Activity Coefficients at Infinite Dilution and Physicochemical Properties for Organic Solutes and Water in the Ionic Liquid 1-Ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate
New data of activity coefficients at infinite dilution, γ 13 ∞ , for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluor...
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| Published in | Journal of solution chemistry Vol. 44; no. 3-4; pp. 413 - 430 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
New York
Springer US
01.04.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | New data of activity coefficients at infinite dilution,
γ
13
∞
, for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate, were determined using inverse gas chromatography within the temperature range from 318.15 to 368.15 K. This is a continuation of our study of ionic liquids based on this anion. The results are compared with the other trifluorotris(perfluoroethyl)phosphate ionic liquids. The
γ
13
∞
values were used to calculate thermodynamic functions such as partial molar excess Gibbs energies
Δ
G
1
E,
∞
, enthalpies
Δ
H
1
E,
∞
and entropies
Δ
S
1
E,
∞
as well as gas–liquid partition coefficients of the solutes,
K
L
. These values were used to determine the linear free energy relationship (LFER) system constants as a function of temperature. The selectivities at infinite dilution needed for some extraction problems were calculated and compared with literature data of ionic liquids based on the trifluorotris(perfluoroethyl)phosphate anion and the 1-ethyl-3-methylimidazolium cation. Additionally, the density and viscosity of the investigated ionic liquid at temperatures from 298.15 to 348.15 K were measured. |
|---|---|
| AbstractList | New data of activity coefficients at infinite dilution,
γ
13
∞
, for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate, were determined using inverse gas chromatography within the temperature range from 318.15 to 368.15 K. This is a continuation of our study of ionic liquids based on this anion. The results are compared with the other trifluorotris(perfluoroethyl)phosphate ionic liquids. The
γ
13
∞
values were used to calculate thermodynamic functions such as partial molar excess Gibbs energies
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\begin{document}$$ \Delta G_{1}^{{{\text{E,}}\infty }} $$\end{document}
Δ
G
1
E,
∞
, enthalpies
\documentclass[12pt]{minimal}
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\begin{document}$$ \Delta H_{1}^{{{\text{E,}}\infty }} $$\end{document}
Δ
H
1
E,
∞
and entropies
\documentclass[12pt]{minimal}
\usepackage{amsmath}
\usepackage{wasysym}
\usepackage{amsfonts}
\usepackage{amssymb}
\usepackage{amsbsy}
\usepackage{mathrsfs}
\usepackage{upgreek}
\setlength{\oddsidemargin}{-69pt}
\begin{document}$$ \Delta S_{1}^{{{\text{E,}}\infty }} $$\end{document}
Δ
S
1
E,
∞
as well as gas–liquid partition coefficients of the solutes,
K
L
. These values were used to determine the linear free energy relationship (LFER) system constants as a function of temperature. The selectivities at infinite dilution needed for some extraction problems were calculated and compared with literature data of ionic liquids based on the trifluorotris(perfluoroethyl)phosphate anion and the 1-ethyl-3-methylimidazolium cation. Additionally, the density and viscosity of the investigated ionic liquid at temperatures from 298.15 to 348.15 K were measured. New data of activity coefficients at infinite dilution, , for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate, were determined using inverse gas chromatography within the temperature range from 318.15 to 368.15 K. This is a continuation of our study of ionic liquids based on this anion. The results are compared with the other trifluorotris(perfluoroethyl)phosphate ionic liquids. The values were used to calculate thermodynamic functions such as partial molar excess Gibbs energies [Formula: see text], enthalpies [Formula: see text] and entropies [Formula: see text] as well as gas-liquid partition coefficients of the solutes, . These values were used to determine the linear free energy relationship (LFER) system constants as a function of temperature. The selectivities at infinite dilution needed for some extraction problems were calculated and compared with literature data of ionic liquids based on the trifluorotris(perfluoroethyl)phosphate anion and the 1-ethyl-3-methylimidazolium cation. Additionally, the density and viscosity of the investigated ionic liquid at temperatures from 298.15 to 348.15 K were measured. New data of activity coefficients at infinite dilution, γ 13 ∞ , for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate, were determined using inverse gas chromatography within the temperature range from 318.15 to 368.15 K. This is a continuation of our study of ionic liquids based on this anion. The results are compared with the other trifluorotris(perfluoroethyl)phosphate ionic liquids. The γ 13 ∞ values were used to calculate thermodynamic functions such as partial molar excess Gibbs energies Δ G 1 E, ∞ , enthalpies Δ H 1 E, ∞ and entropies Δ S 1 E, ∞ as well as gas–liquid partition coefficients of the solutes, K L . These values were used to determine the linear free energy relationship (LFER) system constants as a function of temperature. The selectivities at infinite dilution needed for some extraction problems were calculated and compared with literature data of ionic liquids based on the trifluorotris(perfluoroethyl)phosphate anion and the 1-ethyl-3-methylimidazolium cation. Additionally, the density and viscosity of the investigated ionic liquid at temperatures from 298.15 to 348.15 K were measured. New data of activity coefficients at infinite dilution, gamma sub(13) super( infinity ) , for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons, alcohols, thiophene, ethers, ketones, aldehydes, esters and water in the ionic liquid 1-ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate, were determined using inverse gas chromatography within the temperature range from 318.15 to 368.15 K. This is a continuation of our study of ionic liquids based on this anion. The results are compared with the other trifluorotris(perfluoroethyl)phosphate ionic liquids. The gamma sub(13) super( infinity ) values were used to calculate thermodynamic functions such as partial molar excess Gibbs energies \( \Delta G_{1}{{\text{E,}}\infty }} \), enthalpies \( \Delta H_{1}{{\text{E,}}\infty }} \) and entropies \( \Delta S_{1}{{\text{E,}}\infty }} \) as well as gas-liquid partition coefficients of the solutes, K sub(L). These values were used to determine the linear free energy relationship (LFER) system constants as a function of temperature. The selectivities at infinite dilution needed for some extraction problems were calculated and compared with literature data of ionic liquids based on the trifluorotris(perfluoroethyl)phosphate anion and the 1-ethyl-3-methylimidazolium cation. Additionally, the density and viscosity of the investigated ionic liquid at temperatures from 298.15 to 348.15 K were measured. |
| Author | Letcher, Trevor M. Marciniak, Andrzej Wlazło, Michał |
| Author_xml | – sequence: 1 givenname: Michał surname: Wlazło fullname: Wlazło, Michał email: mwlazlo@ch.pw.edu.pl organization: Department of Physical Chemistry, Faculty of Chemistry, Warsaw University of Technology – sequence: 2 givenname: Andrzej surname: Marciniak fullname: Marciniak, Andrzej organization: Department of Physical Chemistry, Faculty of Chemistry, Warsaw University of Technology – sequence: 3 givenname: Trevor M. surname: Letcher fullname: Letcher, Trevor M. organization: School of Chemistry and Physics, University of KwaZulu-Natal |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25960582$$D View this record in MEDLINE/PubMed |
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| Keywords | 1-Ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate Selectivity LFER [emim][FAP] Activity coefficients at infinite dilution Ionic liquid |
| Language | English |
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| Snippet | New data of activity coefficients at infinite dilution,
γ
13
∞
, for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic... New data of activity coefficients at infinite dilution, , for 65 different solutes including alkanes, alkenes, alkynes, cycloalkanes, aromatic hydrocarbons,... New data of activity coefficients at infinite dilution, gamma sub(13) super( infinity ) , for 65 different solutes including alkanes, alkenes, alkynes,... |
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| SubjectTerms | Activity coefficients Aldehydes Anions Cations Chemistry Chemistry and Materials Science Condensed Matter Physics Dilution Entropy Geochemistry Industrial Chemistry/Chemical Engineering Inorganic Chemistry Ionic liquids Mathematical analysis Oceanography Physical Chemistry |
| Title | Activity Coefficients at Infinite Dilution and Physicochemical Properties for Organic Solutes and Water in the Ionic Liquid 1-Ethyl-3-methylimidazolium trifluorotris(perfluoroethyl)phosphate |
| URI | https://link.springer.com/article/10.1007/s10953-014-0274-0 https://www.ncbi.nlm.nih.gov/pubmed/25960582 https://search.proquest.com/docview/1808056005 https://search.proquest.com/docview/1826616930 https://pubmed.ncbi.nlm.nih.gov/PMC4412692 |
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