Structural characterization of char during co-gasification from torrefied sludge and Yangchangwan bituminous coal

The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO 2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured us...

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Published inInternational journal of coal science & technology Vol. 10; no. 1; pp. 56 - 9
Main Authors Zhang, Xinsha, Bai, Yonghui, Qin, Jie, Shi, Shengli, Liu, Jiazhong, Wang, Shuaibing, Zhao, Minhui, Shi, Guiming, Ye, Changbing, Yu, Guangsuo
Format Journal Article
LanguageEnglish
Published Singapore Springer Nature Singapore 01.12.2023
Springer
Springer Nature B.V
SpringerOpen
Subjects
Atmosphere
Bituminous coal
Carbon dioxide
Char structure
Characteristic
Co-gasification
Coal
Energy
Fossil Fuels (incl. Carbon Capture)
Gasification
Geotechnical Engineering & Applied Earth Sciences
Mineral Resources
Photochemical smog
Raman spectroscopy
Sludge
Sludge treatment
Thermal decomposition
Torrefaction
China
Char structure
Torrefaction
Co-gasification
Characteristic
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Abstract The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO 2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured using a thermogravimetric analyzer. The co-gasification reactivity of torrefied sludge with YC was thoroughly explored in depth by in situ heating stage microscope coupled with traditional characterization means of char sample (Scanning electron microscope, nitrogen adsorption analyzer, laser Raman spectroscopy). The results show that the gasification reaction rate of sludge treated under CO 2 atmosphere and coal blended char was better than other char samples at 1100–1200 °C. The torrefied sludge under CO 2 atmosphere promoted its thermal decomposition to the maximum extent, so that it eventually was transformed into a large number of small broken particles. The specific surface area and I D1 /I G ratio of blended char of torrefied sludge under CO 2 atmosphere and YC were 1.70 and 1.07 times higher than that of YC, respectively. The in situ technique revealed that YC char with the addition of torrefied sludge undergo gasification by shrinking core modes and the presence of obvious ash melting flow phenomenon. It was more obvious than that of YC.
AbstractList The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured using a thermogravimetric analyzer. The co-gasification reactivity of torrefied sludge with YC was thoroughly explored in depth by in situ heating stage microscope coupled with traditional characterization means of char sample (Scanning electron microscope, nitrogen adsorption analyzer, laser Raman spectroscopy). The results show that the gasification reaction rate of sludge treated under CO2 atmosphere and coal blended char was better than other char samples at 1100–1200 °C. The torrefied sludge under CO2 atmosphere promoted its thermal decomposition to the maximum extent, so that it eventually was transformed into a large number of small broken particles. The specific surface area and ID1/IG ratio of blended char of torrefied sludge under CO2 atmosphere and YC were 1.70 and 1.07 times higher than that of YC, respectively. The in situ technique revealed that YC char with the addition of torrefied sludge undergo gasification by shrinking core modes and the presence of obvious ash melting flow phenomenon. It was more obvious than that of YC.
The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO 2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured using a thermogravimetric analyzer. The co-gasification reactivity of torrefied sludge with YC was thoroughly explored in depth by in situ heating stage microscope coupled with traditional characterization means of char sample (Scanning electron microscope, nitrogen adsorption analyzer, laser Raman spectroscopy). The results show that the gasification reaction rate of sludge treated under CO 2 atmosphere and coal blended char was better than other char samples at 1100–1200 °C. The torrefied sludge under CO 2 atmosphere promoted its thermal decomposition to the maximum extent, so that it eventually was transformed into a large number of small broken particles. The specific surface area and I D1 /I G ratio of blended char of torrefied sludge under CO 2 atmosphere and YC were 1.70 and 1.07 times higher than that of YC, respectively. The in situ technique revealed that YC char with the addition of torrefied sludge undergo gasification by shrinking core modes and the presence of obvious ash melting flow phenomenon. It was more obvious than that of YC.
The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO.sub.2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured using a thermogravimetric analyzer. The co-gasification reactivity of torrefied sludge with YC was thoroughly explored in depth by in situ heating stage microscope coupled with traditional characterization means of char sample (Scanning electron microscope, nitrogen adsorption analyzer, laser Raman spectroscopy). The results show that the gasification reaction rate of sludge treated under CO.sub.2 atmosphere and coal blended char was better than other char samples at 1100-1200 °C. The torrefied sludge under CO.sub.2 atmosphere promoted its thermal decomposition to the maximum extent, so that it eventually was transformed into a large number of small broken particles. The specific surface area and I.sub.D1/I.sub.G ratio of blended char of torrefied sludge under CO.sub.2 atmosphere and YC were 1.70 and 1.07 times higher than that of YC, respectively. The in situ technique revealed that YC char with the addition of torrefied sludge undergo gasification by shrinking core modes and the presence of obvious ash melting flow phenomenon. It was more obvious than that of YC.
Abstract The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO2 atmosphere torrefaction pretreated sludge with Yangchangwan bituminous coal (YC) during co-gasification. The co-gasification reactivity of torrefied sludge and YC was measured using a thermogravimetric analyzer. The co-gasification reactivity of torrefied sludge with YC was thoroughly explored in depth by in situ heating stage microscope coupled with traditional characterization means of char sample (Scanning electron microscope, nitrogen adsorption analyzer, laser Raman spectroscopy). The results show that the gasification reaction rate of sludge treated under CO2 atmosphere and coal blended char was better than other char samples at 1100–1200 °C. The torrefied sludge under CO2 atmosphere promoted its thermal decomposition to the maximum extent, so that it eventually was transformed into a large number of small broken particles. The specific surface area and ID1/IG ratio of blended char of torrefied sludge under CO2 atmosphere and YC were 1.70 and 1.07 times higher than that of YC, respectively. The in situ technique revealed that YC char with the addition of torrefied sludge undergo gasification by shrinking core modes and the presence of obvious ash melting flow phenomenon. It was more obvious than that of YC.
ArticleNumber 56
Audience Academic
Author Bai, Yonghui
Qin, Jie
Zhao, Minhui
Zhang, Xinsha
Shi, Shengli
Yu, Guangsuo
Ye, Changbing
Liu, Jiazhong
Wang, Shuaibing
Shi, Guiming
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CitedBy_id crossref_primary_10_1016_j_joei_2024_101946
crossref_primary_10_1016_j_apt_2024_104566
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Snippet The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO 2 atmosphere torrefaction pretreated...
The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO.sub.2 atmosphere torrefaction...
The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO2 atmosphere torrefaction pretreated...
Abstract The present study aims to investigate the physico-chemical structural evolution characteristics of char structure of CO2 atmosphere torrefaction...
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StartPage 56
SubjectTerms Atmosphere
Bituminous coal
Carbon dioxide
Char structure
Characteristic
Co-gasification
Coal
Energy
Fossil Fuels (incl. Carbon Capture)
Gasification
Geotechnical Engineering & Applied Earth Sciences
Mineral Resources
Photochemical smog
Raman spectroscopy
Sludge
Sludge treatment
Thermal decomposition
Torrefaction
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Title Structural characterization of char during co-gasification from torrefied sludge and Yangchangwan bituminous coal
URI https://link.springer.com/article/10.1007/s40789-023-00638-w
https://www.proquest.com/docview/2890356236
https://doaj.org/article/f958b77e0e154621bdf6562b66f31340
Volume 10
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