Distribution and sources of organochlorine pesticides in agricultural soils from central China
There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and...
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| Published in | Ecotoxicology and environmental safety Vol. 93; pp. 163 - 170 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
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San Diego, CA
Elsevier Inc
01.07.2013
Elsevier |
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| Abstract | There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg−1 and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg−1 in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned.
•OCPs in agricultural soils from central China were determined to evaluate the status of contamination.•HCH pollution in most samples of agricultural soil were considered as no contamination by GB15618-1995.•The level of DDTs was classified as low pollution by GB15618-1995.•OCPs residues except heptachlor originated mainly from historical application. |
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| AbstractList | There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg−1 and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg−1 in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned.
•OCPs in agricultural soils from central China were determined to evaluate the status of contamination.•HCH pollution in most samples of agricultural soil were considered as no contamination by GB15618-1995.•The level of DDTs was classified as low pollution by GB15618-1995.•OCPs residues except heptachlor originated mainly from historical application. There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg⁻¹ and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg⁻¹ in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned. There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg−1 and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg−1 in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned. There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg(-1) and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg(-1) in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned.There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg(-1) and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg(-1) in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned. There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil samples were collected from agricultural soils in Wuhan and analyzed to determine twenty-one OCPs. According to the measured concentrations and detection frequencies, dichlorodiphenyltrichloroethanes (DDTs), hexachlorocyclohexanes (HCHs), heptachlor (HEPT), hexachlorobenzene (HCB) and aldrin were the predominant compounds in soil. DDTs accounted for 77.10% of total OCPs, followed by HCHs (7.83%), aldrin (4.21%), HEPTs (2.82%) and HCB (1.53%). The total DDT concentrations ranged from nd to 1198.0ngg(-1) and the main contaminated areas were distributed in Hannan and Xinzhou districts of Wuhan. The total HCH concentrations ranged from nd to 100.58ngg(-1) in soil and relatively higher levels were observed in soil samples from Huangpi and Hannan districts. Source analysis showed that OCPs residues except heptachlor originated mainly from historical application, besides slight recent introduction at some sites. Based on the China National Soil Quality Standard, DDT pollution in most samples of Wuhan agricultural soils could be considered as no and low contamination, while the level of HCHs was classified as no pollution. Our study indicated that there existed potential exposure risk of OCPs in Wuhan agricultural soils although the use of OCPs has been banned. |
| Author | Meng, Beidi Wang, Jingjing Cheng, Junqi Chen, Jiachun Zheng, Dan Zhou, Qun Lin, Guoping Yu, Yanhong |
| Author_xml | – sequence: 1 givenname: Qun surname: Zhou fullname: Zhou, Qun email: qunzhou.hust@gmail.com organization: Hubei Key Laboratory of Natural Medicinal Chemistry and Resource Evaluation, Tongji School of Pharmacy, Huazhong University of Science and Technology, Wuhan 430030, China – sequence: 2 givenname: Jingjing surname: Wang fullname: Wang, Jingjing organization: Hubei Key Laboratory of Natural Medicinal Chemistry and Resource Evaluation, Tongji School of Pharmacy, Huazhong University of Science and Technology, Wuhan 430030, China – sequence: 3 givenname: Beidi surname: Meng fullname: Meng, Beidi organization: Hubei Key Laboratory of Natural Medicinal Chemistry and Resource Evaluation, Tongji School of Pharmacy, Huazhong University of Science and Technology, Wuhan 430030, China – sequence: 4 givenname: Junqi surname: Cheng fullname: Cheng, Junqi organization: Burley Tobacco Experimental Station of CNTC/Hubei Tobacco Research Institute, Wuhan 430030, China – sequence: 5 givenname: Guoping surname: Lin fullname: Lin, Guoping email: lgpfy@126.com organization: Burley Tobacco Experimental Station of CNTC/Hubei Tobacco Research Institute, Wuhan 430030, China – sequence: 6 givenname: Jiachun surname: Chen fullname: Chen, Jiachun organization: Hubei Key Laboratory of Natural Medicinal Chemistry and Resource Evaluation, Tongji School of Pharmacy, Huazhong University of Science and Technology, Wuhan 430030, China – sequence: 7 givenname: Dan surname: Zheng fullname: Zheng, Dan organization: MOE Key Laboratory of Environment and Health, School of Public Health, Huazhong University of Science and Technology, Wuhan 430030, China – sequence: 8 givenname: Yanhong surname: Yu fullname: Yu, Yanhong organization: Hubei Key Laboratory of Natural Medicinal Chemistry and Resource Evaluation, Tongji School of Pharmacy, Huazhong University of Science and Technology, Wuhan 430030, China |
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| Keywords | Agricultural soil Organochlorine pesticide Pollution assessment China Ecotoxicology Toxicity Pesticides Soils Pollution Organochlorine compounds Chlorine Organic compounds Environment Agriculture Organic compounds |
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| Snippet | There is little information on the organochlorine pesticides (OCPs) residues in agricultural soils of Wuhan, the largest city in central China. Surface soil... |
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| SubjectTerms | Agricultural soil agricultural soils Agriculture - statistics & numerical data Agronomy. Soil science and plant productions aldrin Animal, plant and microbial ecology Applied ecology Biological and medical sciences China DDT (pesticide) Ecotoxicology, biological effects of pollution Environmental Monitoring Environmental Pollution - statistics & numerical data Fundamental and applied biological sciences. Psychology General agroecology General agroecology. Agricultural and farming systems. Agricultural development. Rural area planning. Landscaping General agronomy. Plant production General aspects Generalities. Agricultural and farming systems. Agricultural development HCH (pesticide) heptachlor hexachlorobenzene Hexachlorobenzene - analysis Hydrocarbons, Chlorinated - analysis Lindane - analysis Organochlorine pesticide Pesticides - analysis pollution Pollution assessment risk Soil - chemistry Soil Pollutants - analysis soil quality soil sampling |
| Title | Distribution and sources of organochlorine pesticides in agricultural soils from central China |
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