Nickel-cobalt bimetallic anode catalysts for direct urea fuel cell
Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve...
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| Published in | Scientific reports Vol. 4; no. 1; p. 5863 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
29.08.2014
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm
−2
when 0.33 M urea was used as fuel, O
2
as oxidant at 60°C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm
−2
with an open circuit voltage of 0.38 V at 60°C. |
|---|---|
| AbstractList | Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm(-2) when 0.33 M urea was used as fuel, O2 as oxidant at 60 °C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm(-2) with an open circuit voltage of 0.38 V at 60 °C. Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm(-2) when 0.33 M urea was used as fuel, O2 as oxidant at 60 °C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm(-2) with an open circuit voltage of 0.38 V at 60 °C.Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm(-2) when 0.33 M urea was used as fuel, O2 as oxidant at 60 °C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm(-2) with an open circuit voltage of 0.38 V at 60 °C. Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm −2 when 0.33 M urea was used as fuel, O 2 as oxidant at 60°C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm −2 with an open circuit voltage of 0.38 V at 60°C. Nickel is an ideal non-noble metal anode catalyst for direct urea fuel cell (DUFC) due to its high activity. However, there exists a large overpotential toward urea electrooxidation. Herein, NiCo/C bimetallic nanoparticles were prepared with various Co contents (0, 10, 20, 30 and 40 wt%) to improve the activity. The best Co ratio was 10% in the aspect of cell performance, with a maximum power density of 1.57 mW cm-2 when 0.33 M urea was used as fuel, O2 as oxidant at 60°C. The effects of temperature and urea concentration on DUFC performance were investigated. Besides, direct urine fuel cell reaches a maximum power density of 0.19 mW cm-2 with an open circuit voltage of 0.38 V at 60°C. |
| ArticleNumber | 5863 |
| Author | Wu, Zucheng Zhang, Huimin Li, Gang Xu, Wei |
| Author_xml | – sequence: 1 givenname: Wei surname: Xu fullname: Xu, Wei organization: Department of Environmental Engineering, Laboratory of Electrochemistry and Energy Storage, State Key laboratory of Clean Energy Utilization, Zhejiang University – sequence: 2 givenname: Huimin surname: Zhang fullname: Zhang, Huimin organization: Department of Environmental Engineering, Laboratory of Electrochemistry and Energy Storage, State Key laboratory of Clean Energy Utilization, Zhejiang University – sequence: 3 givenname: Gang surname: Li fullname: Li, Gang organization: Department of Environmental Engineering, Laboratory of Electrochemistry and Energy Storage, State Key laboratory of Clean Energy Utilization, Zhejiang University – sequence: 4 givenname: Zucheng surname: Wu fullname: Wu, Zucheng organization: Department of Environmental Engineering, Laboratory of Electrochemistry and Energy Storage, State Key laboratory of Clean Energy Utilization, Zhejiang University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25168632$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | 147/135 147/143 639/638/161 639/638/77 Catalysis Catalysts Cobalt Cobalt - chemistry conference-proceeding Electric Power Supplies Electrodes Fuel cells Fuel technology Humanities and Social Sciences Humans multidisciplinary Nanoparticles Nickel Nickel - chemistry Oxidizing agents Particle Size Science Temperature effects Urea Urea - chemistry Urine Urine - chemistry |
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| Title | Nickel-cobalt bimetallic anode catalysts for direct urea fuel cell |
| URI | https://link.springer.com/article/10.1038/srep05863 https://www.ncbi.nlm.nih.gov/pubmed/25168632 https://www.proquest.com/docview/1898154000 https://www.proquest.com/docview/1559624090 https://pubmed.ncbi.nlm.nih.gov/PMC4148665 |
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