Partitioning and granulometric distribution of metal leachate from urban traffic dry deposition particulate matter subject to acidic rainfall and runoff retention
Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods a...
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| Published in | Water research (Oxford) Vol. 42; no. 15; pp. 4146 - 4162 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.09.2008
Elsevier Science |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a
d
50m
=
304
μm and a peak surface area at 106
μm. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75
μm) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75
μm). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour. |
|---|---|
| AbstractList | Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a d sub(5) sub(0) sub(m)=304km and a peak surface area at 106km. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75km) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75km). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour. Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a d 50m = 304 μm and a peak surface area at 106 μm. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75 μm) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75 μm). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour. Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a d(50 m)=304 microm and a peak surface area at 106 microm. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75 microm) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75 microm). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour.Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a d(50 m)=304 microm and a peak surface area at 106 microm. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75 microm) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75 microm). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour. Impact of partitioning and granulometric distribution of metal leachate from urban traffic dry deposition particulate matter (PM) on acidic rainfall and runoff retention, were analyzed. Dry deposition rates of metals varied for different land uses. Dry deposition particles, recovered from a pavement section at a north-south inter-state in Cincinnati, were analyzed for metals. The PM was composted after weighing and preliminary analysis, in order to have sufficient material for subsequent granulometric analysis. Specific surface area (SSA) and surface area (SA) were measured using the EGME method. Metal analysis was conducted with an inductive coupled plasma-mass spectrometer (ICP-MS). The concentration of metals was also examined for separate PM classes. The results demonstrated that acidic rainfall was capable of leaching metals from dry deposition PM into runoff. Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal inventories in urban systems. This study examines the granulometric distribution of metals from dry deposition PM generated from 17 dryfall periods and equilibrium metal partitioning with runoff PM distribution from eight rainfall-runoff events at an urban inter-state watershed in Baton Rouge, LA. Dry deposition PM is a coarse non-uniform gradation with a d(50 m)=304 microm and a peak surface area at 106 microm. Results indicate acid rain is not a significant metal contributor to runoff but is capable of leaching metals from PM to runoff. Retained runoff partitioning resulted in particulate-bound predominance for As, Cd, Cr, Cu, Pb, and Zn while Ca and Mg remained predominately dissolved. The finer PM fraction (<75 microm) generates the highest metal concentrations and the highest metal mass is associated with the coarser fraction (>75 microm). This coarse fraction is also the most labile when exposed to acidic rainfall; generating up to 90% of the total metal mass leached from the entire PM gradation. Comparing dry deposition and runoff PM of equal mass and size gradation, retained runoff PM is enriched with metals (except Pb). Results indicate the labile coarse fraction of dry deposition PM can be a significant source of metal leaching while runoff PM (mobilized dry deposition PM) stored in a BMP can be metal-enriched with the potential for re-leaching or scour. |
| Author | Sansalone, J. Ying, G. |
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| Keywords | Metals Anthropogenic Rainfall-runoff Acid rain Specific surface area Leaching Dry deposition Atmospheric fallout Urban traffic Pollutant behavior Dry matter Urban area Runoff water Transport process Hydrology Watershed Aerosols Lead Lixiviation Air pollution Phase partition Leachate Anthropogenic factor |
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| Snippet | Vehicular transportation coupled with urban hydrology is a significant source as well as vector of particulate matter (PM) and particulate-bound metal... Impact of partitioning and granulometric distribution of metal leachate from urban traffic dry deposition particulate matter (PM) on acidic rainfall and runoff... |
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| SubjectTerms | acid deposition Acid Rain analysis Anthropogenic Applied sciences arsenic cadmium calcium chemistry chromium Cities copper drainage Dry deposition dry matter partitioning Environmental Monitoring Environmental Monitoring - methods Exact sciences and technology leachates Leaching lead Louisiana magnesium Metals Metals - analysis Metals - chemistry methods Other industrial wastes. Sewage sludge particulate emissions Particulate Matter Particulate Matter - analysis Particulate Matter - chemistry Pollution rain Rainfall-runoff runoff Specific surface area traffic urban areas Wastes Water Movements Water Pollutants, Chemical Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry water pollution Water treatment and pollution watersheds zinc |
| Title | Partitioning and granulometric distribution of metal leachate from urban traffic dry deposition particulate matter subject to acidic rainfall and runoff retention |
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