2D and 3D Porphyrinic Covalent Organic Frameworks: The Influence of Dimensionality on Functionality

The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting desig...

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Published inAngewandte Chemie International Edition Vol. 59; no. 9; pp. 3624 - 3629
Main Authors Meng, Yi, Luo, Yi, Shi, Ji‐Long, Ding, Huimin, Lang, Xianjun, Chen, Wei, Zheng, Anmin, Sun, Junliang, Wang, Cheng
Format Journal Article
LanguageEnglish
Published WEINHEIM Wiley 24.02.2020
Wiley Subscription Services, Inc
EditionInternational ed. in English
Subjects
Carbon dioxide
Chemistry
Chemistry, Multidisciplinary
CO2 adsorption
COFs
Construction
dimensionality effect
functional moieties
Photocatalysis
Physical Sciences
Science & Technology
size-selective catalysis
Three dimensional models
Topology
Two dimensional models
CATALYSIS
METALATION
COFs
dimensionality effect
functional moieties
PORES
SULFOXIDES
DIFFERENT KINDS
CONSTRUCTION
AEROBIC OXIDATION
DIFFRACTION
size-selective catalysis
CRYSTALLINE
CO2 adsorption
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Abstract The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D‐PdPor‐COF and 3D‐PdPor‐COF) are synthesized. By model building and Rietveld refinement of powder X‐ray diffraction, 2D‐PdPor‐COF crystallizes as 2D sheets while 3D‐PdPor‐COF adopts a five‐fold interpenetrated pts topology. Interestingly, compared with 2D‐PdPor‐COF, 3D‐PdPor‐COF showed interesting properties, including 1) higher CO2 adsorption capacity; 2) better photocatalytic performance; and 3) size‐selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities. 2D vs. 3D COFs: To demonstrate the influence of dimensionality on COF functionality, 2D‐PdPor‐COF and 3D‐PdPor‐COF were synthesized. The results showed that, compared to 2D‐PdPor‐COF, 3D‐PdPor‐COF not only displays higher CO2 adsorption capacity but also exhibits better photocatalytic performance and size selectivity.
AbstractList The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D-PdPor-COF and 3D-PdPor-COF) are synthesized. By model building and Rietveld refinement of powder X-ray diffraction, 2D-PdPor-COF crystallizes as 2D sheets while 3D-PdPor-COF adopts a five-fold interpenetrated pts topology. Interestingly, compared with 2D-PdPor-COF, 3D-PdPor-COF showed interesting properties, including 1) higher CO2 adsorption capacity; 2) better photocatalytic performance; and 3) size-selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities.The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D-PdPor-COF and 3D-PdPor-COF) are synthesized. By model building and Rietveld refinement of powder X-ray diffraction, 2D-PdPor-COF crystallizes as 2D sheets while 3D-PdPor-COF adopts a five-fold interpenetrated pts topology. Interestingly, compared with 2D-PdPor-COF, 3D-PdPor-COF showed interesting properties, including 1) higher CO2 adsorption capacity; 2) better photocatalytic performance; and 3) size-selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities.
The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D-PdPor-COF and 3D-PdPor-COF) are synthesized. By model building and Rietveld refinement of powder X-ray diffraction, 2D-PdPor-COF crystallizes as 2D sheets while 3D-PdPor-COF adopts a five-fold interpenetrated pts topology. Interestingly, compared with 2D-PdPor-COF, 3D-PdPor-COF showed interesting properties, including 1) higher CO2 adsorption capacity; 2) better photocatalytic performance; and 3) size-selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities.
The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D‐PdPor‐COF and 3D‐PdPor‐COF) are synthesized. By model building and Rietveld refinement of powder X‐ray diffraction, 2D‐PdPor‐COF crystallizes as 2D sheets while 3D‐PdPor‐COF adopts a five‐fold interpenetrated pts topology. Interestingly, compared with 2D‐PdPor‐COF, 3D‐PdPor‐COF showed interesting properties, including 1) higher CO2 adsorption capacity; 2) better photocatalytic performance; and 3) size‐selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities. 2D vs. 3D COFs: To demonstrate the influence of dimensionality on COF functionality, 2D‐PdPor‐COF and 3D‐PdPor‐COF were synthesized. The results showed that, compared to 2D‐PdPor‐COF, 3D‐PdPor‐COF not only displays higher CO2 adsorption capacity but also exhibits better photocatalytic performance and size selectivity.
The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D‐PdPor‐COF and 3D‐PdPor‐COF) are synthesized. By model building and Rietveld refinement of powder X‐ray diffraction, 2D‐PdPor‐COF crystallizes as 2D sheets while 3D‐PdPor‐COF adopts a five‐fold interpenetrated pts topology. Interestingly, compared with 2D‐PdPor‐COF, 3D‐PdPor‐COF showed interesting properties, including 1) higher CO 2 adsorption capacity; 2) better photocatalytic performance; and 3) size‐selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities.
The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the influence of COFs dimensionality on their functionalities, which can further assist in COF design, has never been explored. Now, by selecting designed precursors and topology diagrams, 2D and 3D porphyrinic COFs (2D-PdPor-COF and 3D-PdPor-COF) are synthesized. By model building and Rietveld refinement of powder X-ray diffraction, 2D-PdPor-COF crystallizes as 2D sheets while 3D-PdPor-COF adopts a five-fold interpenetrated pts topology. Interestingly, compared with 2D-PdPor-COF, 3D-PdPor-COF showed interesting properties, including 1) higher CO adsorption capacity; 2) better photocatalytic performance; and 3) size-selective photocatalysis. Based on this study, we believe that with the incorporation of functional moieties, the dimensionality of COFs can definitely influence their functionalities.
Author Chen, Wei
Meng, Yi
Ding, Huimin
Lang, Xianjun
Wang, Cheng
Luo, Yi
Shi, Ji‐Long
Sun, Junliang
Zheng, Anmin
Author_xml – sequence: 1
  givenname: Yi
  surname: Meng
  fullname: Meng, Yi
  organization: Wuhan University
– sequence: 2
  givenname: Yi
  surname: Luo
  fullname: Luo, Yi
  organization: Stockholm University
– sequence: 3
  givenname: Ji‐Long
  surname: Shi
  fullname: Shi, Ji‐Long
  organization: Wuhan University
– sequence: 4
  givenname: Huimin
  surname: Ding
  fullname: Ding, Huimin
  organization: Wuhan University
– sequence: 5
  givenname: Xianjun
  orcidid: 0000-0001-7479-9044
  surname: Lang
  fullname: Lang, Xianjun
  organization: Wuhan University
– sequence: 6
  givenname: Wei
  surname: Chen
  fullname: Chen, Wei
  organization: Chinese Academy of Sciences
– sequence: 7
  givenname: Anmin
  surname: Zheng
  fullname: Zheng, Anmin
  organization: Chinese Academy of Sciences
– sequence: 8
  givenname: Junliang
  surname: Sun
  fullname: Sun, Junliang
  email: junliang.sun@pku.edu.cn
  organization: Stockholm University
– sequence: 9
  givenname: Cheng
  orcidid: 0000-0003-0326-2674
  surname: Wang
  fullname: Wang, Cheng
  email: chengwang@whu.edu.cn
  organization: Wuhan University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/31773844$$D View this record in MEDLINE/PubMed
https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-178802$$DView record from Swedish Publication Index
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IsPeerReviewed true
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Issue 9
Keywords CATALYSIS
METALATION
COFs
dimensionality effect
functional moieties
PORES
SULFOXIDES
DIFFERENT KINDS
CONSTRUCTION
AEROBIC OXIDATION
DIFFRACTION
size-selective catalysis
CRYSTALLINE
CO2 adsorption
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Notes These authors contributed equally to this work.
Dedicated to Professor Jean‐Pierre Sauvage on the occasion of his 75th birthday
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Snippet The construction of 2D and 3D covalent organic frameworks (COFs) from functional moieties for desired properties has gained much attention. However, the...
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SubjectTerms Carbon dioxide
Chemistry
Chemistry, Multidisciplinary
CO2 adsorption
COFs
Construction
dimensionality effect
functional moieties
Photocatalysis
Physical Sciences
Science & Technology
size-selective catalysis
Three dimensional models
Topology
Two dimensional models
Title 2D and 3D Porphyrinic Covalent Organic Frameworks: The Influence of Dimensionality on Functionality
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.201913091
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https://www.ncbi.nlm.nih.gov/pubmed/31773844
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https://www.proquest.com/docview/2319197673
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Volume 59
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