Enhanced Photocatalytic Activity of CdS-Decorated TiO₂/Carbon Core-Shell Microspheres Derived from Microcrystalline Cellulose

The fabrication of reusable and biodegradation materials from renewable resources such as cellulose is essential for a sustainable world. The core-shell structured CdS-decorated TiO₂/Carbon microspheres (CdS/TiO₂/Carbon MS) photocatalyst was synthesized with controlled hydrolysis and a novel sonoche...

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Published inMaterials Vol. 9; no. 4; p. 245
Main Authors Liu, Xin, Li, Yinliang, Yang, Jun, Wang, Bo, Ma, Mingguo, Xu, Feng, Sun, Runcang, Zhang, Xueming
Format Journal Article
LanguageEnglish
Published Switzerland MDPI AG 29.03.2016
MDPI
Subjects
Biocompatibility
Carbon
Catalytic activity
Cellulose
environmental degradation
functional composites
Microscopy
Microspheres
Morphology
Photocatalysis
Pollutants
Polymers
Reusable
Sustainability
Titanium
Titanium dioxide
Toxicity
Beijing China
China
titanium dioxide
photocatalysis
cellulose
functional composites
environmental degradation
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Abstract The fabrication of reusable and biodegradation materials from renewable resources such as cellulose is essential for a sustainable world. The core-shell structured CdS-decorated TiO₂/Carbon microspheres (CdS/TiO₂/Carbon MS) photocatalyst was synthesized with controlled hydrolysis and a novel sonochemical method. It was prepared by using crosslinked microcrystalline cellulose as the core, tetrabutyl titanate as the titania source and CdS as the photosensitizer. The morphology, chemical structure and properties of the obtained material were characterized by many means. Additionally, the photocatalytic activity of the CdS/TiO₂/Carbon MS was evaluated by the photodegradation efficiency of Rhodamine B solution, which reached 95.24% under visible light irradiation. This study demonstrated the excellent photocatalytic performance of CdS/TiO₂/Carbon MS, which might have promising applications in environmental treatments.
AbstractList The fabrication of reusable and biodegradation materials from renewable resources such as cellulose is essential for a sustainable world. The core-shell structured CdS-decorated TiO2/Carbon microspheres (CdS/TiO2/Carbon MS) photocatalyst was synthesized with controlled hydrolysis and a novel sonochemical method. It was prepared by using crosslinked microcrystalline cellulose as the core, tetrabutyl titanate as the titania source and CdS as the photosensitizer. The morphology, chemical structure and properties of the obtained material were characterized by many means. Additionally, the photocatalytic activity of the CdS/TiO2/Carbon MS was evaluated by the photodegradation efficiency of Rhodamine B solution, which reached 95.24% under visible light irradiation. This study demonstrated the excellent photocatalytic performance of CdS/TiO2/Carbon MS, which might have promising applications in environmental treatments.
The fabrication of reusable and biodegradation materials from renewable resources such as cellulose is essential for a sustainable world. The core-shell structured CdS-decorated TiO₂/Carbon microspheres (CdS/TiO₂/Carbon MS) photocatalyst was synthesized with controlled hydrolysis and a novel sonochemical method. It was prepared by using crosslinked microcrystalline cellulose as the core, tetrabutyl titanate as the titania source and CdS as the photosensitizer. The morphology, chemical structure and properties of the obtained material were characterized by many means. Additionally, the photocatalytic activity of the CdS/TiO₂/Carbon MS was evaluated by the photodegradation efficiency of Rhodamine B solution, which reached 95.24% under visible light irradiation. This study demonstrated the excellent photocatalytic performance of CdS/TiO₂/Carbon MS, which might have promising applications in environmental treatments.
The fabrication of reusable and biodegradation materials from renewable resources such as cellulose is essential for a sustainable world. The core-shell structured CdS-decorated TiO 2 /Carbon microspheres (CdS/TiO 2 /Carbon MS) photocatalyst was synthesized with controlled hydrolysis and a novel sonochemical method. It was prepared by using crosslinked microcrystalline cellulose as the core, tetrabutyl titanate as the titania source and CdS as the photosensitizer. The morphology, chemical structure and properties of the obtained material were characterized by many means. Additionally, the photocatalytic activity of the CdS/TiO 2 /Carbon MS was evaluated by the photodegradation efficiency of Rhodamine B solution, which reached 95.24% under visible light irradiation. This study demonstrated the excellent photocatalytic performance of CdS/TiO 2 /Carbon MS, which might have promising applications in environmental treatments.
Author Wang, Bo
Xu, Feng
Ma, Mingguo
Li, Yinliang
Yang, Jun
Zhang, Xueming
Sun, Runcang
Liu, Xin
AuthorAffiliation 1 Beijing Key Laboratory of Lignocellulosic Chemistry, Beijing Forestry University, Beijing 100083, China; xin_liu@bjfu.edu.cn (X.L.); lylhappy@bjfu.edu.cn (Y.L.); yangjun11@bjfu.edu.cn (J.Y.); mzlwb@bjfu.edu.cn (B.W.); mg_ma@bjfu.edu.cn (M.M.); xfx315@bjfu.edu.cn (F.X.); rcsun3@bjfu.edu.cn (R.S.)
2 State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510640, China
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Issue 4
Keywords titanium dioxide
photocatalysis
cellulose
functional composites
environmental degradation
Language English
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SubjectTerms Biocompatibility
Carbon
Catalytic activity
Cellulose
environmental degradation
functional composites
Microscopy
Microspheres
Morphology
Photocatalysis
Pollutants
Polymers
Reusable
Sustainability
Titanium
Titanium dioxide
Toxicity
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Title Enhanced Photocatalytic Activity of CdS-Decorated TiO₂/Carbon Core-Shell Microspheres Derived from Microcrystalline Cellulose
URI https://www.ncbi.nlm.nih.gov/pubmed/28773368
https://www.proquest.com/docview/1780812056
https://search.proquest.com/docview/1808045711
https://search.proquest.com/docview/1926679348
https://pubmed.ncbi.nlm.nih.gov/PMC5502897
https://doaj.org/article/834a94613e0f41a7a970efda420c3a8a
Volume 9
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