Optical signature of symmetry variations and spin-valley coupling in atomically thin tungsten dichalcogenides
We report systematic optical studies of WS 2 and WSe 2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (...
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| Published in | Scientific reports Vol. 3; no. 1; p. 1608 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
11.04.2013
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | We report systematic optical studies of WS
2
and WSe
2
monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (PL) measurements show the crossover from an indirect band gap semiconductor at multilayers to a direct-gap one at monolayers. A hot luminescence peak (B) is observed at ~0.4 eV above the prominent band edge peak (A) in all samples. The magnitude of A-B splitting is independent of the number of layers and coincides with the spin-valley coupling strength in monolayers.
Ab initio
calculations show that this thickness independent splitting pattern is a direct consequence of the giant spin-valley coupling which fully suppresses interlayer hopping at valence band edge near K points because of the sign change of the spin-valley coupling from layer to layer in the 2H stacking order. |
|---|---|
| AbstractList | We report systematic optical studies of WS2 and WSe2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (PL) measurements show the crossover from an indirect band gap semiconductor at multilayers to a direct-gap one at monolayers. A hot luminescence peak (B) is observed at ~0.4 eV above the prominent band edge peak (A) in all samples. The magnitude of A-B splitting is independent of the number of layers and coincides with the spin-valley coupling strength in monolayers. Ab initio calculations show that this thickness independent splitting pattern is a direct consequence of the giant spin-valley coupling which fully suppresses interlayer hopping at valence band edge near K points because of the sign change of the spin-valley coupling from layer to layer in the 2H stacking order. We report systematic optical studies of WS2 and WSe2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (PL) measurements show the crossover from an indirect band gap semiconductor at multilayers to a direct-gap one at monolayers. A hot luminescence peak (B) is observed at ~0.4 eV above the prominent band edge peak (A) in all samples. The magnitude of A-B splitting is independent of the number of layers and coincides with the spin-valley coupling strength in monolayers. Ab initio calculations show that this thickness independent splitting pattern is a direct consequence of the giant spin-valley coupling which fully suppresses interlayer hopping at valence band edge near K points because of the sign change of the spin-valley coupling from layer to layer in the 2H stacking order.We report systematic optical studies of WS2 and WSe2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (PL) measurements show the crossover from an indirect band gap semiconductor at multilayers to a direct-gap one at monolayers. A hot luminescence peak (B) is observed at ~0.4 eV above the prominent band edge peak (A) in all samples. The magnitude of A-B splitting is independent of the number of layers and coincides with the spin-valley coupling strength in monolayers. Ab initio calculations show that this thickness independent splitting pattern is a direct consequence of the giant spin-valley coupling which fully suppresses interlayer hopping at valence band edge near K points because of the sign change of the spin-valley coupling from layer to layer in the 2H stacking order. We report systematic optical studies of WS 2 and WSe 2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd oscillation with the number of layers, consistent with the presence (absence) of inversion symmetry in even-layer (odd-layer). Photoluminescence (PL) measurements show the crossover from an indirect band gap semiconductor at multilayers to a direct-gap one at monolayers. A hot luminescence peak (B) is observed at ~0.4 eV above the prominent band edge peak (A) in all samples. The magnitude of A-B splitting is independent of the number of layers and coincides with the spin-valley coupling strength in monolayers. Ab initio calculations show that this thickness independent splitting pattern is a direct consequence of the giant spin-valley coupling which fully suppresses interlayer hopping at valence band edge near K points because of the sign change of the spin-valley coupling from layer to layer in the 2H stacking order. |
| ArticleNumber | 1608 |
| Author | Zeng, Hualing Cui, Xiaodong Xie, Lu Yan, Yajun Dai, Junfeng Zhu, Bairen He, Ruicong Liu, Gui-Bin Xu, Shijie Chen, Xianhui Yao, Wang |
| Author_xml | – sequence: 1 givenname: Hualing surname: Zeng fullname: Zeng, Hualing organization: Department of Physics, The University of Hong Kong – sequence: 2 givenname: Gui-Bin surname: Liu fullname: Liu, Gui-Bin organization: Department of Physics, The University of Hong Kong, Center for Theoretical and Computational Physics, The University of Hong Kong, School of Physics, Beijing Institute of Technology – sequence: 3 givenname: Junfeng surname: Dai fullname: Dai, Junfeng organization: Department of Physics, The University of Hong Kong, Department of Physics, South University of Science and Technology of China – sequence: 4 givenname: Yajun surname: Yan fullname: Yan, Yajun organization: Hefei National Laboratory for physical Science at Microscale and Department of Physics, University of Science and Technology of China – sequence: 5 givenname: Bairen surname: Zhu fullname: Zhu, Bairen organization: Department of Physics, The University of Hong Kong – sequence: 6 givenname: Ruicong surname: He fullname: He, Ruicong organization: Department of Physics, The University of Hong Kong – sequence: 7 givenname: Lu surname: Xie fullname: Xie, Lu organization: Department of Physics, The University of Hong Kong – sequence: 8 givenname: Shijie surname: Xu fullname: Xu, Shijie organization: Department of Physics, The University of Hong Kong – sequence: 9 givenname: Xianhui surname: Chen fullname: Chen, Xianhui organization: Hefei National Laboratory for physical Science at Microscale and Department of Physics, University of Science and Technology of China – sequence: 10 givenname: Wang surname: Yao fullname: Yao, Wang organization: Department of Physics, The University of Hong Kong, Center for Theoretical and Computational Physics, The University of Hong Kong – sequence: 11 givenname: Xiaodong surname: Cui fullname: Cui, Xiaodong organization: Department of Physics, The University of Hong Kong |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23575911$$D View this record in MEDLINE/PubMed |
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| Snippet | We report systematic optical studies of WS
2
and WSe
2
monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd... We report systematic optical studies of WS2 and WSe2 monolayers and multilayers. The efficiency of second harmonic generation shows a dramatic even-odd... |
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| SubjectTerms | 639/301/119 639/301/119/1000 639/766/119/1001 639/766/119/995 Chalcogens - chemistry Computer Simulation Efficiency Graphene Humanities and Social Sciences Light Luminescence Luminescent Measurements - methods Materials Testing Models, Chemical multidisciplinary Optical properties Photons Physics Scattering, Radiation Science Semiconductors Spin Labels Splitting Symmetry Tungsten Tungsten Compounds - chemistry |
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| Title | Optical signature of symmetry variations and spin-valley coupling in atomically thin tungsten dichalcogenides |
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