A review of Sb2Se3 photovoltaic absorber materials and thin-film solar cells

Energy generated from environmentally friendly, cost-effective solar cells is a key aspect for developing a clean renewable-energy economy. Non-toxic and Earth-abundant materials with high absorption coefficient (>105 cm−1) and optimal bandgap (1–1.5 eV) have received great attention as photovolt...

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Published in	Solar Energy Vol. 201; pp. 227 - 246
Main Authors	Mavlonov, Abdurashid, Razykov, Takhir, Raziq, Fazal, Gan, Jiantuo, Chantana, Jakapan, Kawano, Yu, Nishimura, Takahito, Wei, Haoming, Zakutayev, Andriy, Minemoto, Takashi, Zu, Xiaotao, Li, Sean, Qiao, Liang
Format	Journal Article
Language	English
Published	New York Elsevier Ltd 01.05.2020 Elsevier BV Pergamon Press Inc Elsevier
Subjects	Absorbers (materials) Absorption Absorptivity Antimony Antimony compounds Carrier management Clean energy Energy conversion efficiency Energy gap Limiting factors Material properties MATERIALS SCIENCE Open-circuit voltage deficit Photovoltaic cells Photovoltaics Sb2Se3 Selenide Selenides Solar cells SOLAR ENERGY Thin films Thin-film solar cells Titanium dioxide Zinc oxide Thin-film solar cells Sb2Se3 Open-circuit voltage deficit Carrier management Photovoltaics
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Abstract	Energy generated from environmentally friendly, cost-effective solar cells is a key aspect for developing a clean renewable-energy economy. Non-toxic and Earth-abundant materials with high absorption coefficient (>105 cm−1) and optimal bandgap (1–1.5 eV) have received great attention as photovoltaic (PV) absorber layers during the last few decades. Among them, antimony selenide (Sb2Se3) has been a promising PV absorber, with steadily increasing power-conversion efficiency (PCE) compared to other emerging compounds. Very recent studies showed that high-quality ZnO:Al/ZnO/CdS/TiO2/Sb2Se3/MoSe2/Mo devices with PCE of 9.2% can be fabricated using cost-effective novel compounds. Considering these recent advances, this article provides an overview of the material properties of Sb2Se3 thin films and the recent progress made with Sb2Se3-based solar cells. Analysis of Sb2Se3-based thin-film solar cells has also shown that the devices have relatively good light management due to their suitable bandgap and high absorption coefficient, whereas carrier management, i.e. collection efficiency of photo-generated carriers, needs significant improvement. Overall, this study provides background knowledge on material properties and device performance and suggests main research directions to overcome the limiting factors of solar cell performance.
AbstractList	Energy generated from environmentally friendly, cost-effective solar cells is a key aspect for developing a clean renewable-energy economy. Non-toxic and Earth-abundant materials with high absorption coefficient (>105 cm−1) and optimal bandgap (1–1.5 eV) have received great attention as photovoltaic (PV) absorber layers during the last few decades. Among them, antimony selenide (Sb2Se3) has been a promising PV absorber, with steadily increasing power-conversion efficiency (PCE) compared to other emerging compounds. Very recent studies showed that high-quality ZnO:Al/ZnO/CdS/TiO2/Sb2Se3/MoSe2/Mo devices with PCE of 9.2% can be fabricated using cost-effective novel compounds. Considering these recent advances, this article provides an overview of the material properties of Sb2Se3 thin films and the recent progress made with Sb2Se3-based solar cells. Analysis of Sb2Se3-based thin-film solar cells has also shown that the devices have relatively good light management due to their suitable bandgap and high absorption coefficient, whereas carrier management, i.e. collection efficiency of photo-generated carriers, needs significant improvement. Overall, this study provides background knowledge on material properties and device performance and suggests main research directions to overcome the limiting factors of solar cell performance. Energy generated from environmentally friendly, cost-effective solar cells is a key aspect for developing a clean renewable-energy economy. Non-toxic and Earth-abundant materials with high absorption coefficient (>105 cm-1) and optimal bandgap (1-1.5 eV) have received great attention as photovoltaic (PV) absorber layers during the last few decades. Among them, antimony selenide (Sb2Se3) has been a promising PV absorber, with steadily increasing power-conversion efficiency (PCE) compared to other emerging compounds. Very recent studies showed that high-quality ZnO:Al/ZnO/CdS/TiO2/Sb2Se3/MoSe2/Mo devices with PCE of 9.2% can be fabricated using cost-effective novel compounds. Considering these recent advances, this article provides an overview of the material properties of Sb2Se3 thin films and the recent progress made with Sb2Se3-based solar cells. Furthermore, analysis of Sb2Se3-based thin-film solar cells has also shown that the devices have relatively good light management due to their suitable bandgap and high absorption coefficient, whereas carrier management, i.e. collection efficiency of photo-generated carriers, needs significant improvement. Overall, this study provides background knowledge on material properties and device performance and suggests main research directions to overcome the limiting factors of solar cell performance.
Author	Mavlonov, Abdurashid Minemoto, Takashi Razykov, Takhir Zu, Xiaotao Wei, Haoming Nishimura, Takahito Chantana, Jakapan Kawano, Yu Gan, Jiantuo Zakutayev, Andriy Li, Sean Raziq, Fazal Qiao, Liang
Author_xml	– sequence: 1 givenname: Abdurashid orcidid: 0000-0001-7486-6382 surname: Mavlonov fullname: Mavlonov, Abdurashid email: mavlonov@uestc.edu.cn organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 610054, China – sequence: 2 givenname: Takhir surname: Razykov fullname: Razykov, Takhir organization: Physical-Technical Institute, Uzbekistan Academy of Sciences, Bodomzor Yoli 2“B”, Tashkent 100084, Uzbekistan – sequence: 3 givenname: Fazal surname: Raziq fullname: Raziq, Fazal organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 610054, China – sequence: 4 givenname: Jiantuo surname: Gan fullname: Gan, Jiantuo organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 610054, China – sequence: 5 givenname: Jakapan orcidid: 0000-0001-9062-0577 surname: Chantana fullname: Chantana, Jakapan organization: Department of Electrical and Electronic Engineering, Ritsumeikan University, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan – sequence: 6 givenname: Yu orcidid: 0000-0002-5711-4979 surname: Kawano fullname: Kawano, Yu organization: Department of Electrical and Electronic Engineering, Ritsumeikan University, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan – sequence: 7 givenname: Takahito orcidid: 0000-0002-3054-5525 surname: Nishimura fullname: Nishimura, Takahito organization: Ritsumeikan Global Innovation Research Organization, Ritsumeikan University, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan – sequence: 8 givenname: Haoming surname: Wei fullname: Wei, Haoming organization: School of Physics and Physical Engineering, Shandong Provincial Key Laboratory of Laser Polarization and Information Technology, Qufu Normal University, Qufu 273165, China – sequence: 9 givenname: Andriy orcidid: 0000-0002-3343-7538 surname: Zakutayev fullname: Zakutayev, Andriy email: andriy.zakutayev@nrel.gov organization: National Renewable Energy Laboratory, Golden, CO 80401, USA – sequence: 10 givenname: Takashi surname: Minemoto fullname: Minemoto, Takashi organization: Department of Electrical and Electronic Engineering, Ritsumeikan University, 1-1-1 Nojihigashi, Kusatsu, Shiga 525-8577, Japan – sequence: 11 givenname: Xiaotao surname: Zu fullname: Zu, Xiaotao organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 610054, China – sequence: 12 givenname: Sean surname: Li fullname: Li, Sean organization: School of Materials, University of New South Wales, Sydney 2052, NSW, Australia – sequence: 13 givenname: Liang surname: Qiao fullname: Qiao, Liang email: liang.qiao@uestc.edu.cn organization: School of Physics, University of Electronic Science and Technology of China, Chengdu 610054, China
BackLink	https://cir.nii.ac.jp/crid/1872272492633937152$$DView record in CiNii https://www.osti.gov/servlets/purl/1606129$$D View this record in Osti.gov
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Snippet	Energy generated from environmentally friendly, cost-effective solar cells is a key aspect for developing a clean renewable-energy economy. Non-toxic and...
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SubjectTerms	Absorbers (materials) Absorption Absorptivity Antimony Antimony compounds Carrier management Clean energy Energy conversion efficiency Energy gap Limiting factors Material properties MATERIALS SCIENCE Open-circuit voltage deficit Photovoltaic cells Photovoltaics Sb2Se3 Selenide Selenides Solar cells SOLAR ENERGY Thin films Thin-film solar cells Titanium dioxide Zinc oxide
Title	A review of Sb2Se3 photovoltaic absorber materials and thin-film solar cells
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