Mesoporous TiO2/TiC@C Composite Membranes with Stable TiO2-C Interface for Robust Lithium Storage
Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by a...
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| Published in | iScience Vol. 3; pp. 149 - 160 |
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| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
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25.05.2018
Elsevier |
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| Abstract | Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by an in situ carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO2-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO2/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO2/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO2/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs.
[Display omitted]
•Mesoporous TiO2/TiC@C membranes were synthesized by a simple method•This method can be extended to the synthesis of other metal oxide/metal carbide@C•The TiC nanodots can alleviate tensile and compression stress effect upon lithiation•Long working life and excellent rate performance can be achieved
Composite Materials; Nanomaterials; Energy Materials |
|---|---|
| AbstractList | Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO
2
/TiC@C composite membranes were synthesized by an
in situ
carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO
2
-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO
2
/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO
2
/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO
2
/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs.
•
Mesoporous TiO
2
/TiC@C membranes were synthesized by a simple method
•
This method can be extended to the synthesis of other metal oxide/metal carbide@C
•
The TiC nanodots can alleviate tensile and compression stress effect upon lithiation
•
Long working life and excellent rate performance can be achieved
Composite Materials; Nanomaterials; Energy Materials Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by an in situ carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO2-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO2/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO2/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO2/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs. [Display omitted] •Mesoporous TiO2/TiC@C membranes were synthesized by a simple method•This method can be extended to the synthesis of other metal oxide/metal carbide@C•The TiC nanodots can alleviate tensile and compression stress effect upon lithiation•Long working life and excellent rate performance can be achieved Composite Materials; Nanomaterials; Energy Materials Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by an in situ carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO2-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO2/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO2/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO2/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs. : Composite Materials; Nanomaterials; Energy Materials Subject Areas: Composite Materials, Nanomaterials, Energy Materials Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by an in situ carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO2-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO2/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO2/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO2/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs.Transition metal oxides/carbon (TMOs/C) composites are important for high-performance lithium-ion batteries (LIBs), but the development of interface-stable TMOs/C composite anodes for robust lithium storage is still a challenge. Herein, mesoporous TiO2/TiC@C composite membranes were synthesized by an in situ carbothermic reduction method. TiC nanodots with high conductivity and electrochemical inactivity at the TiO2-C interface can significantly enhance the electrical conductivity and structural stability of the membranes. Finite element simulations demonstrate that the TiO2/TiC@C membranes can effectively alleviate tensile and compression stress effects upon lithiation, which is beneficial for robust lithium storage. When used as additives and binder-free electrodes, the TiO2/TiC@C membranes show excellent cycling capability and rate performance. Moreover, a flexible full battery can be assembled by employing the TiO2/TiC@C membranes and shows good performance, highlighting the potential of these membranes in flexible electronics. This work opens an avenue to constructing interface-stable composite structures for the next-generation high-performance LIBs. |
| Author | Lan, Kun Zhang, Wei Zu, Lianhai Chen, Bingjie Liu, Yang He, Haili Zhao, Dongyuan Kong, Biao Yang, Jinhu |
| AuthorAffiliation | 3 Research Center for Translational Medicine & Key Laboratory of Arrhythmias of the Ministry of Education of China, East Hospital, Tongji University School of Medicine, No. 150 Jimo Road, Shanghai 200120, P. R. China 2 School of Chemical and Engineering, Tongji University, Siping Road 1239, Shanghai 200092, P. R. China 1 Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China |
| AuthorAffiliation_xml | – name: 1 Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – name: 3 Research Center for Translational Medicine & Key Laboratory of Arrhythmias of the Ministry of Education of China, East Hospital, Tongji University School of Medicine, No. 150 Jimo Road, Shanghai 200120, P. R. China – name: 2 School of Chemical and Engineering, Tongji University, Siping Road 1239, Shanghai 200092, P. R. China |
| Author_xml | – sequence: 1 givenname: Wei surname: Zhang fullname: Zhang, Wei organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – sequence: 2 givenname: Lianhai surname: Zu fullname: Zu, Lianhai organization: School of Chemical and Engineering, Tongji University, Siping Road 1239, Shanghai 200092, P. R. China – sequence: 3 givenname: Biao surname: Kong fullname: Kong, Biao organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – sequence: 4 givenname: Bingjie surname: Chen fullname: Chen, Bingjie organization: School of Chemical and Engineering, Tongji University, Siping Road 1239, Shanghai 200092, P. R. China – sequence: 5 givenname: Haili surname: He fullname: He, Haili organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – sequence: 6 givenname: Kun surname: Lan fullname: Lan, Kun organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – sequence: 7 givenname: Yang surname: Liu fullname: Liu, Yang organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China – sequence: 8 givenname: Jinhu surname: Yang fullname: Yang, Jinhu email: yangjinhu@tongji.edu.cn organization: School of Chemical and Engineering, Tongji University, Siping Road 1239, Shanghai 200092, P. R. China – sequence: 9 givenname: Dongyuan surname: Zhao fullname: Zhao, Dongyuan email: dyzhao@fudan.edu.cn organization: Department of Chemistry, State Key Laboratory of Molecular Engineering of Polymers, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, Laboratory of Advanced Materials and iChEM, Fudan University, Shanghai 200433, P. R. China |
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| Title | Mesoporous TiO2/TiC@C Composite Membranes with Stable TiO2-C Interface for Robust Lithium Storage |
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