Ideal Bandgap Organic–Inorganic Hybrid Perovskite Solar Cells
Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells...
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| Published in | Advanced materials (Weinheim) Vol. 29; no. 47 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Wiley Subscription Services, Inc
01.12.2017
Wiley Blackwell (John Wiley & Sons) |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub‐bandgap photons and thermalization loss of above‐bandgap photons as demonstrated by the Shockley–Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb0.5Sn0.5(I0.8Br0.2)3) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced Voc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement.
An ideal‐bandgap (1.35 eV) perovskite (MAPb0.5Sn0.5(I0.8Br0.2)3) is developed with lower non‐radiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, yielding a reduced open‐circuit voltage loss of 0.45 V and improved efficiency of 17.63%. This work provides a promising platform for unleashing the complete potential of ideal‐bandgap perovskite solar cells. |
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| AbstractList | Abstract
Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub‐bandgap photons and thermalization loss of above‐bandgap photons as demonstrated by the Shockley–Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb
0.5
Sn
0.5
(I
0.8
Br
0.2
)
3
) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced
V
oc,loss
(0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub‐bandgap photons and thermalization loss of above‐bandgap photons as demonstrated by the Shockley–Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb 0.5 Sn 0.5 (I 0.8 Br 0.2 ) 3 ) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced V oc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub‐bandgap photons and thermalization loss of above‐bandgap photons as demonstrated by the Shockley–Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb0.5Sn0.5(I0.8Br0.2)3) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced Voc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. An ideal‐bandgap (1.35 eV) perovskite (MAPb0.5Sn0.5(I0.8Br0.2)3) is developed with lower non‐radiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, yielding a reduced open‐circuit voltage loss of 0.45 V and improved efficiency of 17.63%. This work provides a promising platform for unleashing the complete potential of ideal‐bandgap perovskite solar cells. Extremely high power conversion efficiencies (PCEs) of ≈20-22% are realized through intensive research and development of 1.5-1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3-1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub-bandgap photons and thermalization loss of above-bandgap photons as demonstrated by the Shockley-Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb Sn (I Br ) ) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced V (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. Extremely high power conversion efficiencies (PCEs) of ≈20-22% are realized through intensive research and development of 1.5-1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3-1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub-bandgap photons and thermalization loss of above-bandgap photons as demonstrated by the Shockley-Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb0.5 Sn0.5 (I0.8 Br0.2 )3 ) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced Voc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement.Extremely high power conversion efficiencies (PCEs) of ≈20-22% are realized through intensive research and development of 1.5-1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3-1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub-bandgap photons and thermalization loss of above-bandgap photons as demonstrated by the Shockley-Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb0.5 Sn0.5 (I0.8 Br0.2 )3 ) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced Voc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite absorbers. However, development of ideal bandgap (1.3–1.4 eV) absorbers is pivotal to further improve PCE of single junction perovskite solar cells (PVSCs) because of a better balance between absorption loss of sub‐bandgap photons and thermalization loss of above‐bandgap photons as demonstrated by the Shockley–Queisser detailed balanced calculation. Ideal bandgap PVSCs are currently hindered by the poor optoelectronic quality of perovskite absorbers and their PCEs have stagnated at <15%. In this work, through systematic photoluminescence and photovoltaic analysis, a new ideal bandgap (1.35 eV) absorber composition (MAPb0.5Sn0.5(I0.8Br0.2)3) is rationally designed and developed, which possesses lower nonradiative recombination states, band edge disorder, and Urbach energy coupled with a higher absorption coefficient, which yields a reduced Voc,loss (0.45 V) and improved PCE (as high as 17.63%) for the derived PVSCs. This work provides a promising platform for unleashing the complete potential of ideal bandgap PVSCs and prospects for further improvement. |
| Author | Rajagopal, Adharsh Yang, Zhibin Jen, Alex K.‐Y. |
| Author_xml | – sequence: 1 givenname: Zhibin orcidid: 0000-0003-4036-9446 surname: Yang fullname: Yang, Zhibin organization: University of Washington – sequence: 2 givenname: Adharsh surname: Rajagopal fullname: Rajagopal, Adharsh organization: University of Washington – sequence: 3 givenname: Alex K.‐Y. orcidid: 0000-0002-9219-7749 surname: Jen fullname: Jen, Alex K.‐Y. email: ajen@uw.edu organization: City University of Hong Kong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29134752$$D View this record in MEDLINE/PubMed https://www.osti.gov/biblio/1413784$$D View this record in Osti.gov |
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| Copyright | 2017 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Keywords | Pb-Sn binary alloys Shockley-Queisser limit compositional engineering open-circuit voltage optical simulations |
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| Snippet | Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap perovskite... Extremely high power conversion efficiencies (PCEs) of ≈20-22% are realized through intensive research and development of 1.5-1.6 eV bandgap perovskite... Abstract Extremely high power conversion efficiencies (PCEs) of ≈20–22% are realized through intensive research and development of 1.5–1.6 eV bandgap... |
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| SubjectTerms | Absorbers Absorptivity compositional engineering Energy conversion efficiency Materials science open‐circuit voltage optical simulations Optoelectronics Pb–Sn binary alloys Photoluminescence Photons Photovoltaic cells R&D Research & development Shockley–Queisser limit Solar cells Thermalization (energy absorption) |
| Title | Ideal Bandgap Organic–Inorganic Hybrid Perovskite Solar Cells |
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