Hierarchical silicon nanowires-carbon textiles matrix as a binder-free anode for high-performance advanced lithium-ion batteries
Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile...
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| Published in | Scientific reports Vol. 3; no. 1; p. 1622 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
09.04.2013
Nature Publishing Group |
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| Online Access | Get full text |
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| Abstract | Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile method. Further, complete lithium-ion batteries based on Si and commercial LiCoO
2
materials were assembled to investigate their corresponding across-the-aboard performances, demonstrating their enhanced specific capacity (2950 mAh g
−1
at 0.2 C), good repeatability/rate capability (even >900 mAh g
−1
at high rate of 5 C), long cycling life and excellent stability in various external conditions (curvature, temperature and humidity). Above results light the way to principally replacing graphite anodes with silicon-based electrodes which was confirmed to have better comprehensive performances. |
|---|---|
| AbstractList | Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile method. Further, complete lithium-ion batteries based on Si and commercial LiCoO2 materials were assembled to investigate their corresponding across-the-aboard performances, demonstrating their enhanced specific capacity (2950 mAh g(-1) at 0.2 C), good repeatability/rate capability (even >900 mAh g(-1) at high rate of 5 C), long cycling life, and excellent stability in various external conditions (curvature, temperature, and humidity). Above results light the way to principally replacing graphite anodes with silicon-based electrodes which was confirmed to have better comprehensive performances. Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile method. Further, complete lithium-ion batteries based on Si and commercial LiCoO2 materials were assembled to investigate their corresponding across-the-aboard performances, demonstrating their enhanced specific capacity (2950 mAh g(-1) at 0.2 C), good repeatability/rate capability (even >900 mAh g(-1) at high rate of 5 C), long cycling life, and excellent stability in various external conditions (curvature, temperature, and humidity). Above results light the way to principally replacing graphite anodes with silicon-based electrodes which was confirmed to have better comprehensive performances.Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile method. Further, complete lithium-ion batteries based on Si and commercial LiCoO2 materials were assembled to investigate their corresponding across-the-aboard performances, demonstrating their enhanced specific capacity (2950 mAh g(-1) at 0.2 C), good repeatability/rate capability (even >900 mAh g(-1) at high rate of 5 C), long cycling life, and excellent stability in various external conditions (curvature, temperature, and humidity). Above results light the way to principally replacing graphite anodes with silicon-based electrodes which was confirmed to have better comprehensive performances. Toward the increasing demands of portable energy storage and electric vehicle applications, the widely used graphite anodes with significant drawbacks become more and more unsuitable. Herein, we report a novel scaffold of hierarchical silicon nanowires-carbon textiles anodes fabricated via a facile method. Further, complete lithium-ion batteries based on Si and commercial LiCoO 2 materials were assembled to investigate their corresponding across-the-aboard performances, demonstrating their enhanced specific capacity (2950 mAh g −1 at 0.2 C), good repeatability/rate capability (even >900 mAh g −1 at high rate of 5 C), long cycling life and excellent stability in various external conditions (curvature, temperature and humidity). Above results light the way to principally replacing graphite anodes with silicon-based electrodes which was confirmed to have better comprehensive performances. |
| ArticleNumber | 1622 |
| Author | Liu, Bin Chen, Di Cheng, Yi-Bing Shen, Guozhen Chen, Haitian Wang, Xianfu Wang, Zhuoran Zhou, Chongwu |
| Author_xml | – sequence: 1 givenname: Bin surname: Liu fullname: Liu, Bin organization: Wuhan National Laboratory for Optoelectronics (WNLO) and College of Optical and Electronic Information, Huazhong University of Science and Technology (HUST) – sequence: 2 givenname: Xianfu surname: Wang fullname: Wang, Xianfu organization: Wuhan National Laboratory for Optoelectronics (WNLO) and College of Optical and Electronic Information, Huazhong University of Science and Technology (HUST) – sequence: 3 givenname: Haitian surname: Chen fullname: Chen, Haitian organization: Department of Electric Engineering, University of Southern California – sequence: 4 givenname: Zhuoran surname: Wang fullname: Wang, Zhuoran organization: Wuhan National Laboratory for Optoelectronics (WNLO) and College of Optical and Electronic Information, Huazhong University of Science and Technology (HUST) – sequence: 5 givenname: Di surname: Chen fullname: Chen, Di organization: Wuhan National Laboratory for Optoelectronics (WNLO) and College of Optical and Electronic Information, Huazhong University of Science and Technology (HUST) – sequence: 6 givenname: Yi-Bing surname: Cheng fullname: Cheng, Yi-Bing organization: Faculty of Engineering, Monash University – sequence: 7 givenname: Chongwu surname: Zhou fullname: Zhou, Chongwu organization: Department of Electric Engineering, University of Southern California – sequence: 8 givenname: Guozhen surname: Shen fullname: Shen, Guozhen organization: Wuhan National Laboratory for Optoelectronics (WNLO) and College of Optical and Electronic Information, Huazhong University of Science and Technology (HUST), State Key Laboratory for Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23572030$$D View this record in MEDLINE/PubMed |
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| Copyright | The Author(s) 2013 Copyright Nature Publishing Group Apr 2013 Copyright © 2013, Macmillan Publishers Limited. All rights reserved 2013 Macmillan Publishers Limited. All rights reserved |
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| Title | Hierarchical silicon nanowires-carbon textiles matrix as a binder-free anode for high-performance advanced lithium-ion batteries |
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