrochemical performances. The merits and disadvantages of different Si-based materials, the understanding of the mechanisms behind the performance enhancement as well as the challenges faced in Si anodes are also discussed. We are trying to present a full scope of the Si-based materials, and help understand and design future structures of Si anodes in lithium-ion batteries. •The paper reviewed the merits of silicon-based anodes in lithium ion batteries.•The mechanisms were discussed from in-situ TEM and first-principles simulation.•The challenges faced in silicon-based anodes were analyzed and forecast.
Author	Liang, Bo Xu, Yunhua Liu, Yanping
Author_xml	– sequence: 1 givenname: Bo surname: Liang fullname: Liang, Bo email: liangbo26@126.com, lbscut@126.com organization: Department of Material Forming and Control Engineering, School of Automobile and Mechanic Engineering, Changsha University of Science & Technology, Changsha 410076, PR China – sequence: 2 givenname: Yanping surname: Liu fullname: Liu, Yanping organization: Department of Material Forming and Control Engineering, School of Automobile and Mechanic Engineering, Changsha University of Science & Technology, Changsha 410076, PR China – sequence: 3 givenname: Yunhua surname: Xu fullname: Xu, Yunhua organization: Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, MD 20742, USA
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Publisher	Elsevier B.V Elsevier
Publisher_xml	– name: Elsevier B.V – name: Elsevier
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Snippet	Silicon (Si)-based materials have the highest capacity among the investigated anode materials and have been recognized as one of the most promising materials...
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SubjectTerms	Anode Anodes Applied sciences Composite Design engineering Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Exact sciences and technology Lithium batteries Lithium-ion batteries Materials Nano-structure Nanostructure Recognition Silicon Strategy Synthesis
Title	Silicon-based materials as high capacity anodes for next generation lithium ion batteries
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