Nano-volcanic Eruption of Silver

Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance...

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Published inScientific reports Vol. 6; no. 1; p. 34769
Main Authors Lin, Shih-kang, Nagao, Shijo, Yokoi, Emi, Oh, Chulmin, Zhang, Hao, Liu, Yu-chen, Lin, Shih-guei, Suganuma, Katsuaki
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 05.10.2016
Nature Publishing Group
Subjects
639/301/1005
639/301/1034
639/638/440/951
Alloys
Crystallization
Heavy metals
Humanities and Social Sciences
multidisciplinary
Oxidation
Science
Silver
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Abstract Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O 2 gas and suspended Ag and Ag 2 O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag “nano-volcanic eruption” mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
AbstractList Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O2 gas and suspended Ag and Ag2 O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag "nano-volcanic eruption" mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O gas and suspended Ag and Ag O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag "nano-volcanic eruption" mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O2 gas and suspended Ag and Ag2O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag "nano-volcanic eruption" mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O 2 gas and suspended Ag and Ag 2 O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag “nano-volcanic eruption” mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
Abstract Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its unique noble and catalytic properties. Ag thin films are extensively used in modern electronics primarily because of their oxidation-resistance. Here we report a novel phenomenon of Ag nano-volcanic eruption that is caused by interactions between Ag and oxygen (O). It involves grain boundary liquation, the ejection of transient Ag-O fluids through grain boundaries, and the decomposition of Ag-O fluids into O 2 gas and suspended Ag and Ag 2 O clusters. Subsequent coating with re-deposited Ag-O and the de-alloying of O yield a conformal amorphous Ag coating. Patterned Ag hillock arrays and direct Ag-to-Ag bonding can be formed by the homogenous crystallization of amorphous coatings. The Ag “nano-volcanic eruption” mechanism is elaborated, shedding light on a new mechanism of hillock formation and new applications of amorphous Ag coatings.
ArticleNumber 34769
Author Yokoi, Emi
Suganuma, Katsuaki
Lin, Shih-guei
Lin, Shih-kang
Nagao, Shijo
Oh, Chulmin
Zhang, Hao
Liu, Yu-chen
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  givenname: Shih-kang
  surname: Lin
  fullname: Lin, Shih-kang
  organization: Department of Materials Science and Engineering, National Cheng Kung University, Center for Micro/Nano Science and Technology, National Cheng Kung University
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  givenname: Shijo
  surname: Nagao
  fullname: Nagao, Shijo
  organization: Institute of Scientific and Industrial Research, Osaka University, Department of Adaptive Machine Systems, Osaka University
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  givenname: Emi
  surname: Yokoi
  fullname: Yokoi, Emi
  organization: Institute of Scientific and Industrial Research, Osaka University
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  surname: Oh
  fullname: Oh, Chulmin
  organization: Department of Adaptive Machine Systems, Osaka University
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  givenname: Hao
  surname: Zhang
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  givenname: Shih-guei
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  fullname: Lin, Shih-guei
  organization: Department of Materials Science and Engineering, National Cheng Kung University
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  givenname: Katsuaki
  surname: Suganuma
  fullname: Suganuma, Katsuaki
  organization: Institute of Scientific and Industrial Research, Osaka University, Department of Adaptive Machine Systems, Osaka University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/27703220$$D View this record in MEDLINE/PubMed
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Snippet Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because of its...
Abstract Silver (Ag) is one of the seven metals of antiquity and an important engineering material in the electronic, medical, and chemical industries because...
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SubjectTerms 639/301/1005
639/301/1034
639/638/440/951
Alloys
Crystallization
Heavy metals
Humanities and Social Sciences
multidisciplinary
Oxidation
Science
Silver
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Title Nano-volcanic Eruption of Silver
URI https://link.springer.com/article/10.1038/srep34769
https://www.ncbi.nlm.nih.gov/pubmed/27703220
https://www.proquest.com/docview/1899099677
https://search.proquest.com/docview/1835360810
https://pubmed.ncbi.nlm.nih.gov/PMC5050507
Volume 6
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