Time Delays from One-Photon Transitions in the Continuum

We experimentally resolve the time delay of electron wave packets arising from one-photon transitions in the continuum. This allows us to determine and quantify the angular momentum dependence of the photoionization time delay.

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Published in2020 Conference on Lasers and Electro-Optics (CLEO) Vol. 7; no. 2; pp. 1 - 2
Main Authors Fuchs, Jaco, Douguet, Nicolas, Donsa, Stefan, Martin, Fernando, Burgdorfer, Joachim, Argenti, Luca, Cattaneo, Laura, Keller, Ursula
Format Conference Proceeding Journal Article
LanguageEnglish
Published OSA 20.02.2020
Subjects
Absorption
Amplitude modulation
Delay effects
Delays
Ionization
Photonics
Physics
Online AccessGet full text
ISSN2334-2536
2334-2536
DOI10.1364/optica.378639

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Abstract We experimentally resolve the time delay of electron wave packets arising from one-photon transitions in the continuum. This allows us to determine and quantify the angular momentum dependence of the photoionization time delay.
AbstractList We experimentally resolve the time delay of electron wave packets arising from one-photon transitions in the continuum. This allows us to determine and quantify the angular momentum dependence of the photoionization time delay.
Attosecond photoionization time delays reveal information about the potential energy landscape that an outgoing electron wavepacket probes upon ionization. In this study, we experimentally quantify the dependence of the time delay on the angular momentum of the liberated photoelectrons. For this purpose, we resolved electron quantum-path interference spectra in energy and angle using a two-color attosecond pump–probe photoionization experiment in helium. A fitting procedure of the angle-dependent interference pattern allows us to disentangle the relative phase of all four quantum pathways that are known to contribute to the final photoelectron signal. In particular, we resolve the dependence on angular momentum of the delay of one-photon transitions between continuum states, which is an essential and universal contribution to the total photoionization delay observed in attosecond pump–probe measurements. For such continuum–continuum transitions, we measure a delay between outgoing s and d electrons as large as 12 attoseconds, close to the ionization threshold in helium. Both single-active-electron and first-principles ab initio simulations confirm this observation for helium and hydrogen, demonstrating the universality of the observed delays.
Author Donsa, Stefan
Cattaneo, Laura
Keller, Ursula
Martin, Fernando
Fuchs, Jaco
Douguet, Nicolas
Argenti, Luca
Burgdorfer, Joachim
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  surname: Fuchs
  fullname: Fuchs, Jaco
  organization: Department of Physics, Eidgenössische Technische Hochschule Zürich, Zürich, Switzerland
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  givenname: Nicolas
  surname: Douguet
  fullname: Douguet, Nicolas
  organization: Department of Physics, University of Central Florida, Orlando, Florida, USA
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  surname: Donsa
  fullname: Donsa, Stefan
  organization: Institute of Theoretical Physics, Vienna University of Technology, Vienna, Austria, EU
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  givenname: Fernando
  surname: Martin
  fullname: Martin, Fernando
  organization: Departamento de Química Modulo 13, Universidad Autónoma de Madrid, Madrid, Spain, EU; Condensed Matter Physics Center (IFIMAC), Universidad Autonoma de Madrid, Madrid, Spain, EU; Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA-Nano), Madrid, Spain, EU
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  organization: Department of Physics, University of Central Florida, Orlando, Florida, USA; CREOL, University of Central Florida, Orlando, Florida, USA)
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  givenname: Laura
  surname: Cattaneo
  fullname: Cattaneo, Laura
  organization: Department of Physics, Eidgenössische Technische Hochschule Zürich, Zürich, Switzerland
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  givenname: Ursula
  surname: Keller
  fullname: Keller, Ursula
  organization: Department of Physics, Eidgenössische Technische Hochschule Zürich, Zürich, Switzerland
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Snippet We experimentally resolve the time delay of electron wave packets arising from one-photon transitions in the continuum. This allows us to determine and...
Attosecond photoionization time delays reveal information about the potential energy landscape that an outgoing electron wavepacket probes upon ionization. In...
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ieee
SourceType Enrichment Source
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Publisher
StartPage 1
SubjectTerms Absorption
Amplitude modulation
Delay effects
Delays
Ionization
Photonics
Physics
Title Time Delays from One-Photon Transitions in the Continuum
URI https://ieeexplore.ieee.org/document/9192440
Volume 7
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