Hybrid Wetting Surface with Plasmonic Alloy Nanocomposites for Sensitive SERS Detection
In this paper, a hybrid wetting surface (HWS) with Au/Ag alloy nanocomposites was proposed for rapid, cost-effective, stable and sensitive SERS application. This surface was fabricated in a large area by facile electrospinning, plasma etching and photomask-assisted sputtering processes. The high-den...
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| Published in | Molecules (Basel, Switzerland) Vol. 28; no. 5; p. 2190 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
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| Abstract | In this paper, a hybrid wetting surface (HWS) with Au/Ag alloy nanocomposites was proposed for rapid, cost-effective, stable and sensitive SERS application. This surface was fabricated in a large area by facile electrospinning, plasma etching and photomask-assisted sputtering processes. The high-density ‘hot spots’ and rough surface from plasmonic alloy nanocomposites promoted the significant enhancement of the electromagnetic field. Meanwhile, the condensation effects induced by HWS further improved the density of target analytes at the SERS active area. Thus, the SERS signals increased ~4 orders of magnitude compared to the normal SERS substrate. In addition, the reproducibility, uniformity, as well as thermal performance of HWS were also examined by comparative experiments, indicating their high reliability, portability and practicability for on-site tests. The efficient results suggested that this smart surface had great potential to evolve as a platform for advanced sensor-based applications. |
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| AbstractList | In this paper, a hybrid wetting surface (HWS) with Au/Ag alloy nanocomposites was proposed for rapid, cost-effective, stable and sensitive SERS application. This surface was fabricated in a large area by facile electrospinning, plasma etching and photomask-assisted sputtering processes. The high-density 'hot spots' and rough surface from plasmonic alloy nanocomposites promoted the significant enhancement of the electromagnetic field. Meanwhile, the condensation effects induced by HWS further improved the density of target analytes at the SERS active area. Thus, the SERS signals increased ~4 orders of magnitude compared to the normal SERS substrate. In addition, the reproducibility, uniformity, as well as thermal performance of HWS were also examined by comparative experiments, indicating their high reliability, portability and practicability for on-site tests. The efficient results suggested that this smart surface had great potential to evolve as a platform for advanced sensor-based applications. In this paper, a hybrid wetting surface (HWS) with Au/Ag alloy nanocomposites was proposed for rapid, cost-effective, stable and sensitive SERS application. This surface was fabricated in a large area by facile electrospinning, plasma etching and photomask-assisted sputtering processes. The high-density 'hot spots' and rough surface from plasmonic alloy nanocomposites promoted the significant enhancement of the electromagnetic field. Meanwhile, the condensation effects induced by HWS further improved the density of target analytes at the SERS active area. Thus, the SERS signals increased ~4 orders of magnitude compared to the normal SERS substrate. In addition, the reproducibility, uniformity, as well as thermal performance of HWS were also examined by comparative experiments, indicating their high reliability, portability and practicability for on-site tests. The efficient results suggested that this smart surface had great potential to evolve as a platform for advanced sensor-based applications.In this paper, a hybrid wetting surface (HWS) with Au/Ag alloy nanocomposites was proposed for rapid, cost-effective, stable and sensitive SERS application. This surface was fabricated in a large area by facile electrospinning, plasma etching and photomask-assisted sputtering processes. The high-density 'hot spots' and rough surface from plasmonic alloy nanocomposites promoted the significant enhancement of the electromagnetic field. Meanwhile, the condensation effects induced by HWS further improved the density of target analytes at the SERS active area. Thus, the SERS signals increased ~4 orders of magnitude compared to the normal SERS substrate. In addition, the reproducibility, uniformity, as well as thermal performance of HWS were also examined by comparative experiments, indicating their high reliability, portability and practicability for on-site tests. The efficient results suggested that this smart surface had great potential to evolve as a platform for advanced sensor-based applications. |
| Audience | Academic |
| Author | Jiang, Xiaohan Zhang, Xiaoyang Wang, Shanjiang Zhang, Tong Su, Dan Zhou, Huanli |
| AuthorAffiliation | 1 School of Materials Science and Engineering, Nanjing Tech University, Nanjing 210009, China 2 Joint International Research Laboratory of Information Display and Visualization, School of Electronic Science and Engineering, Southeast University, Nanjing 210096, China |
| AuthorAffiliation_xml | – name: 2 Joint International Research Laboratory of Information Display and Visualization, School of Electronic Science and Engineering, Southeast University, Nanjing 210096, China – name: 1 School of Materials Science and Engineering, Nanjing Tech University, Nanjing 210009, China |
| Author_xml | – sequence: 1 givenname: Shanjiang surname: Wang fullname: Wang, Shanjiang – sequence: 2 givenname: Dan orcidid: 0000-0002-3332-7144 surname: Su fullname: Su, Dan – sequence: 3 givenname: Huanli surname: Zhou fullname: Zhou, Huanli – sequence: 4 givenname: Xiaohan surname: Jiang fullname: Jiang, Xiaohan – sequence: 5 givenname: Xiaoyang surname: Zhang fullname: Zhang, Xiaoyang – sequence: 6 givenname: Tong surname: Zhang fullname: Zhang, Tong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/36903436$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | Alloys Communication condensation effects Contact angle Design Electromagnetic fields Electromagnetism hot spots hybrid wetting surface Hydrophobic surfaces Morphology Nanocomposites Nanoparticles Plasma etching Reproducibility sensor-based applications Sensors SERS Silicon wafers Specialty metals industry Spectrum analysis |
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| Title | Hybrid Wetting Surface with Plasmonic Alloy Nanocomposites for Sensitive SERS Detection |
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