Fabrication and evaluation of nanocellulose sponge for oil/water separation
[Display omitted] •Superhydrophobic nanocellulose sponge (SA/NC) was simply fabricated.•SA/NC sponge showed excellent superhydrophobicity and superoleophilicity.•SA/NC sponge was suitable to absorb oil spilled in water.•SA/NC sponge was easily recovered by hand squeezing and reused. Nanocellulose sp...
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| Published in | Carbohydrate polymers Vol. 190; pp. 184 - 189 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
15.06.2018
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 0144-8617 1879-1344 1879-1344 |
| DOI | 10.1016/j.carbpol.2018.02.066 |
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| Abstract | [Display omitted]
•Superhydrophobic nanocellulose sponge (SA/NC) was simply fabricated.•SA/NC sponge showed excellent superhydrophobicity and superoleophilicity.•SA/NC sponge was suitable to absorb oil spilled in water.•SA/NC sponge was easily recovered by hand squeezing and reused.
Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment with stearoyl chloride at 50 °C for 1 h. The obtained nanocellulose sponge showed superhydrophobicity (160° of water contact angle) and superoleophilicity with high protection from water but selective absorption of oil. Its absorption capacities for various kinds of oil and non-polar liquids were 25–55 times higher than its dry weight and exhibited excellent selectivity for absorbing of oil which spilled on the surface of water or underwater with high separation efficiency. This superhydrophobic nanocellulose sponge can be easily recovered by simple squeezing and reused at least 10 cycles with remained high separation efficiency. It is expected that such a biodegradable nanocellulose sponge can be applied to solve the oil spill accident and treat the oily wastewater from households and industries. |
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| AbstractList | [Display omitted]
•Superhydrophobic nanocellulose sponge (SA/NC) was simply fabricated.•SA/NC sponge showed excellent superhydrophobicity and superoleophilicity.•SA/NC sponge was suitable to absorb oil spilled in water.•SA/NC sponge was easily recovered by hand squeezing and reused.
Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment with stearoyl chloride at 50 °C for 1 h. The obtained nanocellulose sponge showed superhydrophobicity (160° of water contact angle) and superoleophilicity with high protection from water but selective absorption of oil. Its absorption capacities for various kinds of oil and non-polar liquids were 25–55 times higher than its dry weight and exhibited excellent selectivity for absorbing of oil which spilled on the surface of water or underwater with high separation efficiency. This superhydrophobic nanocellulose sponge can be easily recovered by simple squeezing and reused at least 10 cycles with remained high separation efficiency. It is expected that such a biodegradable nanocellulose sponge can be applied to solve the oil spill accident and treat the oily wastewater from households and industries. Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment with stearoyl chloride at 50 °C for 1 h. The obtained nanocellulose sponge showed superhydrophobicity (160° of water contact angle) and superoleophilicity with high protection from water but selective absorption of oil. Its absorption capacities for various kinds of oil and non-polar liquids were 25-55 times higher than its dry weight and exhibited excellent selectivity for absorbing of oil which spilled on the surface of water or underwater with high separation efficiency. This superhydrophobic nanocellulose sponge can be easily recovered by simple squeezing and reused at least 10 cycles with remained high separation efficiency. It is expected that such a biodegradable nanocellulose sponge can be applied to solve the oil spill accident and treat the oily wastewater from households and industries.Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment with stearoyl chloride at 50 °C for 1 h. The obtained nanocellulose sponge showed superhydrophobicity (160° of water contact angle) and superoleophilicity with high protection from water but selective absorption of oil. Its absorption capacities for various kinds of oil and non-polar liquids were 25-55 times higher than its dry weight and exhibited excellent selectivity for absorbing of oil which spilled on the surface of water or underwater with high separation efficiency. This superhydrophobic nanocellulose sponge can be easily recovered by simple squeezing and reused at least 10 cycles with remained high separation efficiency. It is expected that such a biodegradable nanocellulose sponge can be applied to solve the oil spill accident and treat the oily wastewater from households and industries. Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment with stearoyl chloride at 50 °C for 1 h. The obtained nanocellulose sponge showed superhydrophobicity (160° of water contact angle) and superoleophilicity with high protection from water but selective absorption of oil. Its absorption capacities for various kinds of oil and non-polar liquids were 25–55 times higher than its dry weight and exhibited excellent selectivity for absorbing of oil which spilled on the surface of water or underwater with high separation efficiency. This superhydrophobic nanocellulose sponge can be easily recovered by simple squeezing and reused at least 10 cycles with remained high separation efficiency. It is expected that such a biodegradable nanocellulose sponge can be applied to solve the oil spill accident and treat the oily wastewater from households and industries. |
| Author | Samart, Chanatip Reubroycharoen, Prasert Hao, Xiaogang Phanthong, Patchiya Abudula, Abuliti Guan, Guoqing Wang, Zhongde Kongparakul, Suwadee |
| Author_xml | – sequence: 1 givenname: Patchiya surname: Phanthong fullname: Phanthong, Patchiya organization: Graduate School of Science and Technology, Hirosaki University, 1-Bunkyocho, Hirosaki 036-8560, Japan – sequence: 2 givenname: Prasert surname: Reubroycharoen fullname: Reubroycharoen, Prasert organization: Department of Chemical Technology, Chulalongkorn University, Bangkok 10330, Thailand – sequence: 3 givenname: Suwadee surname: Kongparakul fullname: Kongparakul, Suwadee organization: Department of Chemistry, Faculty of Science and Technology, Thammasat University, Pathumthani 12120, Thailand – sequence: 4 givenname: Chanatip surname: Samart fullname: Samart, Chanatip organization: Department of Chemistry, Faculty of Science and Technology, Thammasat University, Pathumthani 12120, Thailand – sequence: 5 givenname: Zhongde surname: Wang fullname: Wang, Zhongde organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan, Shanxi 030024, PR China – sequence: 6 givenname: Xiaogang surname: Hao fullname: Hao, Xiaogang organization: Department of Chemical Engineering, Taiyuan University of Technology, Taiyuan, Shanxi 030024, PR China – sequence: 7 givenname: Abuliti surname: Abudula fullname: Abudula, Abuliti organization: Graduate School of Science and Technology, Hirosaki University, 1-Bunkyocho, Hirosaki 036-8560, Japan – sequence: 8 givenname: Guoqing orcidid: 0000-0002-5875-3596 surname: Guan fullname: Guan, Guoqing email: guan@hirosaki-u.ac.jp organization: Graduate School of Science and Technology, Hirosaki University, 1-Bunkyocho, Hirosaki 036-8560, Japan |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29628236$$D View this record in MEDLINE/PubMed |
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| Keywords | Oil absorbent Nanocellulose Sponge Oil/water separation Superoleophilicity Superhydrophobicity |
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•Superhydrophobic nanocellulose sponge (SA/NC) was simply fabricated.•SA/NC sponge showed excellent superhydrophobicity and... Nanocellulose sponge was fabricated by a facile method: freeze-drying of nanocellulose aqueous suspension to sponge state, following by hydrophobic treatment... |
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| SubjectTerms | absorption accidents biodegradability cellulose chlorides contact angle freeze drying households hydrophobicity industry Nanocellulose Oil absorbent oil spills Oil/water separation oils organochlorine compounds Sponge Superhydrophobicity Superoleophilicity wastewater |
| Title | Fabrication and evaluation of nanocellulose sponge for oil/water separation |
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