Ethene/ethane separation by the MOF membrane ZIF-8: Molecular correlation of permeation, adsorption, diffusion

[Display omitted] ▶ ZIF-8 membrane can separate ethene/ethane mixtures with selectivities between 2 and 3. ▶ From mixture adsorption and diffusion data, the membrane selectivity can be predicted. ▶ Both IR microscopy and grand canonical Monte Carlo simulation can give the mixture data. The newly dev...

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Published in	Journal of membrane science Vol. 369; no. 1; pp. 284 - 289
Main Authors	Bux, Helge, Chmelik, Christian, Krishna, Rajamani, Caro, Juergen
Format	Journal Article
Language	English
Published	Amsterdam Elsevier B.V 01.03.2011 Elsevier
Subjects	adsorption ambient temperature artificial membranes Chemistry Colloidal state and disperse state ethane Ethene/ethane separation ethylene Exact sciences and technology GCMC simulations General and physical chemistry IR microscopy Membranes microscopy MOF membrane Monte Carlo method Surface physical chemistry ZIF-8 membrane Ethene/ethane separation ZIF-8 membrane IR microscopy MOF membrane GCMC simulations Monte Carlo method Correlation Separation Ethylene Permeation Selectivity Ethane Single crystal Sorption Adsorption Simulation Membrane Diffusion Room temperature
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Abstract	[Display omitted] ▶ ZIF-8 membrane can separate ethene/ethane mixtures with selectivities between 2 and 3. ▶ From mixture adsorption and diffusion data, the membrane selectivity can be predicted. ▶ Both IR microscopy and grand canonical Monte Carlo simulation can give the mixture data. The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6 bar feed pressure, respectively, with a selectivity of 2.8 and 2.4. Independent sorption uptake studies of an ethene/ethane mixture on a big ZIF-8 single crystal by IR microscopy detection show in combination with grand canonical Monte Carlo simulations that this moderate ethene selectivity of the ZIF-8 membrane can be explained by the interplay of a preferential ethane adsorption selectivity competing with a preferential ethene diffusion selectivity. This means, that ethane adsorbs stronger than ethene, but ethene diffuses faster and overcompensates the adsorption preference of ethane, resulting in a membrane permeation selectivity for ethene.
AbstractList	The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6bar feed pressure, respectively, with a selectivity of 2.8 and 2.4. Independent sorption uptake studies of an ethene/ethane mixture on a big ZIF-8 single crystal by IR microscopy detection show in combination with grand canonical Monte Carlo simulations that this moderate ethene selectivity of the ZIF-8 membrane can be explained by the interplay of a preferential ethane adsorption selectivity competing with a preferential ethene diffusion selectivity. This means, that ethane adsorbs stronger than ethene, but ethene diffuses faster and overcompensates the adsorption preference of ethane, resulting in a membrane permeation selectivity for ethene. [Display omitted] ▶ ZIF-8 membrane can separate ethene/ethane mixtures with selectivities between 2 and 3. ▶ From mixture adsorption and diffusion data, the membrane selectivity can be predicted. ▶ Both IR microscopy and grand canonical Monte Carlo simulation can give the mixture data. The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6 bar feed pressure, respectively, with a selectivity of 2.8 and 2.4. Independent sorption uptake studies of an ethene/ethane mixture on a big ZIF-8 single crystal by IR microscopy detection show in combination with grand canonical Monte Carlo simulations that this moderate ethene selectivity of the ZIF-8 membrane can be explained by the interplay of a preferential ethane adsorption selectivity competing with a preferential ethene diffusion selectivity. This means, that ethane adsorbs stronger than ethene, but ethene diffuses faster and overcompensates the adsorption preference of ethane, resulting in a membrane permeation selectivity for ethene. The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6 bar feed pressure, respectively, with a selectivity of 2.8 and 2.4. Independent sorption uptake studies of an ethene/ethane mixture on a big ZIF-8 single crystal by IR microscopy detection show in combination with grand canonical Monte Carlo simulations that this moderate ethene selectivity of the ZIF-8 membrane can be explained by the interplay of a preferential ethane adsorption selectivity competing with a preferential ethene diffusion selectivity. This means, that ethane adsorbs stronger than ethene, but ethene diffuses faster and overcompensates the adsorption preference of ethane, resulting in a membrane permeation selectivity for ethene.
Author	Bux, Helge Caro, Juergen Krishna, Rajamani Chmelik, Christian
Author_xml	– sequence: 1 givenname: Helge surname: Bux fullname: Bux, Helge organization: Institute of Physical Chemistry and Electrochemistry, Leibniz University Hannover, Callinstr. 3A, D-30167 Hannover, Germany – sequence: 2 givenname: Christian surname: Chmelik fullname: Chmelik, Christian organization: Faculty of Physics and Geosciences, Leipzig University, Linnéstr. 5, D-04103 Leipzig, Germany – sequence: 3 givenname: Rajamani surname: Krishna fullname: Krishna, Rajamani organization: Van’t Hoff Institute for Molecular Sciences, University of Amsterdam, Science Park 904, 1098 XH, Amsterdam, The Netherlands – sequence: 4 givenname: Juergen surname: Caro fullname: Caro, Juergen email: juergen.caro@pci.uni-hannover.de, caro@pci.uni-hannover.de organization: Institute of Physical Chemistry and Electrochemistry, Leibniz University Hannover, Callinstr. 3A, D-30167 Hannover, Germany
BackLink	http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=23897575$$DView record in Pascal Francis
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Snippet	[Display omitted] ▶ ZIF-8 membrane can separate ethene/ethane mixtures with selectivities between 2 and 3. ▶ From mixture adsorption and diffusion data, the... The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6bar feed pressure, respectively, with a... The newly developed MOF membrane ZIF-8 separates an equimolar ethene/ethane mixture at room temperature for 1 and 6 bar feed pressure, respectively, with a...
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SubjectTerms	adsorption ambient temperature artificial membranes Chemistry Colloidal state and disperse state ethane Ethene/ethane separation ethylene Exact sciences and technology GCMC simulations General and physical chemistry IR microscopy Membranes microscopy MOF membrane Monte Carlo method Surface physical chemistry ZIF-8 membrane
Title	Ethene/ethane separation by the MOF membrane ZIF-8: Molecular correlation of permeation, adsorption, diffusion
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