Study on the impact of industrial flue gases on the PCDD/Fs congener profile in ambient air
•We examined the impact of combustion processes on the PCDD/F profile in ambient air.•We determined seventeen PCDD/F congeners in flue gas and ambient air samples.•PCDD distribution in flue gas samples is similar regardless of emission source.•PCDD profiles in ambient air are parallel and related to...
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| Published in | Chemosphere (Oxford) Vol. 114; pp. 76 - 83 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier Ltd
01.11.2014
Elsevier |
| Subjects | |
| Online Access | Get full text |
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| Abstract | •We examined the impact of combustion processes on the PCDD/F profile in ambient air.•We determined seventeen PCDD/F congeners in flue gas and ambient air samples.•PCDD distribution in flue gas samples is similar regardless of emission source.•PCDD profiles in ambient air are parallel and related to those in flue gas samples.•PCDF distribution in ambient air depends on the site of sampling and flue gas emitter.
The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the PCDD and PCDF congener profile in ambient air in Krakow (city in Poland).
The subject matter of the study were air samples from the outskirts and the city center.
It was found that in flue gases from industrial sources and in ambient air the share of PCDF congeners in relation to the total content of PCDD/Fs was higher than the share of PCDDs. However, in air samples collected in the city center, this relationship was reversed.
The PCDD congener profiles in flue gases and in air samples are comparable. However, in the samples from the city centre, the share of OCDD is significantly higher and amounts to about 80%.
The PCDF congener shares show higher spatial diversity, although in all the analyzed air samples, ODCF and 1,2,3,4,6,7,8 HpCDF dominated.
Analyzing the share of congeners in regard to the sum of PCDDs/Fs a mutual resemblance of air from the suburbs, exhaust gases from the sinter ore and sewage sludge incinerator plant was observed. The study showed a similarity between the profile of congeners in air from the city centre and exhaust gases from the medical waste incinerator. |
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| AbstractList | •We examined the impact of combustion processes on the PCDD/F profile in ambient air.•We determined seventeen PCDD/F congeners in flue gas and ambient air samples.•PCDD distribution in flue gas samples is similar regardless of emission source.•PCDD profiles in ambient air are parallel and related to those in flue gas samples.•PCDF distribution in ambient air depends on the site of sampling and flue gas emitter.
The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the PCDD and PCDF congener profile in ambient air in Krakow (city in Poland).
The subject matter of the study were air samples from the outskirts and the city center.
It was found that in flue gases from industrial sources and in ambient air the share of PCDF congeners in relation to the total content of PCDD/Fs was higher than the share of PCDDs. However, in air samples collected in the city center, this relationship was reversed.
The PCDD congener profiles in flue gases and in air samples are comparable. However, in the samples from the city centre, the share of OCDD is significantly higher and amounts to about 80%.
The PCDF congener shares show higher spatial diversity, although in all the analyzed air samples, ODCF and 1,2,3,4,6,7,8 HpCDF dominated.
Analyzing the share of congeners in regard to the sum of PCDDs/Fs a mutual resemblance of air from the suburbs, exhaust gases from the sinter ore and sewage sludge incinerator plant was observed. The study showed a similarity between the profile of congeners in air from the city centre and exhaust gases from the medical waste incinerator. The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the PCDD and PCDF congener profile in ambient air in Krakow (city in Poland). The subject matter of the study were air samples from the outskirts and the city center. It was found that in flue gases from industrial sources and in ambient air the share of PCDF congeners in relation to the total content of PCDD/Fs was higher than the share of PCDDs. However, in air samples collected in the city center, this relationship was reversed. The PCDD congener profiles in flue gases and in air samples are comparable. However, in the samples from the city centre, the share of OCDD is significantly higher and amounts to about 80%. The PCDF congener shares show higher spatial diversity, although in all the analyzed air samples, ODCF and 1,2,3,4,6,7,8 HpCDF dominated. Analyzing the share of congeners in regard to the sum of PCDDs/Fs a mutual resemblance of air from the suburbs, exhaust gases from the sinter ore and sewage sludge incinerator plant was observed. The study showed a similarity between the profile of congeners in air from the city centre and exhaust gases from the medical waste incinerator. The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the PCDD and PCDF congener profile in ambient air in Krakow (city in Poland). The subject matter of the study were air samples from the outskirts and the city center. It was found that in flue gases from industrial sources and in ambient air the share of PCDF congeners in relation to the total content of PCDD/Fs was higher than the share of PCDDs. However, in air samples collected in the city center, this relationship was reversed. The PCDD congener profiles in flue gases and in air samples are comparable. However, in the samples from the city centre, the share of OCDD is significantly higher and amounts to about 80%. The PCDF congener shares show higher spatial diversity, although in all the analyzed air samples, ODCF and 1,2,3,4,6,7,8 HpCDF dominated. Analyzing the share of congeners in regard to the sum of PCDDs/Fs a mutual resemblance of air from the suburbs, exhaust gases from the sinter ore and sewage sludge incinerator plant was observed. The study showed a similarity between the profile of congeners in air from the city centre and exhaust gases from the medical waste incinerator.The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the PCDD and PCDF congener profile in ambient air in Krakow (city in Poland). The subject matter of the study were air samples from the outskirts and the city center. It was found that in flue gases from industrial sources and in ambient air the share of PCDF congeners in relation to the total content of PCDD/Fs was higher than the share of PCDDs. However, in air samples collected in the city center, this relationship was reversed. The PCDD congener profiles in flue gases and in air samples are comparable. However, in the samples from the city centre, the share of OCDD is significantly higher and amounts to about 80%. The PCDF congener shares show higher spatial diversity, although in all the analyzed air samples, ODCF and 1,2,3,4,6,7,8 HpCDF dominated. Analyzing the share of congeners in regard to the sum of PCDDs/Fs a mutual resemblance of air from the suburbs, exhaust gases from the sinter ore and sewage sludge incinerator plant was observed. The study showed a similarity between the profile of congeners in air from the city centre and exhaust gases from the medical waste incinerator. |
| Author | Chrząszcz, Ryszard Maślanka, Anna Grochowalski, Adam Węgiel, Małgorzata |
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| Keywords | Emission PCDD/Fs congener profile Ambient air Passive sampling Dioxin derivatives Metallurgical industry Air quality Urban area Pollutant emission Isomer Persistent organic pollutant Gaseous effluent Incineration plant Passive detection Ambient air concentration Chlorine Organic compounds Air pollution Sampling |
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| Snippet | •We examined the impact of combustion processes on the PCDD/F profile in ambient air.•We determined seventeen PCDD/F congeners in flue gas and ambient air... The aim of this study was to examine the impact of emissions from combustion processes from sinter, medical, waste and sewage waste incineration plants on the... |
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| SubjectTerms | air Air - analysis Air Pollutants - analysis Ambient air Applied sciences Atmospheric pollution Benzofurans - analysis City centres combustion Combustion and energy production Congeners Dibenzofurans, Polychlorinated Emission emissions Exact sciences and technology Exhaust gases Flue gases Gases - analysis Incineration Incinerators Industry Medical Waste - analysis Medical wastes Passive sampling PCDD/Fs congener profile Poland Pollution Pollution sources. Measurement results polychlorinated dibenzodioxins Polychlorinated Dibenzodioxins - analogs & derivatives Polychlorinated Dibenzodioxins - analysis polychlorinated dibenzofurans sewage Sewage - analysis sewage sludge Similarity Sinter waste incineration |
| Title | Study on the impact of industrial flue gases on the PCDD/Fs congener profile in ambient air |
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