Alkynyl Coinage Metal Clusters and Complexes–Syntheses, Structures, and Strategies

In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end‐on) and η2 (side on) modes, includes non‐bridged systems, as well as bridging of up to four (or six) metal...

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Published inChemistry : a European journal Vol. 24; no. 30; pp. 7536 - 7559
Main Authors Gupta, Arvind Kumar, Orthaber, Andreas
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 28.05.2018
Subjects
alkynyl ligands
Chemistry
cluster compounds
coinage metals
Coordination compounds
Ligands
Metal clusters
Metal complexes
metallophilic interactions
X-ray crystallography
X-ray crystallography
coinage metals
cluster compounds
alkynyl ligands
metallophilic interactions
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Abstract In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end‐on) and η2 (side on) modes, includes non‐bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co‐ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero‐bi‐metallic coinage metal clusters of alkynyl ligands. Coin toss: Syntheses, structural traits and properties of alkynyl coinage metals clusters are discussed and compared. Concepts and synthetic strategies are highlighted.
AbstractList In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end‐on) and η2 (side on) modes, includes non‐bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co‐ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero‐bi‐metallic coinage metal clusters of alkynyl ligands.
In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end-on) and η2 (side on) modes, includes non-bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co-ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero-bi-metallic coinage metal clusters of alkynyl ligands.In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end-on) and η2 (side on) modes, includes non-bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co-ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero-bi-metallic coinage metal clusters of alkynyl ligands.
In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both (1) (end-on) and (2) (side on) modes, includes non-bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co-ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero-bi-metallic coinage metal clusters of alkynyl ligands.
In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η 1 (end‐on) and η 2 (side on) modes, includes non‐bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co‐ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero‐bi‐metallic coinage metal clusters of alkynyl ligands.
In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η1 (end‐on) and η2 (side on) modes, includes non‐bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co‐ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero‐bi‐metallic coinage metal clusters of alkynyl ligands. Coin toss: Syntheses, structural traits and properties of alkynyl coinage metals clusters are discussed and compared. Concepts and synthetic strategies are highlighted.
In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of alkynyl, that exhibit both η (end-on) and η (side on) modes, includes non-bridged systems, as well as bridging of up to four (or six) metal centres. Resulting metal clusters often exhibit highly regular structures and typical coordination motifs forming fascinating assemblies exploiting this versatile coordination. Metallophilic interactions are often an important driving force for the formation of large clusters. In addition, the use of co-ligands as well the possibility to encapsulate counter ions greatly increases the chemical and structural diversity. Herein we attempt to summarize and highlight design principles towards multinuclear homo and hetero-bi-metallic coinage metal clusters of alkynyl ligands.
Author Orthaber, Andreas
Gupta, Arvind Kumar
Author_xml – sequence: 1
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  surname: Gupta
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  givenname: Andreas
  orcidid: 0000-0001-5403-9902
  surname: Orthaber
  fullname: Orthaber, Andreas
  email: andreas.orthaber@kemi.uu.se
  organization: Uppsala University
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Issue 30
Keywords X-ray crystallography
coinage metals
cluster compounds
alkynyl ligands
metallophilic interactions
Language English
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Snippet In this Concept we discuss how the chemistry of coinage metal complexes based on alkynyl ligands has developed over the past decades. The rich coordination of...
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SubjectTerms alkynyl ligands
Chemistry
cluster compounds
coinage metals
Coordination compounds
Ligands
Metal clusters
Metal complexes
metallophilic interactions
X-ray crystallography
Title Alkynyl Coinage Metal Clusters and Complexes–Syntheses, Structures, and Strategies
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fchem.201704667
https://www.ncbi.nlm.nih.gov/pubmed/29390168
https://www.proquest.com/docview/2047355127
https://www.proquest.com/docview/1993999816
https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-357737
Volume 24
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