The Origin of Fluorescence from Graphene Oxide
Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination from the bottom of the conduction band and nearby localized states to wide-range valance band is suggested as origin of the fluorescence. Exc...
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| Published in | Scientific reports Vol. 2; no. 1; p. 792 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
09.11.2012
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination from the bottom of the conduction band and nearby localized states to wide-range valance band is suggested as origin of the fluorescence. Excitation wavelength dependence of the fluorescence was caused by relative intensity changes of few emission species. By introducing the molecular orbital concept, the dominant fluorescence was found to originate from the electronic transitions among/between the non-oxidized carbon regions and the boundary of oxidized carbon atom regions, where all three kinds of functionalized groups C-O, C = O and O = C-OH were participating. In the visible spectral range, the ultrafast fluorescence of graphene oxide was observed for the first time. |
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| AbstractList | Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination from the bottom of the conduction band and nearby localized states to wide-range valance band is suggested as origin of the fluorescence. Excitation wavelength dependence of the fluorescence was caused by relative intensity changes of few emission species. By introducing the molecular orbital concept, the dominant fluorescence was found to originate from the electronic transitions among/between the non-oxidized carbon regions and the boundary of oxidized carbon atom regions, where all three kinds of functionalized groups C-O, C = O and O = C-OH were participating. In the visible spectral range, the ultrafast fluorescence of graphene oxide was observed for the first time.Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination from the bottom of the conduction band and nearby localized states to wide-range valance band is suggested as origin of the fluorescence. Excitation wavelength dependence of the fluorescence was caused by relative intensity changes of few emission species. By introducing the molecular orbital concept, the dominant fluorescence was found to originate from the electronic transitions among/between the non-oxidized carbon regions and the boundary of oxidized carbon atom regions, where all three kinds of functionalized groups C-O, C = O and O = C-OH were participating. In the visible spectral range, the ultrafast fluorescence of graphene oxide was observed for the first time. Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination from the bottom of the conduction band and nearby localized states to wide-range valance band is suggested as origin of the fluorescence. Excitation wavelength dependence of the fluorescence was caused by relative intensity changes of few emission species. By introducing the molecular orbital concept, the dominant fluorescence was found to originate from the electronic transitions among/between the non-oxidized carbon regions and the boundary of oxidized carbon atom regions, where all three kinds of functionalized groups C-O, C = O and O = C-OH were participating. In the visible spectral range, the ultrafast fluorescence of graphene oxide was observed for the first time. |
| ArticleNumber | 792 |
| Author | Ma, Lin Ai, Wei Li, Jiewei Gurzadyan, Gagik G. Shang, Jingzhi Yu, Ting |
| Author_xml | – sequence: 1 givenname: Jingzhi surname: Shang fullname: Shang, Jingzhi organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 2 givenname: Lin surname: Ma fullname: Ma, Lin organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University – sequence: 3 givenname: Jiewei surname: Li fullname: Li, Jiewei organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Key Laboratory for Organic Electronics & Information Displays (KLOEID) and Institute of Advanced Materials (IAM), Nanjing University of Posts and Telecommunications – sequence: 4 givenname: Wei surname: Ai fullname: Ai, Wei organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Key Laboratory for Organic Electronics & Information Displays (KLOEID) and Institute of Advanced Materials (IAM), Nanjing University of Posts and Telecommunications – sequence: 5 givenname: Ting surname: Yu fullname: Yu, Ting organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Department of Physics, Faculty of Science, National University of Singapore, Graphene Research Centre, National University of Singapore – sequence: 6 givenname: Gagik G. surname: Gurzadyan fullname: Gurzadyan, Gagik G. organization: Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23145316$$D View this record in MEDLINE/PubMed |
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| Snippet | Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination... Time-resolved fluorescence measurements of graphene oxide in water show multiexponential decay kinetics ranging from 1 ps to 2 ns. Electron-hole recombination... |
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| SubjectTerms | 639/624 639/624/399 639/624/584 639/766 Carbon Conduction Fluorescence Graphene Graphite Graphite - chemistry Humanities and Social Sciences Introduced species Kinetics multidisciplinary Optics Oxidation-Reduction Oxides - chemistry Photonics Physics Recombination Science Spectrometry, Fluorescence Spectrum analysis Spectrum Analysis, Raman Water - chemistry |
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| Title | The Origin of Fluorescence from Graphene Oxide |
| URI | https://link.springer.com/article/10.1038/srep00792 https://www.ncbi.nlm.nih.gov/pubmed/23145316 https://www.proquest.com/docview/1897400825 https://www.proquest.com/docview/1151922059 https://pubmed.ncbi.nlm.nih.gov/PMC3494035 |
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