Applications of light scattering in dye-sensitized solar cells
Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar cells, large TiO 2 particles with sizes comparable to the wavelength of visible light are used as scatterers by either being mixed into the nanoc...
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Published in | Physical chemistry chemical physics : PCCP Vol. 14; no. 43; pp. 14982 - 14998 |
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Main Authors | , , , , |
Format | Journal Article |
Language | English |
Published |
Cambridge
Royal Society of Chemistry
01.01.2012
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Abstract | Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar cells, large TiO
2
particles with sizes comparable to the wavelength of visible light are used as scatterers by either being mixed into the nanocrystalline film to generate light scattering or forming a scattering layer on the top of the nanocrystalline film to reflect the incident light, with the aim to extend the traveling distance of incident light within the photoelectrode film. Recently, hierarchical nanostructures, for example nanocrystallite aggregates (among others), have been applied to dye-sensitized solar cells. When used to form a photoelectrode film, these hierarchical nanostructures have demonstrated a dual function: providing large specific surface area; and generating light scattering. Some other merits, such as the capability to enhance electron transport, have been also observed on the hierarchically structured photoelectrode films. Hierarchical nanostructures possessing an architecture that may provide sufficient internal surface area for dye adsorption and meanwhile may generate highly effective light scattering, make them able to create photoelectrode films with optical absorption significantly more efficient than the dispersed nanoparticles used in conventional dye-sensitized solar cells. This allows reduction of the thickness of the photoelectrode film and thus lowering of the charge recombination in dye-sensitized solar cells, making it possible to increase further the efficiency of existing dye-sensitized solar cells.
This paper reviews the applications of light scattering in DSCs over the past two decades and some recent progress in this topic. |
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AbstractList | Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar cells, large TiO(2) particles with sizes comparable to the wavelength of visible light are used as scatterers by either being mixed into the nanocrystalline film to generate light scattering or forming a scattering layer on the top of the nanocrystalline film to reflect the incident light, with the aim to extend the traveling distance of incident light within the photoelectrode film. Recently, hierarchical nanostructures, for example nanocrystallite aggregates (among others), have been applied to dye-sensitized solar cells. When used to form a photoelectrode film, these hierarchical nanostructures have demonstrated a dual function: providing large specific surface area; and generating light scattering. Some other merits, such as the capability to enhance electron transport, have been also observed on the hierarchically structured photoelectrode films. Hierarchical nanostructures possessing an architecture that may provide sufficient internal surface area for dye adsorption and meanwhile may generate highly effective light scattering, make them able to create photoelectrode films with optical absorption significantly more efficient than the dispersed nanoparticles used in conventional dye-sensitized solar cells. This allows reduction of the thickness of the photoelectrode film and thus lowering of the charge recombination in dye-sensitized solar cells, making it possible to increase further the efficiency of existing dye-sensitized solar cells. Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar cells, large TiO sub(2) particles with sizes comparable to the wavelength of visible light are used as scatterers by either being mixed into the nanocrystalline film to generate light scattering or forming a scattering layer on the top of the nanocrystalline film to reflect the incident light, with the aim to extend the traveling distance of incident light within the photoelectrode film. Recently, hierarchical nanostructures, for example nanocrystallite aggregates (among others), have been applied to dye-sensitized solar cells. When used to form a photoelectrode film, these hierarchical nanostructures have demonstrated a dual function: providing large specific surface area; and generating light scattering. Some other merits, such as the capability to enhance electron transport, have been also observed on the hierarchically structured photoelectrode films. Hierarchical nanostructures possessing an architecture that may provide sufficient internal surface area for dye adsorption and meanwhile may generate highly effective light scattering, make them able to create photoelectrode films with optical absorption significantly more efficient than the dispersed nanoparticles used in conventional dye-sensitized solar cells. This allows reduction of the thickness of the photoelectrode film and thus lowering of the charge recombination in dye-sensitized solar cells, making it possible to increase further the efficiency of existing dye-sensitized solar cells. Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar cells, large TiO 2 particles with sizes comparable to the wavelength of visible light are used as scatterers by either being mixed into the nanocrystalline film to generate light scattering or forming a scattering layer on the top of the nanocrystalline film to reflect the incident light, with the aim to extend the traveling distance of incident light within the photoelectrode film. Recently, hierarchical nanostructures, for example nanocrystallite aggregates (among others), have been applied to dye-sensitized solar cells. When used to form a photoelectrode film, these hierarchical nanostructures have demonstrated a dual function: providing large specific surface area; and generating light scattering. Some other merits, such as the capability to enhance electron transport, have been also observed on the hierarchically structured photoelectrode films. Hierarchical nanostructures possessing an architecture that may provide sufficient internal surface area for dye adsorption and meanwhile may generate highly effective light scattering, make them able to create photoelectrode films with optical absorption significantly more efficient than the dispersed nanoparticles used in conventional dye-sensitized solar cells. This allows reduction of the thickness of the photoelectrode film and thus lowering of the charge recombination in dye-sensitized solar cells, making it possible to increase further the efficiency of existing dye-sensitized solar cells. This paper reviews the applications of light scattering in DSCs over the past two decades and some recent progress in this topic. |
Author | Cao, Guozhong Myers, Daniel Jenekhe, Samson A Zhang, Qifeng Lan, Jolin |
AuthorAffiliation | Department of Chemistry Department of Chemical Engineering Department of Materials Science and Engineering University of Washington |
AuthorAffiliation_xml | – name: Department of Chemical Engineering – name: Department of Chemistry – name: University of Washington – name: Department of Materials Science and Engineering |
Author_xml | – sequence: 1 givenname: Qifeng surname: Zhang fullname: Zhang, Qifeng – sequence: 2 givenname: Daniel surname: Myers fullname: Myers, Daniel – sequence: 3 givenname: Jolin surname: Lan fullname: Lan, Jolin – sequence: 4 givenname: Samson A surname: Jenekhe fullname: Jenekhe, Samson A – sequence: 5 givenname: Guozhong surname: Cao fullname: Cao, Guozhong |
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Keywords | Dye-sensitized solar cell Binary compound Particle size Recombination Dyes Film Nanoparticle Light scattering Transition element compounds Nanostructure Wavelength Absorption spectrum Thickness Chemical reduction Adsorption Efficiency Aggregate Surface area Titanium oxide Optical absorption Nanocrystal Photoelectrode |
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Notes | Guozhong Cao is Boeing-Steiner Professor of Materials Science and Engineering, Professor of Chemical Engineering, and Adjunct Professor of Mechanical Engineering at University of Washington. He received his PhD degree from Eindhoven University of Technology, MS from Shanghai Institute of Ceramics of Chinese Academy of Sciences and BS from East China University of Science and Technology. His current research is focused mainly on chemical processing of nanomaterials for energy related applications including solar cells, lithium-ion batteries, supercapacitors, and hydrogen storage. 2 ZnSnS 4 (CZTS)-based thin film solar cells, quantum dot solar cells, and organic/inorganic hybrid solar cells. Samson A. Jenekhe received his BS degree from Michigan Technological University in 1977 and PhD degree from University of Minnesota in 1985. He is currently Boeing-Martin Professor of Chemical Engineering and Professor of Chemistry in the Department of Chemical Engineering at University of Washington. His research interests involve: (1) organic electronics and optoelectronics, including thin film transistors, solar cells, and LEDs; (2) self-assembly and nanotechnology, including block copolymers, nanowires, and multicomponent self-assembly; and (3) polymer science, including synthesis, processing, properties, and photonic applications. Qifeng Zhang earned his PhD degree from Peking University. Currently he is Research Assistant Professor in the Department of Materials Science and Engineering at University of Washington. His research interests involve engineering nano-structured materials for applications to electrical devices, including solar cells, UV light-emitting diodes (LEDs), field-effect transistors (FETs), and gas sensors. His current research is focused on dye-sensitized solar cells (DSCs), Cu ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
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Snippet | Light scattering is a method that has been employed in dye-sensitized solar cells for optical absorption enhancement. In conventional dye-sensitized solar... |
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SubjectTerms | Chemistry Colloidal state and disperse state Dyes Exact sciences and technology General and physical chemistry Incident light Light scattering Nanocrystals Nanostructure Photovoltaic cells Physical and chemical studies. Granulometry. Electrokinetic phenomena Solar cells Surface physical chemistry Titanium dioxide |
Title | Applications of light scattering in dye-sensitized solar cells |
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