Enhanced PCBs sorption on biochars as affected by environmental factors: Humic acid and metal cations
Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil wa...
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| Published in | Environmental pollution (1987) Vol. 172; pp. 86 - 93 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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Kidlington
Elsevier Ltd
01.01.2013
Elsevier |
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| Abstract | Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment.
► Application of the biochars for PCBs sorption was a new and effective way. ► The biochars had higher adsorption affinity for PCBs in the soil extracted solution. ► Pine needle chars adsorbed less nonplanar PCBs than planar ones. ► Coexisting humic acid or metal cations increased PCBs sorption on the biochars.
The biochars had higher adsorption affinity for PCBs in the extracted soil solution because coexisting humic acid and metal cations increased their sorption. |
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| AbstractList | Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment.
► Application of the biochars for PCBs sorption was a new and effective way. ► The biochars had higher adsorption affinity for PCBs in the soil extracted solution. ► Pine needle chars adsorbed less nonplanar PCBs than planar ones. ► Coexisting humic acid or metal cations increased PCBs sorption on the biochars.
The biochars had higher adsorption affinity for PCBs in the extracted soil solution because coexisting humic acid and metal cations increased their sorption. Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment.Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment. Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment. Biochar plays an important role in the behaviors of organic pollutants in the soil environment. The role of humic acid (HA) and metal cations on the adsorption affinity of polychlorinated biphenyls (PCBs) to the biochars in an aqueous medium and an extracted solution from a PCBs-contaminated soil was studied using batch experiments. Biochars were produced with pine needles and wheat straw at 350 °C and 550 °C under anaerobic condition. The results showed that the biochars had high adsorption affinity for PCBs. Pine needle chars adsorbed less nonplanar PCBs than planar ones due to dispersive interactions and separation. Coexistence of HA and metal cations increased PCBs sorption on the biochars accounted for HA adsorption and cation complexation. The results will aid in a better understanding of biochar sorption mechanism of contaminants in the environment. |
| Author | Cang, Long Wang, Yu Herath, H.M.S.K. Fang, Guodong Wang, Yujun Wang, Lei Xie, Zubin Zhou, Dongmei |
| Author_xml | – sequence: 1 givenname: Yu surname: Wang fullname: Wang, Yu organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 2 givenname: Lei surname: Wang fullname: Wang, Lei organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 3 givenname: Guodong surname: Fang fullname: Fang, Guodong organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 4 givenname: H.M.S.K. surname: Herath fullname: Herath, H.M.S.K. organization: New Zealand Biochar Research Centre, Institute of Natural Resources, Massey University, Palmerston North 4442, New Zealand – sequence: 5 givenname: Yujun surname: Wang fullname: Wang, Yujun organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 6 givenname: Long surname: Cang fullname: Cang, Long organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 7 givenname: Zubin surname: Xie fullname: Xie, Zubin organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China – sequence: 8 givenname: Dongmei surname: Zhou fullname: Zhou, Dongmei email: dmzhou@issas.ac.cn organization: Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences, 71st East Beijing Road, Nanjing 210008, China |
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| Keywords | Polychlorinated biphenyls Metal cations Adsorption Biochar Humic acid Organic waste Combustion residue Adsorption capacity Environmental factor Soil pollution Organic halogen compounds Persistent organic pollutant Decontamination Upgrading Chlorocarbon Aromatic compound Agricultural waste Organic compounds Polychlorobiphenyls Cation effect Organic chlorine compounds Vegetal waste Waste management Halogenated hydrocarbon Waste reuse Charcoal |
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| SubjectTerms | Adsorption analysis Applied sciences Biochar cations Cations - chemistry Charcoal Charcoal - chemistry chemistry conifer needles Decontamination. Miscellaneous Earth sciences Earth, ocean, space edaphic factors Engineering and environment geology. Geothermics Environmental Restoration and Remediation Environmental Restoration and Remediation - methods Exact sciences and technology Humic acid humic acids Humic Substances Metal cations Metals Metals - chemistry methods Pollution Pollution, environment geology Polychlorinated biphenyls Polychlorinated Biphenyls - analysis Polychlorinated Biphenyls - chemistry soil Soil - chemistry Soil and sediments pollution Soil Pollutants Soil Pollutants - analysis Soil Pollutants - chemistry soil pollution wheat straw |
| Title | Enhanced PCBs sorption on biochars as affected by environmental factors: Humic acid and metal cations |
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